Extreme ultraviolet time- and angle-resolved photoemission setup with 21.5 meV resolution using high-order harmonic generation from a turn-key Yb:KGW amplifier

Liu, Yangyang; Beetar, John E.; Hosen, Md Mofazzel; Dhakal, Gyanendra; Sims, Christopher; Kabir, Firoza; Etienne, Marc B.; Dimitri, Klauss; Regmi, Sabin; Liu, Yong; Pathak, Arjun K.; Kaczorowski, Dariusz; Neupane, Madhab; Chini, Michael

doi:10.1063/1.5121425

Extreme ultraviolet time- and angle-resolved photoemission setup with 21.5 meV resolution using high-order harmonic generation from a turn-key Yb:KGW amplifier

Journal Article · Mon Jan 06 00:00:00 EST 2020 · Review of Scientific Instruments

DOI:https://doi.org/10.1063/1.5121425· OSTI ID:1581205

Liu, Yangyang; Beetar, John E.; Hosen, Md Mofazzel; Dhakal, Gyanendra; Sims, Christopher; Kabir, Firoza; Etienne, Marc B.; Dimitri, Klauss; ; Liu, Yong; Pathak, Arjun K.; ; Neupane, Madhab;

Characterizing and controlling electronic properties of quantum materials require direct measurements of nonequilibrium electronic band structures over large regions of momentum space. Here, we demonstrate an experimental apparatus for time- and angle-resolved photoemission spectroscopy using high-order harmonic probe pulses generated by a robust, moderately high power (20 W) Yb:KGW amplifier with a tunable repetition rate between 50 and 150 kHz. By driving high-order harmonic generation (HHG) with the second harmonic of the fundamental 1025 nm laser pulses, we show that single-harmonic probe pulses at 21.8 eV photon energy can be effectively isolated without the use of a monochromator. The on-target photon flux can reach 5 × 1010 photons/s at 50 kHz, and the time resolution is measured to be 320 fs. The relatively long pulse duration of the Yb-driven HHG source allows us to reach an excellent energy resolution of 21.5 meV, which is achieved by suppressing the space-charge broadening using a low photon flux of 1.5 × 108 photons/s at a higher repetition rate of 150 kHz. The capabilities of the setup are demonstrated through measurements in the topological semimetal ZrSiS and the topological insulator Sb2−xGdxTe3.

View Accepted Manuscript (Publisher)

Sponsoring Organization:: USDOE

Grant/Contract Number:: AC02-07CH11358

OSTI ID:: 1581205

Journal Information:: Review of Scientific Instruments, Journal Name: Review of Scientific Instruments Journal Issue: 1 Vol. 91; ISSN 0034-6748

Publisher:: American Institute of PhysicsCopyright Statement

Country of Publication:: United States

Language:: English

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