Source apportionment of soot particles and aqueous-phase processing of black carbon coatings in an urban environment

Farley, Ryan N.; Collier, Sonya; Cappa, Christopher D.; Williams, Leah R.; Onasch, Timothy B.; Russell, Lynn M.; Kim, Hwajin; Zhang, Qi

doi:10.5194/acp-23-15039-2023

Title: Source apportionment of soot particles and aqueous-phase processing of black carbon coatings in an urban environment

Journal Article · Thu Dec 07 00:00:00 EST 2023 · Atmospheric Chemistry and Physics (Online)

DOI:https://doi.org/10.5194/acp-23-15039-2023· OSTI ID:2229017

Farley, Ryan N.; Collier, Sonya;

; Williams, Leah R.;

;

; Kim, Hwajin;

The impacts of soot particles on climate and human health depend on the concentration of black carbon (BC) as well as the thickness and composition of the coating material, i.e., organic and inorganic compounds internally mixed with BC. In this study, the size-resolved chemical composition of BC-containing aerosol was measured using a high-resolution soot particle aerosol mass spectrometer (SP-AMS) during wintertime in Fresno, California, a location influenced by abundant combustion emissions and frequent fog events. Concurrently, particle optical properties were measured to investigate the BC absorption enhancement. Positive matrix factorization (PMF) analysis was performed on the SP-AMS mass spectral measurements to explore the sources of soot particles and the atmospheric processes affecting the properties of BC coatings. The analysis revealed that residential woodburning and traffic are the dominant sources of soot particles. Alongside primary soot particles originating from biomass burning (BBOA_BC) and vehicles (HOA_BC) two distinct types of processed BC-containing aerosol were identified: fog-related oxidized organic aerosol (FOOA_BC) and winter-background OOA_BC (WOOA_BC). Both types of OOA_BC showed evidence of having undergone aqueous processing, albeit with differences. The concentration of FOOA_BC was substantially elevated during fog events, indicating the formation of aqueous secondary organic aerosol (aqSOA) within fog droplets. On the other hand, WOOA_BC was present at a relatively consistent concentration throughout the winter and was likely related to the formation of secondary organic aerosol (SOA) in both the gas phase and aerosol liquid water. By comparing the chemical properties and temporal variations in FOOA_BC and WOOA_BC, we gain insights into the key aging processes of BC aerosol. It was found that aqueous-phase reactions facilitated by fog droplets had a significant impact on the thickness and chemical composition of BC coatings, thereby affecting the light absorption and hygroscopic properties of soot particles. These findings underscore the important role of chemical reactions occurring within clouds and fogs and influencing the climate forcing of BC aerosol in the atmosphere

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Atmospheric Radiation Measurement (ARM) Data Center; Univ. of California, Davis, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Biological and Environmental Research (BER); California Air Resources Board

Contributing Organization:: PNNL, BNL, ANL, ORNL

Grant/Contract Number:: SC0022140; SC0020182; 13-330

OSTI ID:: 2229017

Alternate ID(s):: OSTI ID: 2279037

Journal Information:: Atmospheric Chemistry and Physics (Online), Journal Name: Atmospheric Chemistry and Physics (Online) Vol. 23 Journal Issue: 23; ISSN 1680-7324

Publisher:: Copernicus GmbHCopyright Statement

Country of Publication:: Germany

Language:: English

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