Solitary Oxygen Dopant Emission from Carbon Nanotubes Modified by Dielectric Metasurfaces

Ma, Xuedan; James, Anthony R.; Hartmann, Nicolai F.; Baldwin, Jon Kevin Scott; Dominguez, Jason; Sinclair, Michael B.; Luk, Ting S.; Wolf, Omri; Liu, Sheng; Doorn, Stephen K.; Htoon, Han; Brener, Igal

doi:10.1021/acsnano.7b02951

Title: Solitary Oxygen Dopant Emission from Carbon Nanotubes Modified by Dielectric Metasurfaces

Journal Article · Thu May 18 00:00:00 EDT 2017 · ACS Nano

DOI:https://doi.org/10.1021/acsnano.7b02951· OSTI ID:1481990

^[1]; James, Anthony R. ^[1];

^[2]; Baldwin, Jon Kevin Scott ^[2]; Dominguez, Jason ^[3]; Sinclair, Michael B. ^[3]; Luk, Ting S. ^[1]; Wolf, Omri ^[1]; Liu, Sheng ^[1];

^[2];

^[2]; Brener, Igal ^[1]

Sandia National Lab. (SNL-NM), Albuquerque, NM (United States). Center for Integrated Nanotechnologies
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)

All-dielectric metasurfaces made from arrays of high index nanoresonators supporting strong magnetic dipole modes have emerged as a low-loss alternative to plasmonic metasurfaces. Here we use oxygen-doped single-walled carbon nanotubes (SWCNTs) as quantum emitters and couple them to silicon metasurfaces to study effects of the magnetic dipole modes of the constituent nanoresonators on the photoluminescence (PL) of individual SWCNTs. We find that when in resonance, the magnetic mode of the silicon nanoresonators can lead to a moderate average PL enhancement of 0.8–4.0 of the SWCNTs, accompanied by an average increase in the radiative decay rate by a factor of 1.5–3.0. More interestingly, single dopant polarization experiments show an anomalous photoluminescence polarization rotation by coupling individual SWCNTs to silicon nanoresonators. Numerical simulations indicate that this is caused by modification of near-field polarization distribution at certain areas in the proximity of the silicon nanoresonators at the excitation wavelength, thus presenting an approach to control emission polarization. In conclusion, these findings indicate silicon nanoresonators as potential building blocks of quantum photonic circuits capable of manipulating PL intensity and polarization of single photon sources.

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Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: AC52-06NA25396; NA0003525

OSTI ID:: 1481990

Report Number(s):: LA-UR-18-21087

Journal Information:: ACS Nano, Vol. 11, Issue 6; ISSN 1936-0851

Publisher:: American Chemical Society (ACS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 13 works

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77 NANOSCIENCE AND NANOTECHNOLOGY
36 MATERIALS SCIENCE
Material Science
all-dielectric metasurfaces
magnetic resonance
oxygen-doped single-walled carbon nanotubes
photoluminescence
polarization

Title: Solitary Oxygen Dopant Emission from Carbon Nanotubes Modified by Dielectric Metasurfaces

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