A Tunable 3D Nanostructured Conductive Gel Framework Electrode for High-Performance Lithium Ion Batteries

Shi, Ye; Takeuchi, Esther S.

doi:10.1002/adma.201603922

A Tunable 3D Nanostructured Conductive Gel Framework Electrode for High-Performance Lithium Ion Batteries

Journal Article · Tue Jun 13 04:00:00 EDT 2017 · Advanced Materials

DOI:https://doi.org/10.1002/adma.201603922· OSTI ID:1462424

Shi, Ye; Takeuchi, Esther S.

This study develops a tunable 3D nanostructured conductive gel framework as both binder and conductive framework for lithium ion batteries. A 3D nanostructured gel framework with continuous electron pathways can provide hierarchical pores for ion transport and form uniform coatings on each active particle against aggregation. The hybrid gel electrodes based on a polypyrrole gel framework and Fe3O4 nanoparticles as a model system in this study demonstrate the best rate performance, the highest achieved mass ratio of active materials, and the highest achieved specific capacities when considering total mass, compared to current literature. This 3D nanostructured gelbased framework represents a powerful platform for various electrochemically active materials to enable the next-generation high-energy batteries.

Research Organization:: Brookhaven National Laboratory (BNL), Upton, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); National Science Foundation

DOE Contract Number:: SC0012704

OSTI ID:: 1462424

Report Number(s):: BNL-207905-2018-JARP

Journal Information:: Advanced Materials, Journal Name: Advanced Materials Journal Issue: 22 Vol. 29; ISSN 0935-9648

Country of Publication:: United States

Language:: English

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