Giant tunneling magnetoresistance in spin-filter van der Waals heterostructures

Song, Tiancheng; Cai, Xinghan; Tu, Matisse Wei-Yuan; Zhang, Xiaoou; Huang, Bevin; Wilson, Nathan P.; Seyler, Kyle L.; Zhu, Lin; Taniguchi, Takashi; Watanabe, Kenji; McGuire, Michael A.; Cobden, David H.; Xiao, Di; Yao, Wang; Xu, Xiaodong

doi:10.1126/science.aar4851

Giant tunneling magnetoresistance in spin-filter van der Waals heterostructures

Journal Article · Fri Jun 15 00:00:00 EDT 2018 · Science

DOI:https://doi.org/10.1126/science.aar4851· OSTI ID:1439141

^[1]; ^[1]; ^[2]; Zhang, Xiaoou ^[3]; ^[1]; Wilson, Nathan P. ^[1]; ^[1]; Zhu, Lin ^[1]; Taniguchi, Takashi ^[4]; ^[4]; ^[5]; Cobden, David H. ^[1]; ^[3]; ^[2]; ^[1]

Univ. of Washington, Seattle, WA (United States)
Univ. of Hong Kong, Hong Kong (China)
Carnegie Mellon Univ., Pittsburgh, PA (United States)
National Institute for Materials Science, Ibaraki (Japan)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Magnetic multilayer devices that exploit magnetoresistance are the backbone of magnetic sensing and data storage technologies. Here, we report multiple-spin-filter magnetic tunnel junctions (sf-MTJs) based on van der Waals (vdW) heterostructures in which atomically thin chromium triiodide (CrI3) acts as a spin-filter tunnel barrier sandwiched between graphene contacts. We demonstrate tunneling magnetoresistance which is drastically enhanced with increasing CrI₃ layer thickness, reaching a record 19,000% for magnetic multilayer structures using four-layer sf-MTJs at low temperatures. Using magnetic circular dichroism measurements, we attribute these effects to the intrinsic layer-by-layer antiferromagnetic ordering of the atomically thin CrI₃. In conclusion, our work reveals the possibility to push magnetic information storage to the atomically thin limit and highlights CrI₃ as a superlative magnetic tunnel barrier for vdW heterostructure spintronic devices.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1439141

Journal Information:: Science, Journal Name: Science Journal Issue: 6394 Vol. 360; ISSN 0036-8075

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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