Doping-dependent phonon anomaly and charge-order phenomena in the HgBa 2 CuO 4 + δ and HgBa 2 CaCu 2 O 6 + δ superconductors

Wang, Lichen; Yu, Biqiong; Jing, Ran; Luo, Xiangpeng; Zeng, Junbang; Li, Jiarui; Bialo, Izabela; Bluschke, Martin; Tang, Yang; Freyermuth, Jacob; Yu, Guichuan; Sutarto, Ronny; He, Feizhou; Weschke, Eugen; Tabis, Wojciech; Greven, Martin; Li, Yuan

doi:10.1103/physrevb.101.220509

Doping-dependent phonon anomaly and charge-order phenomena in the ${HgBa}_{2} {CuO}_{4 + δ}$ and ${HgBa}_{2} {CaCu}_{2} O_{6 + δ}$ superconductors

Journal Article · Fri Jun 19 00:00:00 EDT 2020 · Physical Review B

DOI:https://doi.org/10.1103/physrevb.101.220509· OSTI ID:1656778

^[1]; Yu, Biqiong ^[2]; ^[3]; ^[3]; Zeng, Junbang ^[3]; ^[4]; ^[5]; Bluschke, Martin ^[6]; Tang, Yang ^[2]; Freyermuth, Jacob ^[2]; Yu, Guichuan ^[2]; Sutarto, Ronny ^[7]; He, Feizhou ^[7]; Weschke, Eugen ^[8]; ^[9]; Greven, Martin ^[2]; ^[10]

Peking Univ., Beijing (China); University of Minnesota
Univ. of Minnesota, Minneapolis, MN (United States)
Peking Univ., Beijing (China)
Peking Univ., Beijing (China); Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
AGH University of Science and Technology, Krakow (Poland); Technische Univ. Wien (Austria)
Max Planck Inst. for Solid State Research, Stuttgart (Germany); Helmholtz-Zentrum Berlin für Materialien und Energie, Berlin (Germany)
Canadian Light Sources, Inc., Saskatoon, SK (Canada)
Helmholtz-Zentrum Berlin für Materialien und Energie, Berlin (Germany)
Univ. of Minnesota, Minneapolis, MN (United States); AGH University of Science and Technology, Krakow (Poland); Technische Univ. Wien (Austria)
Peking Univ., Beijing (China); Collaborative Innovation Center of Quantum Matter, Beijing (China)

Using resonant x-ray diffraction and Raman spectroscopy, we study charge correlations and lattice dynamics in two model cuprates,

{HgBa}_{2} {CuO}_{4 + δ}

and

{HgBa}_{2} {CaCu}_{2} O_{6 + δ}

. We observe a maximum of the characteristic charge order temperature around the same hole concentration (p ≈ 0.09) in both compounds, and concomitant pronounced anomalies in the lattice dynamics that involve the motion of atoms in and/or adjacent to the CuO₂ layers. These anomalies are already present at room temperature, and therefore precede the formation of the static charge correlations, and we attribute them to an instability of the CuO₂ layers. Our finding implies that the charge order in the cuprates is an emergent phenomenon, driven by a fundamental variation in both lattice and electronic properties as a function of doping.

View Accepted Manuscript (DOE)

Research Organization:: Univ. of Minnesota, Minneapolis, MN (United States)

Sponsoring Organization:: Canadian Light Source; European Research Council (ERC); National Natural Science Foundation of China (NNSFC); National Science Center (NCN), Poland; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division

Grant/Contract Number:: SC0016371

OSTI ID:: 1656778

Journal Information:: Physical Review B, Journal Name: Physical Review B Journal Issue: 22 Vol. 101; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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