Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Standing Waves Induced by Valley-Mismatched Domains in Ferroelectric SnTe Monolayers

Journal Article · · Physical Review Letters
 [1];  [2];  [3];  [4];  [3];  [2];  [4];  [4];  [5]
  1. Tsinghua Univ., Beijing (China); Max-Planck Inst. of Microstructure Physics, Halle (Germany); Collaborative Innovation Center of Quantum Matter, Beijing (China); DOE/OSTI
  2. Univ. of Arkansas, Fayetteville, AR (United States)
  3. Max-Planck Inst. of Microstructure Physics, Halle (Germany)
  4. Tsinghua Univ., Beijing (China); Collaborative Innovation Center of Quantum Matter, Beijing (China)
  5. Tsinghua Univ., Beijing (China); Collaborative Innovation Center of Quantum Matter, Beijing (China); RIKEN Center for Emergent Matter Science (CEMS)-Wako, Saitama (Japan)
Two-dimensional (2D) quasiparticle standing waves originate from the interference of coherent quantum states and are usually created by the scattering off edges, atomic steps, or adatoms that induce large potential barriers. We report standing waves close to the valence band maximum (EV), confined by electrically neutral domain walls of newly discovered ferroelectric SnTe monolayers, as revealed by spatially resolved scanning tunneling spectroscopy. Ab initio calculations show that this novel confinement arises from the polarization lifted hole valley degeneracy and a ~90° rotation of the Brillouin zones that render holes’ momentum mismatched across neighboring domains. These results show a potential for polarization-tuned valleytronics in 2D ferroelectrics.
Research Organization:
Univ. of Arkansas, Fayetteville, AR (United States)
Sponsoring Organization:
National Natural Science Foundation of China; USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
SC0016139
OSTI ID:
1612402
Alternate ID(s):
OSTI ID: 1515593
Journal Information:
Physical Review Letters, Journal Name: Physical Review Letters Journal Issue: 20 Vol. 122; ISSN 0031-9007
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

References (40)

Enhanced Spontaneous Polarization in Ultrathin SnTe Films with Layered Antipolar Structure journal September 2018
Out-of-Plane Piezoelectricity and Ferroelectricity in Layered α-In 2 Se 3 Nanoflakes journal August 2017
Intercorrelated In-Plane and Out-of-Plane Ferroelectricity in Ultrathin Two-Dimensional Layered Semiconductor In 2 Se 3 journal January 2018
Quantum mirages formed by coherent projection of electronic structure journal February 2000
Two-dimensional ferroelectric films journal February 1998
Imaging standing waves in a two-dimensional electron gas journal June 1993
Transmission of topological surface states through surface barriers journal July 2010
Room-temperature ferroelectricity in CuInP2S6 ultrathin flakes journal August 2016
Electrical spin injection and detection in molybdenum disulfide multilayer channel journal April 2017
Ferroelectric switching of a two-dimensional metal journal July 2018
Piezoelectric response of epitaxial Pb(Zr0.2Ti0.8)O3 films measured by scanning tunneling microscopy journal September 2000
Nanoscale polarization manipulation and conductance switching in ultrathin films of a ferroelectric copolymer journal June 2003
Direct observation of ferroelectric polarization-modulated band bending at oxide interfaces journal March 2012
The SIESTA method for ab initio order- N materials simulation journal March 2002
On-site approximation for spin–orbit coupling in linear combination of atomic orbitals density functional methods journal August 2006
On-site approximation for spin–orbit coupling in linear combination of atomic orbitals density functional methods journal November 2007
Ultrathin BaTiO 3 templates for multiferroic nanostructures journal August 2011
Special points for Brillouin-zone integrations journal June 1976
Efficient pseudopotentials for plane-wave calculations journal January 1991
Numerical atomic orbitals for linear-scaling calculations journal November 2001
Power-law decay of standing waves on the surface of topological insulators journal December 2011
Scattering of surface electrons by isolated steps versus periodic step arrays journal March 2013
Interpretation of van der Waals density functionals journal August 2014
Phosphorene analogues: Isoelectronic two-dimensional group-IV monochalcogenides with orthorhombic structure journal August 2015
Valley physics in tin (II) sulfide journal January 2016
Polarization and valley switching in monolayer group-IV monochalcogenides journal July 2016
Efficient Implementation of a van der Waals Density Functional: Application to Double-Wall Carbon Nanotubes journal August 2009
Experimental Demonstration of Topological Surface States Protected by Time-Reversal Symmetry journal December 2009
Spin Relaxation in Single-Layer and Bilayer Graphene journal July 2011
Structural Phase Transition and Material Properties of Few-Layer Monochalcogenides journal December 2016
Intrinsic Two-Dimensional Ferroelectricity with Dipole Locking journal May 2018
Direct observation of standing wave formation at surface steps using scanning tunneling spectroscopy journal August 1993
Confinement of Surface State Electrons in Fabry-Perot Resonators journal December 1998
Probing Hot-Electron Dynamics at Surfaces with a Cold Scanning Tunneling Microscope journal May 1999
Colloquium: Theory of quantum corrals and quantum mirages journal July 2003
Confinement of Electrons to Quantum Corrals on a Metal Surface journal October 1993
Observation of Quantum-Size Effects at Room Temperature on Metal Surfaces With STM journal May 1994
Discovery of robust in-plane ferroelectricity in atomic-thick SnTe journal July 2016
Transmission of topological surface states through surface barriers text January 2010
Ultrathin BaTiO3 templates for multiferroic nanostructures text January 2011

Cited By (3)

The rise of 2D dielectrics/ferroelectrics journal December 2019
Emergence of the giant out-of-plane Rashba effect and tunable nanoscale persistent spin helix in ferroelectric SnTe thin films journal January 2020
Group-IV monochalcogenide monolayers: Two-dimensional ferroelectrics with weak intralayer bonds and a phosphorenelike monolayer dissociation energy journal December 2019