Optimizing hybrid rotational femtosecond/picosecond coherent anti-Stokes Raman spectroscopy in nitrogen at high pressures and temperatures

Torge Mecker, Nils; Courtney, Trevor L.; Patterson, Brian D.; Escofet-Martin, David; Peterson, Brian; Kliewer, Christopher J.; Linne, Mark

doi:10.1364/JOSAB.383575

Title: Optimizing hybrid rotational femtosecond/picosecond coherent anti-Stokes Raman spectroscopy in nitrogen at high pressures and temperatures

Journal Article · Thu Mar 12 00:00:00 EDT 2020 · Journal of the Optical Society of America. Part B, Optical Physics

DOI:https://doi.org/10.1364/JOSAB.383575· OSTI ID:1603833

; Courtney, Trevor L.; Patterson, Brian D.; Escofet-Martin, David; Peterson, Brian; Kliewer, Christopher J.; Linne, Mark

We demonstrate the use of hybrid rotational femtosecond/picosecond (fs/ps) coherent anti-Stokes Raman spectroscopy (HR-CARS) as a technique for temperature measurements in nitrogen gas at high pressures and temperatures. A broadband pulse shaper-adjusted 42 fs pulse interacts with a narrow-bandwidth, frequency-upconverted 5.5 ps pulse in a cell containing $N_{2}$ at pressures of 1–70 atm and temperatures of 300–1000 K. A computational code is used to model spectra and fit experimental results to obtain best-fit temperatures. We demonstrate good qualitative fits as well as good accuracy and precision between thermocouple measured and best-fit temperatures over the explored pressure and temperature regimes. The overall average percentage temperature difference between thermocouple measurements and best-fit temperatures is $- <#comment/> 0.3 % <#comment/>$ with a standard deviation of 7.1%, showing the suitability of HR-CARS for characterizing high-pressure and -temperature environments.

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Sponsoring Organization:: USDOE

OSTI ID:: 1603833

Journal Information:: Journal of the Optical Society of America. Part B, Optical Physics, Journal Name: Journal of the Optical Society of America. Part B, Optical Physics Vol. 37 Journal Issue: 4; ISSN 0740-3224

Publisher:: Optical Society of AmericaCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 6 works

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References (34)

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