High resolution time- and angle-resolved photoemission spectroscopy with 11 eV laser pulses

Lee, Changmin; Rohwer, Timm; Sie, Edbert J.; Zong, Alfred; Baldini, Edoardo; Straquadine, Joshua; Walmsley, Philip; Gardner, Dillon; Lee, Young S.; Fisher, Ian R.; Gedik, Nuh

doi:10.1063/1.5139556

High resolution time- and angle-resolved photoemission spectroscopy with 11 eV laser pulses

Journal Article · Thu Apr 09 00:00:00 EDT 2020 · Review of Scientific Instruments

DOI:https://doi.org/10.1063/1.5139556· OSTI ID:1616758

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Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States). Materials Sciences Division
Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States); Deutsches Elektronen-Synchrotron (DESY), Hamburg (Germany). Center for Free-Electron Laser Science
Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States); Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials
Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)
Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials; SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES)
Stanford Univ., CA (United States). Geballe Lab. for Advanced Materials; SLAC National Accelerator Lab., Menlo Park, CA (United States). Stanford Institute for Materials and Energy Science (SIMES); Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)

Performing time- and angle-resolved photoemission (tr-ARPES) spectroscopy at high momenta necessitates extreme ultraviolet laser pulses, which are typically produced via high harmonic generation (HHG). Despite current advances, HHG-based setups still require large pulse energies (from hundreds of μJ to mJ) and their energy resolution is limited to tens of meV. Here, we present a novel 11 eV tr-ARPES setup that generates a flux of 5 × 10¹⁰ photons/s and achieves an unprecedented energy resolution of 16 meV. It can be operated at high repetition rates (up to 250 kHz) while using input pulse energies down to 3 µJ. We demonstrate these unique capabilities by simultaneously capturing the energy and momentum resolved dynamics in two well-separated momentum space regions of a charge density wave material ErTe₃. This novel setup provides the opportunity to study the non-equilibrium band structure of solids with exceptional energy and time resolutions at high repetition rates.

View Accepted Manuscript (DOE)

Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States); Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); Gordon and Betty Moore Foundation; Army Research Office (ARO); Swiss National Science Foundation

Grant/Contract Number:: FG02-08ER46521; AC02-76SF00515

OSTI ID:: 1616758

Alternate ID(s):: OSTI ID: 1616480

Journal Information:: Review of Scientific Instruments, Journal Name: Review of Scientific Instruments Journal Issue: 4 Vol. 91; ISSN 0034-6748

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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