Influence of Emissions and Aqueous Processing on Particles Containing Black Carbon in a Polluted Urban Environment: Insights From a Soot Particle-Aerosol Mass Spectrometer

Collier, Sonya; Williams, Leah R.; Onasch, Timothy B.; Cappa, Christopher D.; Zhang, Xiaolu; Russell, Lynn M.; Chen, Chia-Li; Sanchez, Kevin J.; Worsnop, Douglas R.; Zhang, Qi

doi:10.1002/2017jd027851

Title: Influence of Emissions and Aqueous Processing on Particles Containing Black Carbon in a Polluted Urban Environment: Insights From a Soot Particle-Aerosol Mass Spectrometer

Journal Article · Wed Feb 21 00:00:00 EST 2018 · Journal of Geophysical Research: Atmospheres

DOI:https://doi.org/10.1002/2017jd027851· OSTI ID:1537325

^[1]; Williams, Leah R. ^[2];

^[2];

^[1]; Zhang, Xiaolu ^[1];

^[3];

^[3]; Worsnop, Douglas R. ^[2];

^[1]

Univ. of California, Davis, CA (United States)
Aerodyne Research, Inc., Billerica, MA (United States)
Univ. of California, San Diego, CA (United States). Scripps Inst. of Oceanography

Abstract Inorganic and organic coatings on black carbon (BC) particles can enhance light absorption and affect atmospheric lifetimes of BC‐containing particles and thus have significant implications for climate. To study the physical and chemical characteristics of atmospheric BC and BC‐associated coatings, a soot particle‐aerosol mass spectrometer was deployed during the winter of 2014–2015 in Fresno, a city located in the San Joaquin Valley of California, to selectively analyze BC‐containing particles. Comparing soot particle‐aerosol mass spectrometer measurements to those from the collocated single‐particle soot photometer (SP2) and high‐resolution aerosol mass spectrometer, we found that 17% of total submicrometer aerosol mass was associated with BC‐containing particles, suggesting that a majority of the fine particles in Fresno contained no BC. Most BC‐containing particles appeared to be associated with residential wood burning and vehicular traffic. These particles typically had a bulk‐average mass ratio of coating to BC ( R _coat/rBC ) less than 2. However, during periods of persistent fog larger R _coat/rBC values were observed, with the coatings primarily composed of secondary inorganic and organic components that likely resulted from aqueous‐phase processing. Specifically, compared to periods with less fog, the BC coating increased in concentration and contained a larger fraction of nitrate and oxidized organic matter. The size distributions of BC and associated organic coating were generally centered around 300 nm in vacuum aerodynamic diameter. However, during foggy periods BC had an additional peak at ~400 nm and organics and nitrate displayed a prominent mode in the accumulation size range.

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Research Organization:: Aerodyne Research, Inc., Billerica, MA (United States); Univ. of California, Davis, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: FG02-07ER84890; SC0014620; DE‐SC0014620; DE‐FG02‐07ER84890

OSTI ID:: 1537325

Alternate ID(s):: OSTI ID: 1457592

Journal Information:: Journal of Geophysical Research: Atmospheres, Vol. 123, Issue 12; ISSN 2169-897X

Publisher:: American Geophysical UnionCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 30 works

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Organic PM Emissions from Vehicles: Composition, O/C Ratio, and Dependence on PM Concentration Collier, Sonya; Zhou, Shan; Kuwayama, Toshihiro Taylor & Francis https://doi.org/10.6084/m9.figshare.1285021.v2	text	January 2015
Mexico city aerosol analysis during MILAGRO using high resolution aerosol mass spectrometry at the urban supersite (T0) - Part 2: Analysis of the biomass burning contribution and the non-fossil carbon fraction Wiedinmyer, C.; Zheng, J.; Volkamer, R. European Geosciences Union https://doi.org/10.7892/boris.5173	text	January 2010

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