All-Printed, Stretchable Zn-Ag2O Rechargeable Battery via Hyperelastic Binder for Self-Powering Wearable Electronics

Kumar, Rajan; Shin, Jaewook; Yin, Lu; You, Jung-Min; Meng, Ying Shirley; Wang, Joseph

doi:10.1002/aenm.201602096

All-Printed, Stretchable Zn-Ag₂O Rechargeable Battery via Hyperelastic Binder for Self-Powering Wearable Electronics

Journal Article · Sun Dec 18 23:00:00 EST 2016 · Advanced Energy Materials

DOI:https://doi.org/10.1002/aenm.201602096· OSTI ID:1533074

Kumar, Rajan ^[1]; Shin, Jaewook ^[2]; Yin, Lu ^[2]; You, Jung-Min ^[2]; Meng, Ying Shirley ^[2]; Wang, Joseph ^[2]

Univ. of California, San Diego, CA (United States); DOE/OSTI
Univ. of California, San Diego, CA (United States)

While several stretchable batteries utilizing either deterministic or random composite architectures have been described, none have been fabricated using inexpensive printing technologies. In this study, the authors printed a highly stretchable, zinc-silver oxide (Zn-Ag₂O) battery by incorporating polystyrene-block-polyisoprene-block-polystyrene (SIS) as a hyperelastic binder for custom-made printable inks. The remarkable mechanical properties of the SIS binder lead to an all-printed, stretchable Zn-Ag₂O rechargeable battery with a ≈2.5 mA h cm^-2 reversible capacity density even after multiple iterations of 100% stretching. This battery offers the highest reversible capacity and discharge current density for intrinsically stretchable batteries reported to date. The electrochemical and mechanical properties are characterized under different strain conditions. The new stress-enduring printable inks pave ways for further developing stretchable electronics for the wide range of wearable applications.

View Accepted Manuscript (DOE)

Research Organization:: Univ. of California, San Diego, CA (United States)

Sponsoring Organization:: USDOE Advanced Research Projects Agency - Energy (ARPA-E)

Grant/Contract Number:: AR0000535

OSTI ID:: 1533074

Alternate ID(s):: OSTI ID: 1401499

Journal Information:: Advanced Energy Materials, Journal Name: Advanced Energy Materials Journal Issue: 8 Vol. 7; ISSN 1614-6832

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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