Low-voltage CMOS-free synaptic memory based on LiXTiO2 redox transistors.

Li, Yiyang; Fuller, Elliot James; Agarwal, Sapan; Talin, Albert Alec

doi:10.1021/acsami.9b14338

Low-voltage CMOS-free synaptic memory based on LiXTiO2 redox transistors.

Conference · Mon Apr 01 00:00:00 EDT 2019

DOI:https://doi.org/10.1021/acsami.9b14338· OSTI ID:1639895

Li, Yiyang; Fuller, Elliot James; Agarwal, Sapan; Talin, Albert Alec

Abstract not provided.

View Conference

Research Organization:: Energy Frontier Research Centers (EFRC) (United States). Nanostructures for Electrical Energy Storage (NEES); Sandia National Laboratories (SNL-CA), Livermore, CA (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA)

DOE Contract Number:: AC04-94AL85000

OSTI ID:: 1639895

Report Number(s):: SAND2019-4756C; 675071

Country of Publication:: United States

Language:: English

References (62)

Interfacial Challenges in Solid-State Li Ion Batteries Luntz, Alan C.; Voss, Johannes; Reuter, Karsten The Journal of Physical Chemistry Letters, Vol. 6, Issue 22 https://doi.org/10.1021/acs.jpclett.5b02352	journal	October 2015
Organic electronics for neuromorphic computing van de Burgt, Yoeri; Melianas, Armantas; Keene, Scott Tom Nature Electronics, Vol. 1, Issue 7 https://doi.org/10.1038/s41928-018-0103-3	journal	July 2018
All-Solid-State Synaptic Transistor with Ultralow Conductance for Neuromorphic Computing Yang, Chuan-Sen; Shang, Da-Shan; Liu, Nan Advanced Functional Materials, Vol. 28, Issue 42 https://doi.org/10.1002/adfm.201804170	journal	September 2018
Atomic Layer Deposition of the Solid Electrolyte Garnet Li ₇ La ₃ Zr ₂ O ₁₂ Kazyak, Eric; Chen, Kuan-Hung; Wood, Kevin N. Chemistry of Materials, Vol. 29, Issue 8 https://doi.org/10.1021/acs.chemmater.7b00944	journal	April 2017
SiGe epitaxial memory for neuromorphic computing with reproducible high performance based on engineered dislocations Choi, Shinhyun; Tan, Scott H.; Li, Zefan Nature Materials, Vol. 17, Issue 4 https://doi.org/10.1038/s41563-017-0001-5	journal	January 2018
Acceleration of Deep Neural Network Training with Resistive Cross-Point Devices: Design Considerations Gokmen, Tayfun; Vlasov, Yurii Frontiers in Neuroscience, Vol. 10 https://doi.org/10.3389/fnins.2016.00333	journal	July 2016
Memristive crossbar arrays for brain-inspired computing Xia, Qiangfei; Yang, J. Joshua Nature Materials, Vol. 18, Issue 4 https://doi.org/10.1038/s41563-019-0291-x	journal	March 2019
GGA + U description of lithium intercalation into anatase TiO 2 Morgan, Benjamin J.; Watson, Graeme W. Physical Review B, Vol. 82, Issue 14 https://doi.org/10.1103/PhysRevB.82.144119	journal	October 2010
Memristive devices for computing Yang, J. Joshua; Strukov, Dmitri B.; Stewart, Duncan R. Nature Nanotechnology, Vol. 8, Issue 1, p. 13-24 https://doi.org/10.1038/nnano.2012.240	journal	January 2013
A non-volatile organic electrochemical device as a low-voltage artificial synapse for neuromorphic computing van de Burgt, Yoeri; Lubberman, Ewout; Fuller, Elliot J. Nature Materials, Vol. 16, Issue 4 https://doi.org/10.1038/nmat4856	journal	February 2017
Ultrathin Conformable Organic Artificial Synapse for Wearable Intelligent Device Applications Jang, Sukjae; Jang, Seonghoon; Lee, Eun-Hye ACS Applied Materials & Interfaces, Vol. 11, Issue 1 https://doi.org/10.1021/acsami.8b12092	journal	December 2018
Review of memristor devices in neuromorphic computing: materials sciences and device challenges Li, Yibo; Wang, Zhongrui; Midya, Rivu Journal of Physics D: Applied Physics, Vol. 51, Issue 50 https://doi.org/10.1088/1361-6463/aade3f	journal	September 2018
A fully integrated reprogrammable memristor–CMOS system for efficient multiply–accumulate operations Cai, Fuxi; Correll, Justin M.; Lee, Seung Hwan Nature Electronics, Vol. 2, Issue 7 https://doi.org/10.1038/s41928-019-0270-x	journal	July 2019
Access devices for 3D crosspoint memory Burr, Geoffrey W.; Shenoy, Rohit S.; Virwani, Kumar Journal of Vacuum Science & Technology B, Nanotechnology and Microelectronics: Materials, Processing, Measurement, and Phenomena, Vol. 32, Issue 4 https://doi.org/10.1116/1.4889999	journal	July 2014
ECRAM as Scalable Synaptic Cell for High-Speed, Low-Power Neuromorphic Computing Tang, Jianshi; Bishop, Douglas; Kim, Seyoung 2018 IEEE International Electron Devices Meeting (IEDM) https://doi.org/10.1109/IEDM.2018.8614551	conference	December 2018
Electrochemical and Chemical Insertion for Energy Transformation and Switching Li, Yiyang; Chueh, William C. Annual Review of Materials Research, Vol. 48, Issue 1 https://doi.org/10.1146/annurev-matsci-070317-124525	journal	July 2018
Optimized pulsed write schemes improve linearity and write speed for low-power organic neuromorphic devices Keene, Scott T.; Melianas, Armantas; Fuller, Elliot J. Journal of Physics D: Applied Physics, Vol. 51, Issue 22 https://doi.org/10.1088/1361-6463/aabe70	journal	May 2018
Equilibrium lithium transport between nanocrystalline phases in intercalated TiO2 anatase Wagemaker, M.; Kentgens, A. P. M.; Mulder, F. M. Nature, Vol. 418, Issue 6896 https://doi.org/10.1038/nature00901	journal	July 2002
Energy Scaling Advantages of Resistive Memory Crossbar Based Computation and Its Application to Sparse Coding Agarwal, Sapan; Quach, Tu-Thach; Parekh, Ojas Frontiers in Neuroscience, Vol. 9 https://doi.org/10.3389/fnins.2015.00484	journal	January 2016
A single-transistor silicon synapse Diorio, C.; Hasler, P.; Minch, A. IEEE Transactions on Electron Devices, Vol. 43, Issue 11 https://doi.org/10.1109/16.543035	journal	January 1996
Fully Printed All-Solid-State Organic Flexible Artificial Synapse for Neuromorphic Computing Liu, Qingzhou; Liu, Yihang; Li, Ji ACS Applied Materials & Interfaces, Vol. 11, Issue 18 https://doi.org/10.1021/acsami.9b00226	journal	April 2019
Li-Ion Synaptic Transistor for Low Power Analog Computing Fuller, Elliot J.; Gabaly, Farid El; Léonard, François Advanced Materials, Vol. 29, Issue 4 https://doi.org/10.1002/adma.201604310	journal	November 2016
Understanding of proton induced synaptic behaviors in three-terminal synapse device for neuromorphic systems Lee, Jongwon; Lim, Seokjae; Kwak, Myonghoon Nanotechnology, Vol. 30, Issue 25 https://doi.org/10.1088/1361-6528/ab0b97	journal	April 2019
Emerging Artificial Synaptic Devices for Neuromorphic Computing Wan, Qingzhou; Sharbati, Mohammad T.; Erickson, John R. Advanced Materials Technologies, Vol. 4, Issue 4 https://doi.org/10.1002/admt.201900037	journal	February 2019
Neuromorphic computing using non-volatile memory Burr, Geoffrey W.; Shelby, Robert M.; Sebastian, Abu Advances in Physics: X, Vol. 2, Issue 1 https://doi.org/10.1080/23746149.2016.1259585	journal	October 2016
Synergies of Electrochemical Metallization and Valance Change in All-Inorganic Perovskite Quantum Dots for Resistive Switching Wang, Yan; Lv, Ziyu; Liao, Qiufan Advanced Materials, Vol. 30, Issue 28 https://doi.org/10.1002/adma.201800327	journal	May 2018
Glass-Type Polyamorphism in Li-Garnet Thin Film Solid State Battery Conductors Garbayo, Iñigo; Struzik, Michal; Bowman, William J. Advanced Energy Materials, Vol. 8, Issue 12 https://doi.org/10.1002/aenm.201702265	journal	January 2018
The crystal structures of the lithium-inserted metal oxides Li0.5TiO2 anatase, LiTi2O4 spinel, and Li2Ti2O4 Cava, R. J.; Murphy, D. W.; Zahurak, S. Journal of Solid State Chemistry, Vol. 53, Issue 1 https://doi.org/10.1016/0022-4596(84)90228-7	journal	June 1984
Quasi‐Hodgkin–Huxley Neurons with Leaky Integrate‐and‐Fire Functions Physically Realized with Memristive Devices Huang, He‐Ming; Yang, Rui; Tan, Zheng‐Hua Advanced Materials, Vol. 31, Issue 3 https://doi.org/10.1002/adma.201803849	journal	September 2018
Parallel programming of an ionic floating-gate memory array for scalable neuromorphic computing Fuller, Elliot J.; Keene, Scott T.; Melianas, Armantas Science, Vol. 364, Issue 6440 https://doi.org/10.1126/science.aaw5581	journal	April 2019
Nanoelectronic Programmable Synapses Based on Phase Change Materials for Brain-Inspired Computing Kuzum, Duygu; Jeyasingh, Rakesh G. D.; Lee, Byoungil Nano Letters, Vol. 12, Issue 5 https://doi.org/10.1021/nl201040y	journal	June 2011
Deep learning LeCun, Yann; Bengio, Yoshua; Hinton, Geoffrey Nature, Vol. 521, Issue 7553 https://doi.org/10.1038/nature14539	journal	May 2015
Orthorhombic distortion on Li intercalation in anatase Koudriachova, Marina V.; de Leeuw, Simon W.; Harrison, Nicholas M. Physical Review B, Vol. 69, Issue 5 https://doi.org/10.1103/PhysRevB.69.054106	journal	February 2004
Electron transport via polaron hopping in bulk Ti O 2 : A density functional theory characterization Deskins, N. Aaron; Dupuis, Michel Physical Review B, Vol. 75, Issue 19 https://doi.org/10.1103/PhysRevB.75.195212	journal	May 2007
The future of electronics based on memristive systems Zidan, Mohammed A.; Strachan, John Paul; Lu, Wei D. Nature Electronics, Vol. 1, Issue 1 https://doi.org/10.1038/s41928-017-0006-8	journal	January 2018
Multiscale Co-Design Analysis of Energy, Latency, Area, and Accuracy of a ReRAM Analog Neural Training Accelerator Marinella, Matthew J.; Agarwal, Sapan; Hsia, Alexander IEEE Journal on Emerging and Selected Topics in Circuits and Systems, Vol. 8, Issue 1 https://doi.org/10.1109/JETCAS.2018.2796379	journal	March 2018
All-Solid-State Synaptic Transistors with High-Temperature Stability Using Proton Pump Gating of Strongly Correlated Materials Oh, Chadol; Jo, Minguk; Son, Junwoo ACS Applied Materials & Interfaces, Vol. 11, Issue 17 https://doi.org/10.1021/acsami.9b00392	journal	April 2019
Nanoscale Solid State Batteries Enabled by Thermal Atomic Layer Deposition of a Lithium Polyphosphazene Solid State Electrolyte Pearse, Alexander J.; Schmitt, Thomas E.; Fuller, Elliot J. Chemistry of Materials, Vol. 29, Issue 8 https://doi.org/10.1021/acs.chemmater.7b00805	journal	April 2017
Ionic modulation and ionic coupling effects in MoS2 devices for neuromorphic computing Zhu, Xiaojian; Li, Da; Liang, Xiaogan Nature Materials, Vol. 18, Issue 2 https://doi.org/10.1038/s41563-018-0248-5	journal	December 2018
Raman investigation of the structural changes in anatase LixTiO2 upon electrochemical lithium insertion Baddour-Hadjean, Rita; Bach, Stéphane; Smirnov, Mikhail Journal of Raman Spectroscopy, Vol. 35, Issue 7 https://doi.org/10.1002/jrs.1200	journal	June 2004
Low-Power, Electrochemically Tunable Graphene Synapses for Neuromorphic Computing Sharbati, Mohammad Taghi; Du, Yanhao; Torres, Jorge Advanced Materials, Vol. 30, Issue 36 https://doi.org/10.1002/adma.201802353	journal	July 2018
Elucidating the Phase Transformation of Li ₄ Ti ₅ O ₁₂ Lithiation at the Nanoscale Verde, Michael G.; Baggetto, Loïc; Balke, Nina ACS Nano, Vol. 10, Issue 4 https://doi.org/10.1021/acsnano.5b07875	journal	March 2016
Training and operation of an integrated neuromorphic network based on metal-oxide memristors Prezioso, M.; Merrikh-Bayat, F.; Hoskins, B. D. Nature, Vol. 521, Issue 7550 https://doi.org/10.1038/nature14441	journal	May 2015
Role of Lithium Ordering in the Li _x TiO ₂ Anatase → Titanate Phase Transition Morgan, Benjamin J.; Watson, Graeme W. The Journal of Physical Chemistry Letters, Vol. 2, Issue 14 https://doi.org/10.1021/jz200718e	journal	June 2011
Understanding volumetric capacitance in conducting polymers Proctor, Christopher M.; Rivnay, Jonathan; Malliaras, George G. Journal of Polymer Science Part B: Polymer Physics, Vol. 54, Issue 15 https://doi.org/10.1002/polb.24038	journal	March 2016
Anatomy of Ag/Hafnia-Based Selectors with 10 ¹⁰ Nonlinearity Midya, Rivu; Wang, Zhongrui; Zhang, Jiaming Advanced Materials, Vol. 29, Issue 12 https://doi.org/10.1002/adma.201604457	journal	January 2017
Reliable reference electrodes for lithium-ion batteries La Mantia, F.; Wessells, C. D.; Deshazer, H. D. Electrochemistry Communications, Vol. 31 https://doi.org/10.1016/j.elecom.2013.03.015	journal	June 2013
A low ride on processing temperature for fast lithium conduction in garnet solid-state battery films Pfenninger, Reto; Struzik, Michal; Garbayo, Iñigo Nature Energy, Vol. 4, Issue 6 https://doi.org/10.1038/s41560-019-0384-4	journal	May 2019
Ferroelectric Analog Synaptic Transistors Kim, Min-Kyu; Lee, Jang-Sik Nano Letters, Vol. 19, Issue 3 https://doi.org/10.1021/acs.nanolett.9b00180	journal	January 2019
Electrical and optical properties of TiO2 in accumulation and of lithium titanate Li0.5TiO2 van de Krol, Roel; Goossens, Albert; Meulenkamp, Eric A. Journal of Applied Physics, Vol. 90, Issue 5 https://doi.org/10.1063/1.1388165	journal	September 2001
Defect Chemistry, Surface Structures, and Lithium Insertion in Anatase TiO ₂ Olson, Carol L.; Nelson, Jenny; Islam, M. Saiful The Journal of Physical Chemistry B, Vol. 110, Issue 20 https://doi.org/10.1021/jp057261l	journal	May 2006
Neuromorphic Computing: Ion Gated Synaptic Transistors Based on 2D van der Waals Crystals with Tunable Diffusive Dynamics (Adv. Mater. 21/2018) Zhu, Jiadi; Yang, Yuchao; Jia, Rundong Advanced Materials, Vol. 30, Issue 21 https://doi.org/10.1002/adma.201870149	journal	May 2018
Electronic structure of lithium-doped anatase Ti O 2 prepared in ultrahigh vacuum Richter, J. H.; Henningsson, A.; Karlsson, P. G. Physical Review B, Vol. 71, Issue 23 https://doi.org/10.1103/PhysRevB.71.235418	journal	June 2005
Electrochemically Driven Phase Transitions in Insertion Electrodes for Lithium-Ion Batteries: Examples in Lithium Metal Phosphate Olivines Tang, Ming; Carter, W. Craig; Chiang, Yet-Ming Annual Review of Materials Research, Vol. 40, Issue 1 https://doi.org/10.1146/annurev-matsci-070909-104435	journal	June 2010
Phase separation and charge localization in UHV-lithiated anatase Ti O 2 nanoparticles Richter, J. H.; Henningsson, A.; Sanyal, B. Physical Review B, Vol. 71, Issue 23 https://doi.org/10.1103/PhysRevB.71.235419	journal	June 2005
Kinetics of Anatase Electrodes: The Role of Ordering, Anisotropy, and Shape Memory Effects Belak, Anna A.; Wang, Yizhou; Van der Ven, Anton Chemistry of Materials, Vol. 24, Issue 15 https://doi.org/10.1021/cm300881t	journal	July 2012
Memristors with diffusive dynamics as synaptic emulators for neuromorphic computing Wang, Zhongrui; Joshi, Saumil; Savel’ev, Sergey E. Nature Materials, Vol. 16, Issue 1 https://doi.org/10.1038/nmat4756	journal	September 2016
From biomaterial-based data storage to bio-inspired artificial synapse Lv, Ziyu; Zhou, Ye; Han, Su-Ting Materials Today, Vol. 21, Issue 5 https://doi.org/10.1016/j.mattod.2017.12.001	journal	June 2018
Fully memristive neural networks for pattern classification with unsupervised learning Wang, Zhongrui; Joshi, Saumil; Savel’ev, Sergey Nature Electronics, Vol. 1, Issue 2 https://doi.org/10.1038/s41928-018-0023-2	journal	February 2018
Atomic and Electronic Bulk versus Surface Structure: Lithium Intercalation in Anatase TiO ₂ Wagemaker, M.; Lützenkirchen-Hecht, D.; van Well, A. A. The Journal of Physical Chemistry B, Vol. 108, Issue 33 https://doi.org/10.1021/jp048567f	journal	August 2004
Fabrication, Testing, and Simulation of All-Solid-State Three-Dimensional Li-Ion Batteries Talin, A. Alec; Ruzmetov, Dmitry; Kolmakov, Andrei ACS Applied Materials & Interfaces, Vol. 8, Issue 47 https://doi.org/10.1021/acsami.6b12244	journal	November 2016
Equivalent-accuracy accelerated neural-network training using analogue memory Ambrogio, Stefano; Narayanan, Pritish; Tsai, Hsinyu Nature, Vol. 558, Issue 7708 https://doi.org/10.1038/s41586-018-0180-5	journal	June 2018

Cited By (2)

Near ideal synaptic functionalities in Li ion synaptic transistor using Li3POxSex electrolyte with high ionic conductivity Nikam, Revannath Dnyandeo; Kwak, Myonghoon; Lee, Jongwon Scientific Reports, Vol. 9, Issue 1 https://doi.org/10.1038/s41598-019-55310-8	journal	December 2019
Controlled Ionic Tunneling in Lithium Nanoionic Synaptic Transistor through Atomically Thin Graphene Layer for Neuromorphic Computing Nikam, Revannath Dnyandeo; Kwak, Myonghoon; Lee, Jongwon Advanced Electronic Materials, Vol. 6, Issue 2 https://doi.org/10.1002/aelm.201901100	journal	December 2019

Similar Records

Analog redox memory based on electrochemical ion insertion.

Conference · Sun Sep 01 00:00:00 EDT 2019 · OSTI ID:1641918

Lithium ion synaptic transistor for analog computation (LISTA).

Conference · Sun May 01 00:00:00 EDT 2016 · OSTI ID:1368863

Non-volatile redox transistors for analog low power computing.

Conference · Thu Jun 01 00:00:00 EDT 2017 · OSTI ID:1458221

Low-voltage CMOS-free synaptic memory based on LiXTiO2 redox transistors.

Citation Formats

References (62)

Cited By (2)

Similar Records

Related Subjects