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Coprecipitation of {sup 152}Eu with Iron(III) hydroxide formed upon reduction of sodium ferrate(VI) in aqueous medium

Journal Article · · Radiochemistry
OSTI ID:160278
;  [1]
  1. St. Petersburg State Agricultural Univ. (Russian Federation)
The results are presented on coprecipitation of {sup 152}Eu with iron(III) hydroxide formed either upon hydrolysis of Fe(III) sulfate or upon spontaneous reduction of sodium ferrate(VI) (Na{sub 4}FeO{sub 5}) by water with pH variation from 2.5 to 12 and constant ionic strength I=1. Iron(III) hydroxide formed according to the second mechanism has more developed surface and coprecipitates with Eu{sup 3+} more efficiently, especially when concentration of Fe(III) is low({approx}1.2 mg 1{sup -1} or 2.2x10{sup -5} M). Introduction of oxalate ions (C=6.7x10{sup -4} M) into the solution inhibits the coprecipitation of Eu{sup 3+}; however, oxalate is readily oxidized by ferrate ion, which in this case additionally favors sorption using ferrate. Tentative data on coprecipitation of {sup 242}Pu and {sup 241}Am with Fe(OH){sub 3} produced from ferrate are presented. The data obtained show that sodium ferrate may be useful for decontamination of liquid radioactive wastes, because only ozone is a stronger oxidant than sodium ferrate (among common oxidants) and sodium ferrate is one of the best coagulating agents.
OSTI ID:
160278
Journal Information:
Radiochemistry, Journal Name: Radiochemistry Journal Issue: 4 Vol. 37; ISSN RDIOEO; ISSN 1066-3622
Country of Publication:
United States
Language:
English

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