Magnetic structure of Nd in NdFeAsO studied by x-ray resonant magnetic scattering
Journal Article
·
· Physical Review B
- Rutgers Univ., Piscataway, NJ (United States). Dept. of Physics and Astronomy; Ames Lab., and Iowa State Univ., Ames, IA (United States). Dept. of Physics and Astronomy
- Argonne National Lab. (ANL), Argonne, IL (United States). Advanced Photon Source (APS)
- Ames Lab., and Iowa State Univ., Ames, IA (United States). Dept. of Physics and Astronomy; Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science and Technology Division
- Ames Lab., and Iowa State Univ., Ames, IA (United States). Dept. of Physics and Astronomy
The magnetic structure of Nd in NdFeAsO compound has been explored by x-ray resonant magnetic scattering at the Nd edge ( keV) at K. At K we find that the Nd moments are aligned along the crystallographic direction with the (1, 0, 0) propagation vector, and are arranged antiferromagnetically along the direction and ferromagnetically along the and directions. At K, we observe an unusual temperature dependence of the magnetic Bragg peaks that appear differently at and . From the changes of magnetic intensities and our representation analysis, we find that the Nd moments are reoriented toward the direction with a gradual decrease of the moment component in the direction with increasing temperature. We postulate that the reorientation of the Nd moment is due to a strong interplay with the Fe moment which is fully ordered in this temperature range.
- Research Organization:
- Argonne National Laboratory (ANL), Argonne, IL (United States); Iowa State Univ., Ames, IA (United States); Rutgers Univ., Piscataway, NJ (United States)
- Sponsoring Organization:
- USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22). Materials Sciences & Engineering Division
- Grant/Contract Number:
- AC02-06CH11357; AC02-07CH11358; FG02-07ER46382
- OSTI ID:
- 1607450
- Journal Information:
- Physical Review B, Journal Name: Physical Review B Journal Issue: 22 Vol. 100; ISSN 2469-9950; ISSN PRBMDO
- Publisher:
- American Physical Society (APS)Copyright Statement
- Country of Publication:
- United States
- Language:
- English
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