Schalten in Metall‐organischen Gerüsten

Bigdeli, Fahime; Lollar, Christina T.; Morsali, Ali; Zhou, Hong‐Cai

doi:10.1002/ange.201900666

Schalten in Metall‐organischen Gerüsten

Journal Article · Mon Dec 02 00:00:00 EST 2019 · Angewandte Chemie

DOI:https://doi.org/10.1002/ange.201900666· OSTI ID:1576806

Bigdeli, Fahime ^[1]; ^[2]; Morsali, Ali ^[1]; ^[3]

Department of Chemistry Faculty of Sciences Tarbiat Modares University P.O. Box 14155-4838 Teheran Iran
Department of Chemistry Texas A&,M University College Station TX 77843 USA
Department of Chemistry Texas A&,M University College Station TX 77843 USA, Department of Materials Science and Engineering Texas A&,M University College Station TX 77843 USA

Abstract

Aufgrund ihrer einstellbaren Poren und nahezu grenzenlosen Strukturdiversität, die sich aus dem Design verschiedener organischer Linker und metallischer Strukturbaueinheiten ableitet, haben sich Metall‐organische Gerüste (MOFs) in den vergangenen Jahren zu einem intensiv beforschten Gebiet entwickelt. Zu den größten Aufgaben gehören schaltbare MOFs und ihre Anwendung. Schaltbare MOFs sind “intelligente” Materialien, die bei Exposition gegenüber externen Stimuli eine deutliche, reversible, chemische Veränderung ihrer Struktur durchlaufen, was interessante technische Anwendungen ermöglicht. Obwohl dieser Prozess des Schaltens Ähnlichkeiten mit Flexibilität aufweist, haben sich nur sehr wenige Studien speziell mit Schalten beschäftigt, wohingegen sich eine recht große Zahl von Arbeiten und Übersichten mit der Flexibilität in MOFs beschäftigt. Dieser Aufsatz konzentriert sich auf die Eigenschaften und das allgemeine Design schaltbarer MOFs. Dabei wird die Schaltaktivität basierend auf der Ursache des Schaltens beschrieben: Licht, Spincrossover, Redoxchemie, Temperatur und Benetzbarkeit.

View Accepted Manuscript (Publisher)

Sponsoring Organization:: USDOE

Grant/Contract Number:: SC0001015

OSTI ID:: 1576806

Journal Information:: Angewandte Chemie, Journal Name: Angewandte Chemie Journal Issue: 12 Vol. 132; ISSN 0044-8249

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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Microwave-assisted crystallization inclusion of spiropyran molecules in indium trimesate films with antidromic reversible photochromism Zhang, Feng; Zou, Xiaoqin; Feng, Wei Journal of Materials Chemistry, Vol. 22, Issue 48 https://doi.org/10.1039/c2jm34618d	journal	January 2012
Photo-responsive MOFs: light-induced switching of porous single crystals containing a photochromic diarylethene Walton, Ian M.; Cox, Jordan M.; Coppin, Jarrett A. Chemical Communications, Vol. 49, Issue 73 https://doi.org/10.1039/c3cc44119a	journal	January 2013
Photophysical pore control in an azobenzene-containing metal–organic framework Brown, Jonathan W.; Henderson, Bryana L.; Kiesz, Matthew D. Chemical Science, Vol. 4, Issue 7 https://doi.org/10.1039/c3sc21659d	journal	January 2013
Electrochemically addressable trisradical rotaxanes organized within a metal–organic framework McGonigal, Paul R.; Deria, Pravas; Hod, Idan Proceedings of the National Academy of Sciences, Vol. 112, Issue 36 https://doi.org/10.1073/pnas.1514485112	journal	August 2015
Recent progress in the synthesis of metal–organic frameworks Sun, Yujia; Zhou, Hong-Cai Science and Technology of Advanced Materials, Vol. 16, Issue 5 https://doi.org/10.1088/1468-6996/16/5/054202	journal	October 2015
Pressure and Temperature Control of Spin-Switchable Metal-Organic Coordination Polymers from Ab Initio Calculations Tarafder, K.; Kanungo, S.; Oppeneer, P. M. Physical Review Letters, Vol. 109, Issue 7 https://doi.org/10.1103/PhysRevLett.109.077203	journal	August 2012
Mechanized azobenzene-functionalized zirconium metal-organic framework for on-command cargo release Meng, Xiangshi; Gui, Bo; Yuan, Daqiang Science Advances, Vol. 2, Issue 8 https://doi.org/10.1126/sciadv.1600480	journal	August 2016
On/off switchable electronic conduction in intercalated metal-organic frameworks Ogihara, Nobuhiro; Ohba, Nobuko; Kishida, Yoshihiro Science Advances, Vol. 3, Issue 8 https://doi.org/10.1126/sciadv.1603103	journal	August 2017

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