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Title: Neutron diffraction study on magnetic structures and transitions in Sr 2 Cr 3 As 2 O 2

Journal Article · · Physical Review B
 [1];  [1];  [2]; ORCiD logo [3]; ORCiD logo [3]; ORCiD logo [3];  [4];  [5];  [6];  [7];  [6];  [1]
  1. Renmin Univ. of China, Beijing (China)
  2. Renmin Univ. of China, Beijing (China); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  3. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
  4. China Academy of Engineering Physics, Mianyang (China); Renmin Univ. of China, Beijing (China)
  5. China Academy of Engineering Physics, Mianyang (China)
  6. Zhejiang Univ., Hangzhou (China)
  7. Xiangtan Univ., Xiangtan (China)

Sr2Cr3As2O2 is composed of alternating square-lattice CrO2 and Cr2As2 stacking layers, where CrO2 is isostructural to the CuO2 building-block of cuprate high-Tc superconductors and Cr2As2 to Fe2As2 of Fe-based superconductors. Current interest in this material is raised by theoretic prediction of possible superconductivity. In this neutron powder diffraction study, we discovered that magnetic moments of Cr(II) ions in the Cr2As2 sublattice develop a C-type antiferromagnetic structure below 590 K, and the moments of Cr(I) in the CrO2 sublattice form the La2CuO4-like antiferromagnetic order below 291 K. The staggered magnetic moment 2.19(4)μB/Cr(II) in the more itinerant Cr2As2 layer is smaller than 3.10(6)μB/Cr(I) in the more localized CrO2 layer. Furthermore, different from previous expectations, a spin-flop transition of the Cr(II) magnetic order observed at 291 K indicates a strong coupling between the CrO2 and Cr2As2 magnetic subsystems.

Research Organization:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC05-00OR22725
OSTI ID:
1479776
Alternate ID(s):
OSTI ID: 1477562
Journal Information:
Physical Review B, Vol. 98, Issue 13; ISSN 2469-9950
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 6 works
Citation information provided by
Web of Science

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Figures / Tables (6)


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