Enhanced Single-Photon Emission from Carbon-Nanotube Dopant States Coupled to Silicon Microcavities

Ishii, Akihiro; He, Xiaowei; Hartmann, Nicolai F.; Machiya, Hidenori; Htoon, Han; Doorn, Stephen K.; Kato, Yuichiro K.

doi:10.1021/acs.nanolett.8b01170

Title: Enhanced Single-Photon Emission from Carbon-Nanotube Dopant States Coupled to Silicon Microcavities

Journal Article · Mon May 21 00:00:00 EDT 2018 · Nano Letters

DOI:https://doi.org/10.1021/acs.nanolett.8b01170· OSTI ID:1440454

Ishii, Akihiro ^[1];

^[2];

^[2]; Machiya, Hidenori ^[3];

^[2];

^[1]

RIKEN, Saitama (Japan). Nanoscale Quantum Photonics Lab.; RIKEN Center for Advanced Photonics, Saitama (Japan). Quantum Optoelectronics Research Team
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
RIKEN, Saitama (Japan). Nanoscale Quantum Photonics Lab.; Univ. of Tokyo (Japan). Dept. of Electrical Engineering

Single-walled carbon nanotubes are a promising material as quantum light sources at room temperature and as nanoscale light sources for integrated photonic circuits on silicon. Here, we show that the integration of dopant states in carbon nanotubes and silicon microcavities can provide bright and high-purity single-photon emitters on a silicon photonics platform at room temperature. We perform photoluminescence spectroscopy and observe the enhancement of emission from the dopant states by a factor of ~50, and cavity-enhanced radiative decay is confirmed using time-resolved measurements, in which a ~30% decrease of emission lifetime is observed. The statistics of photons emitted from the cavity-coupled dopant states are investigated by photon-correlation measurements, and high-purity single photon generation is observed. The excitation power dependence of photon emission statistics shows that the degree of photon antibunching can be kept high even when the excitation power increases, while the single-photon emission rate can be increased to ~1.7 × 10⁷ Hz.

View Accepted Manuscript (DOE)

Cite

Export

Save

Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE Office of Science (SC); USDOE Laboratory Directed Research and Development (LDRD) Program; Japan Society for the Promotion of Science (JSPS); Ministry of Education, Culture, Sports, Science and Technology (MEXT) (Japan)

Grant/Contract Number:: AC52-06NA25396; JP16K13613; JP17H07359

OSTI ID:: 1440454

Report Number(s):: LA-UR-18-22596

Journal Information:: Nano Letters, Vol. 18, Issue 6; ISSN 1530-6984

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

Citation Metrics:

Cited by: 37 works

Citation information provided by
Web of Science

References (45)

Photonic quantum technologies O'Brien, Jeremy L.; Furusawa, Akira; Vučković, Jelena Nature Photonics, Vol. 3, Issue 12 https://doi.org/10.1038/nphoton.2009.229	journal	December 2009
Solid-state single-photon emitters Aharonovich, Igor; Englund, Dirk; Toth, Milos Nature Photonics, Vol. 10, Issue 10 https://doi.org/10.1038/nphoton.2016.186	journal	September 2016
Carbon-nanotube photonics and optoelectronics Avouris, Phaedon; Freitag, Marcus; Perebeinos, Vasili Nature Photonics, Vol. 2, Issue 6 https://doi.org/10.1038/nphoton.2008.94	journal	June 2008
The Optical Resonances in Carbon Nanotubes Arise from Excitons Wang, F. Science, Vol. 308, Issue 5723 https://doi.org/10.1126/science.1110265	journal	May 2005
Exciton binding energies in carbon nanotubes from two-photon photoluminescence Maultzsch, J.; Pomraenke, R.; Reich, S. Physical Review B, Vol. 72, Issue 24 https://doi.org/10.1103/PhysRevB.72.241402	journal	December 2005
Ubiquity of Exciton Localization in Cryogenic Carbon Nanotubes Hofmann, Matthias S.; Noé, Jonathan; Kneer, Alexander Nano Letters, Vol. 16, Issue 5 https://doi.org/10.1021/acs.nanolett.5b04901	journal	April 2016
Photon Antibunching in the Photoluminescence Spectra of a Single Carbon Nanotube Högele, Alexander; Galland, Christophe; Winger, Martin Physical Review Letters, Vol. 100, Issue 21 https://doi.org/10.1103/PhysRevLett.100.217401	journal	May 2008
Bright, long-lived and coherent excitons in carbon nanotube quantum dots Hofmann, Matthias S.; Glückert, Jan T.; Noé, Jonathan Nature Nanotechnology, Vol. 8, Issue 7 https://doi.org/10.1038/nnano.2013.119	journal	June 2013
Photon antibunching in single-walled carbon nanotubes at telecommunication wavelengths and room temperature Endo, Takumi; Ishi-Hayase, Junko; Maki, Hideyuki Applied Physics Letters, Vol. 106, Issue 11 https://doi.org/10.1063/1.4915618	journal	March 2015
Room-temperature single-photon generation from solitary dopants of carbon nanotubes Ma, Xuedan; Hartmann, Nicolai F.; Baldwin, Jon K. S. Nature Nanotechnology, Vol. 10, Issue 8 https://doi.org/10.1038/nnano.2015.136	journal	July 2015
Tunable room-temperature single-photon emission at telecom wavelengths from sp3 defects in carbon nanotubes He, Xiaowei; Hartmann, Nicolai F.; Ma, Xuedan Nature Photonics, Vol. 11, Issue 9 https://doi.org/10.1038/nphoton.2017.119	journal	July 2017
Influences of Exciton Diffusion and Exciton-Exciton Annihilation on Photon Emission Statistics of Carbon Nanotubes Ma, Xuedan; Roslyak, Oleskiy; Duque, Juan G. Physical Review Letters, Vol. 115, Issue 1 https://doi.org/10.1103/PhysRevLett.115.017401	journal	July 2015
Room-Temperature Single-Photon Emission from Micrometer-Long Air-Suspended Carbon Nanotubes Ishii, A.; Uda, T.; Kato, Y. K. Physical Review Applied, Vol. 8, Issue 5 https://doi.org/10.1103/PhysRevApplied.8.054039	journal	November 2017
Brightening of carbon nanotube photoluminescence through the incorporation of sp3 defects Piao, Yanmei; Meany, Brendan; Powell, Lyndsey R. Nature Chemistry, Vol. 5, Issue 10 https://doi.org/10.1038/nchem.1711	journal	July 2013
Brightening of excitons in carbon nanotubes on dimensionality modification Miyauchi, Yuhei; Iwamura, Munechiyo; Mouri, Shinichiro Nature Photonics, Vol. 7, Issue 9 https://doi.org/10.1038/nphoton.2013.179	journal	July 2013
Photoluminescence Dynamics of Aryl sp ³ Defect States in Single-Walled Carbon Nanotubes Hartmann, Nicolai F.; Velizhanin, Kirill A.; Haroz, Erik H. ACS Nano, Vol. 10, Issue 9 https://doi.org/10.1021/acsnano.6b02986	journal	August 2016
High-frequency single-photon source with polarization control Strauf, Stefan; Stoltz, Nick G.; Rakher, Matthew T. Nature Photonics, Vol. 1, Issue 12 https://doi.org/10.1038/nphoton.2007.227	journal	November 2007
Deterministic Coupling of a Single Nitrogen Vacancy Center to a Photonic Crystal Cavity Englund, Dirk; Shields, Brendan; Rivoire, Kelley Nano Letters, Vol. 10, Issue 10 https://doi.org/10.1021/nl101662v	journal	October 2010
Purcell-Enhanced Single-Photon Emission from Nitrogen-Vacancy Centers Coupled to a Tunable Microcavity Kaupp, Hanno; Hümmer, Thomas; Mader, Matthias Physical Review Applied, Vol. 6, Issue 5 https://doi.org/10.1103/PhysRevApplied.6.054010	journal	November 2016
Quantum Light Signatures and Nanosecond Spectral Diffusion from Cavity-Embedded Carbon Nanotubes Walden-Newman, William; Sarpkaya, Ibrahim; Strauf, Stefan Nano Letters, Vol. 12, Issue 4 https://doi.org/10.1021/nl204402v	journal	January 2012
Widely Tunable Single-Photon Source from a Carbon Nanotube in the Purcell Regime Jeantet, A.; Chassagneux, Y.; Raynaud, C. Physical Review Letters, Vol. 116, Issue 24 https://doi.org/10.1103/PhysRevLett.116.247402	journal	June 2016
Purcell-enhanced quantum yield from carbon nanotube excitons coupled to plasmonic nanocavities Luo, Yue; Ahmadi, Ehsaneh D.; Shayan, Kamran Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/s41467-017-01777-w	journal	November 2017
Large-scale quantum photonic circuits in silicon Harris, Nicholas C.; Bunandar, Darius; Pant, Mihir Nanophotonics, Vol. 5, Issue 3 https://doi.org/10.1515/nanoph-2015-0146	journal	August 2016
Enhancement of carbon nanotube photoluminescence by photonic crystal nanocavities Watahiki, R.; Shimada, T.; Zhao, P. Applied Physics Letters, Vol. 101, Issue 14 https://doi.org/10.1063/1.4757876	journal	October 2012
Enhanced light emission from carbon nanotubes integrated in silicon micro-resonator Noury, Adrien; Roux, Xavier Le; Vivien, Laurent Nanotechnology, Vol. 26, Issue 34 https://doi.org/10.1088/0957-4484/26/34/345201	journal	August 2015
Cavity-enhanced Raman scattering of single-walled carbon nanotubes Sumikura, Hisashi; Kuramochi, Eiichi; Taniyama, Hideaki Applied Physics Letters, Vol. 102, Issue 23 https://doi.org/10.1063/1.4810761	journal	June 2013
Optical control of individual carbon nanotube light emitters by spectral double resonance in silicon microdisk resonators Imamura, S.; Watahiki, R.; Miura, R. Applied Physics Letters, Vol. 102, Issue 16 https://doi.org/10.1063/1.4802930	journal	April 2013
Ultralow mode-volume photonic crystal nanobeam cavities for high-efficiency coupling to individual carbon nanotube emitters Miura, R.; Imamura, S.; Ohta, R. Nature Communications, Vol. 5, Issue 1 https://doi.org/10.1038/ncomms6580	journal	November 2014
Spectral tuning of optical coupling between air-mode nanobeam cavities and individual carbon nanotubes Machiya, H.; Uda, T.; Ishii, A. Applied Physics Letters, Vol. 112, Issue 2 https://doi.org/10.1063/1.5008299	journal	January 2018
High-Q photonic nanocavity in a two-dimensional photonic crystal Akahane, Yoshihiro; Asano, Takashi; Song, Bong-Shik Nature, Vol. 425, Issue 6961 https://doi.org/10.1038/nature02063	journal	October 2003
Photoluminescence imaging of solitary dopant sites in covalently doped single-wall carbon nanotubes Hartmann, Nicolai F.; Yalcin, Sibel Ebru; Adamska, Lyudmyla Nanoscale, Vol. 7, Issue 48 https://doi.org/10.1039/C5NR06343D	journal	January 2015
Chirality dependence of the $K$ -momentum dark excitons in carbon nanotubes Vora, P. M.; Tu, X.; Mele, E. J. Physical Review B, Vol. 81, Issue 15 https://doi.org/10.1103/PhysRevB.81.155123	journal	April 2010
Exciton diffusion, end quenching, and exciton-exciton annihilation in individual air-suspended carbon nanotubes Ishii, A.; Yoshida, M.; Kato, Y. K. Physical Review B, Vol. 91, Issue 12 https://doi.org/10.1103/PhysRevB.91.125427	journal	March 2015
Localized Guided-Mode and Cavity-Mode Double Resonance in Photonic Crystal Nanocavities Liu, X.; Shimada, T.; Miura, R. Physical Review Applied, Vol. 3, Issue 1 https://doi.org/10.1103/PhysRevApplied.3.014006	journal	January 2015
Simultaneous Inhibition and Redistribution of Spontaneous Light Emission in Photonic Crystals Fujita, M. Science, Vol. 308, Issue 5726 https://doi.org/10.1126/science.1110417	journal	May 2005
Direct printing of nanostructures by electrostatic autofocussing of ink nanodroplets Galliker, P.; Schneider, J.; Eghlidi, H. Nature Communications, Vol. 3, Issue 1 https://doi.org/10.1038/ncomms1891	journal	January 2012
Near-Field Light Design with Colloidal Quantum Dots for Photonics and Plasmonics Kress, Stephan J. P.; Richner, Patrizia; Jayanti, Sriharsha V. Nano Letters, Vol. 14, Issue 10 https://doi.org/10.1021/nl5026997	journal	September 2014
Synthesis and Characterization of Hexagonal Boron Nitride Film as a Dielectric Layer for Graphene Devices Kim, Ki Kang; Hsu, Allen; Jia, Xiaoting ACS Nano, Vol. 6, Issue 10 https://doi.org/10.1021/nn301675f	journal	September 2012
Mode structure of the L3 photonic crystal cavity Chalcraft, A. R. A.; Lam, S.; O’Brien, D. Applied Physics Letters, Vol. 90, Issue 24 https://doi.org/10.1063/1.2748310	journal	June 2007
Light Emission From Silicon in Photonic Crystal Nanocavity Fujita, Masayuki; Tanaka, Yoshinori; Noda, Susumu IEEE Journal of Selected Topics in Quantum Electronics, Vol. 14, Issue 4 https://doi.org/10.1109/JSTQE.2008.918941	journal	January 2008
Room-temperature single photon emission from micron-long air-suspended carbon nanotubes Ishii, A.; Uda, T.; Kato, Y. K. JSAP-OSA Joint Symposia 2017 Abstracts https://doi.org/10.1364/jsap.2017.7p_a404_3	conference	January 2017
Are we evil? Yes we are – but at least not crazy! How to test implicit associations of fans and non-fans with metal music Kneer, Julia Metal Music Studies, Vol. 2, Issue 1 https://doi.org/10.1386/mms.2.1.69_1	journal	March 2016
Optical control of individual carbon nanotube light emitters by spectral double resonance in silicon microdisk resonators Imamura, S.; Watahiki, R.; Miura, R. arXiv https://doi.org/10.48550/arxiv.1303.6035	text	January 2013
Influences of Exciton Diffusion and Exciton-Exciton Annihilation on Photon Emission Statistics of Carbon Nanotubes Ma, Xuedan; Roslyak, Oleskiy; Duque, Juan G. arXiv https://doi.org/10.48550/arxiv.1502.05964	text	January 2015
Purcell-Enhanced Single-Photon Emission from Nitrogen-Vacancy Centers Coupled to a Tunable Microcavity Kaupp, Hanno; Hümmer, Thomas; Mader, Matthias Karlsruhe https://doi.org/10.5445/ir/1000064882	text	January 2016

Cited By (10)

High Efficiency Dark-to-Bright Exciton Conversion in Carbon Nanotubes Ishii, A.; Machiya, H.; Kato, Y. K. Physical Review X, Vol. 9, Issue 4 https://doi.org/10.1103/physrevx.9.041048	journal	December 2019
Controlling photon antibunching from 1D emitters using optical antennas Lange, Lucas; Schäfer, Frank; Biewald, Alexander Nanoscale, Vol. 11, Issue 31 https://doi.org/10.1039/c9nr03688a	journal	January 2019
Single‐photon emission from a further confined InGaN/GaN quantum disc via reverse‐reaction growth Sun, Xiaoxiao; Wang, Ping; Sheng, Bowen Quantum Engineering, Vol. 1, Issue 3 https://doi.org/10.1002/que2.20	journal	June 2019
Metal-dielectric nanoantenna for radiation control of a single-photon emitter Sun, Yali; Yaroshenko, Vitaly; Chebykin, Alexander Optical Materials Express, Vol. 10, Issue 1 https://doi.org/10.1364/ome.10.000029	journal	December 2019
Atomic Self‐reconstruction of Catalyst Dominated Growth Mechanism of Graphite Structures Hu, Yang; Zhu, Liu; Peng, Yong ChemCatChem, Vol. 12, Issue 5 https://doi.org/10.1002/cctc.201902087	journal	December 2019
New Light on Molecule–Nanotube Hybrids Chen, Yani; Marty, Laëtitia; Bendiab, Nedjma Advanced Materials, Vol. 31, Issue 48 https://doi.org/10.1002/adma.201902917	journal	September 2019
High efficiency dark-to-bright exciton conversion in carbon nanotubes Ishii, A.; Machiya, H.; Kato, Y. K. arXiv https://doi.org/10.48550/arxiv.1905.10043	text	January 2019
Quantum Emission Assisted by Energy Landscape Modification in Pentacene-Decorated Carbon Nanotubes Li, Zhen; Otsuka, Keigo; Yamashita, Daiki ACS Photonics, Vol. 8, Issue 8 https://doi.org/10.1021/acsphotonics.1c00539	journal	July 2021
Near-unity radiative quantum efficiency of excitons in carbon nanotubes Machiya, H.; Yamashita, D.; Ishii, A. arXiv https://doi.org/10.48550/arxiv.2102.10718	text	January 2021
Formation of Organic Color Centers in Air-Suspended Carbon Nanotubes Using Vapor-Phase Reaction Kozawa, D.; Wu, X.; Ishii, A. arXiv https://doi.org/10.48550/arxiv.2103.00689	text	January 2021

Similar Records

Solitary Oxygen Dopant Emission from Carbon Nanotubes Modified by Dielectric Metasurfaces

Journal Article · Thu May 18 00:00:00 EDT 2017 · ACS Nano · OSTI ID:1440454

Ma, Xuedan; James, Anthony R.; Hartmann, Nicolai F.; +9 more

Photoluminescence imaging of solitary dopant sites in covalently doped single-wall carbon nanotubes

Journal Article · Wed Nov 11 00:00:00 EST 2015 · Nanoscale · OSTI ID:1440454

Hartmann, Nicolai F.; Yalcin, Sibel Ebru; Adamska, Lyudmyla; +5 more

Low-Temperature Single Carbon Nanotube Spectroscopy of sp³ Quantum Defects

Journal Article · Thu Sep 28 00:00:00 EDT 2017 · ACS Nano · OSTI ID:1440454

He, Xiaowei; Gifford, Brendan Joel; Hartmann, Nicolai; +10 more

Related Subjects

71 CLASSICAL AND QUANTUM MECHANICS
GENERAL PHYSICS
Material Science
Carbon nanotubes
diazonium doping
photoluminescence
photonic crystal
single-photon source

Title: Enhanced Single-Photon Emission from Carbon-Nanotube Dopant States Coupled to Silicon Microcavities

Citation Formats

References (45)

Cited By (10)

Similar Records

Related Subjects