Protected Lithium-Metal Anodes in Batteries: From Liquid to Solid

Yang, Chunpeng; Fu, Kun; Zhang, Ying; Hitz, Emily; Hu, Liangbing

doi:10.1002/adma.201701169

Protected Lithium-Metal Anodes in Batteries: From Liquid to Solid

Journal Article · Mon Jul 24 00:00:00 EDT 2017 · Advanced Materials

DOI:https://doi.org/10.1002/adma.201701169· OSTI ID:1433803

^[1]; Fu, Kun ^[2]; Zhang, Ying ^[2]; Hitz, Emily ^[2]; Hu, Liangbing ^[2]

Univ. of Maryland, College Park, MD (United States). Dept. of Materials Science and Engineering; University of Maryland
Univ. of Maryland, College Park, MD (United States). Dept. of Materials Science and Engineering

High-energy lithium-metal batteries are among the most promising candidates for next-generation energy storage systems. With a high specific capacity and a low reduction potential, the Li-metal anode has attracted extensive interest for decades. Dendritic Li formation, uncontrolled interfacial reactions, and huge volume effect are major hurdles to the commercial application of Li-metal anodes. Recent studies have shown that the performance and safety of Li-metal anodes can be significantly improved via organic electrolyte modification, Li-metal interface protection, Li-electrode framework design, separator coating, and so on. Superior to the liquid electrolytes, solid-state electrolytes are considered able to inhibit problematic Li dendrites and build safe solid Li-metal batteries. Inspired by the bright prospects of solid Li-metal batteries, increasing efforts have been devoted to overcoming the obstacles of solid Li-metal batteries, such as low ionic conductivity of the electrolyte and Li–electrolyte interfacial problems. In this paper, the approaches to protect Li-metal anodes from liquid batteries to solid-state batteries are outlined and analyzed in detail. Finally, perspectives regarding the strategies for developing Li-metal anodes are discussed to facilitate the practical application of Li-metal batteries.

View Accepted Manuscript (DOE)

Research Organization:: Univ. of Maryland, College Park, MD (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Vehicle Technologies Office (EE-3V); USDOE Advanced Research Projects Agency - Energy (ARPA-E); USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); China Scholarship Council

Grant/Contract Number:: EE0006860; AR0000384; SC0001160

OSTI ID:: 1433803

Alternate ID(s):: OSTI ID: 1389033
OSTI ID: 1393692

Journal Information:: Advanced Materials, Journal Name: Advanced Materials Journal Issue: 36 Vol. 29; ISSN 0935-9648

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Recent Progress of the Solid-State Electrolytes for High-Energy Metal-Based Batteries Fan, Lei; Wei, Shuya; Li, Siyuan Advanced Energy Materials, Vol. 8, Issue 11 https://doi.org/10.1002/aenm.201702657	journal	January 2018
Vertically Aligned Lithiophilic CuO Nanosheets on a Cu Collector to Stabilize Lithium Deposition for Lithium Metal Batteries Zhang, Chen; Lv, Wei; Zhou, Guangmin Advanced Energy Materials, Vol. 8, Issue 21 https://doi.org/10.1002/aenm.201703404	journal	April 2018
Compact 3D Copper with Uniform Porous Structure Derived by Electrochemical Dealloying as Dendrite-Free Lithium Metal Anode Current Collector Zhao, Heng; Lei, Danni; He, Yan-Bing Advanced Energy Materials, Vol. 8, Issue 19 https://doi.org/10.1002/aenm.201800266	journal	March 2018
3D Wettable Framework for Dendrite-Free Alkali Metal Anodes Zhang, Ying; Wang, Chengwei; Pastel, Glenn Advanced Energy Materials, Vol. 8, Issue 18 https://doi.org/10.1002/aenm.201800635	journal	May 2018
Ethers Illume Sodium-Based Battery Chemistry: Uniqueness, Surprise, and Challenges Zhang, Jun; Wang, Da-Wei; Lv, Wei Advanced Energy Materials, Vol. 8, Issue 26 https://doi.org/10.1002/aenm.201801361	journal	July 2018
Enabling Stable Lithium Metal Anode via 3D Inorganic Skeleton with Superlithiophilic Interphase Fan, Lei; Li, Siyuan; Liu, Lei Advanced Energy Materials, Vol. 8, Issue 33 https://doi.org/10.1002/aenm.201802350	journal	October 2018
Improved Rechargeability of Lithium Metal Anode via Controlling Lithium-Ion Flux Xiang, Jingwei; Yuan, Lixia; Shen, Yue Advanced Energy Materials, Vol. 8, Issue 36 https://doi.org/10.1002/aenm.201802352	journal	October 2018
High Performance Lithium Metal Batteries Enabled by Surface Tailoring of Polypropylene Separator with a Polydopamine/Graphene Layer Kim, Patrick J.; Pol, Vilas G. Advanced Energy Materials, Vol. 8, Issue 36 https://doi.org/10.1002/aenm.201802665	journal	November 2018
2D Materials for Lithium/Sodium Metal Anodes Zhang, Chanyuan; Wang, Aoxuan; Zhang, Jiahua Advanced Energy Materials, Vol. 8, Issue 34 https://doi.org/10.1002/aenm.201802833	journal	October 2018
Single-Ion Conducting Electrolyte Based on Electrospun Nanofibers for High-Performance Lithium Batteries Li, Cuicui; Qin, Bingsheng; Zhang, Yunfeng Advanced Energy Materials, Vol. 9, Issue 10 https://doi.org/10.1002/aenm.201803422	journal	January 2019
Dopant‐Dependent Stability of Garnet Solid Electrolyte Interfaces with Lithium Metal Zhu, Yisi; Connell, Justin G.; Tepavcevic, Sanja Advanced Energy Materials, Vol. 9, Issue 12 https://doi.org/10.1002/aenm.201803440	journal	January 2019
Thick Electrode Batteries: Principles, Opportunities, and Challenges Kuang, Yudi; Chen, Chaoji; Kirsch, Dylan Advanced Energy Materials, Vol. 9, Issue 33 https://doi.org/10.1002/aenm.201901457	journal	July 2019
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Normalized Lithium Growth from the Nucleation Stage for Dendrite‐Free Lithium Metal Anodes Li, Nan; Ye, Qian; Zhang, Kun Angewandte Chemie, Vol. 131, Issue 50 https://doi.org/10.1002/ange.201911267	journal	October 2019
Fast Lithium Ion Conduction in Lithium Phosphidoaluminates Restle, Tassilo M. F.; Sedlmeier, Christian; Kirchhain, Holger Angewandte Chemie, Vol. 132, Issue 14 https://doi.org/10.1002/ange.201914613	journal	January 2020
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Protecting the Lithium Metal Anode for a Safe Flexible Lithium-Air Battery in Ambient Air Liu, Tong; Feng, Xi-lan; Jin, Xin Angewandte Chemie International Edition, Vol. 58, Issue 50 https://doi.org/10.1002/anie.201911229	journal	October 2019
Normalized Lithium Growth from the Nucleation Stage for Dendrite‐Free Lithium Metal Anodes Li, Nan; Ye, Qian; Zhang, Kun Angewandte Chemie International Edition, Vol. 58, Issue 50 https://doi.org/10.1002/anie.201911267	journal	December 2019
Fast Lithium Ion Conduction in Lithium Phosphidoaluminates Restle, Tassilo M. F.; Sedlmeier, Christian; Kirchhain, Holger Angewandte Chemie International Edition, Vol. 59, Issue 14 https://doi.org/10.1002/anie.201914613	journal	January 2020
Preparation and performance of poly(ethylene oxide)‐based composite solid electrolyte for all solid‐state lithium batteries Li, Xiaolong; Wang, Xianyou; Shao, Dingsheng Journal of Applied Polymer Science, Vol. 136, Issue 19 https://doi.org/10.1002/app.47498	journal	January 2019
Preparation and application of poly(ethylene oxide)‐based all solid‐state electrolyte with a walnut‐like SiO ₂ as nano‐fillers Li, Xiaolong; Yang, Li; Shao, Dingsheng Journal of Applied Polymer Science, Vol. 137, Issue 24 https://doi.org/10.1002/app.48810	journal	December 2019
Antimony‐Doped Lithium Phosphate Artificial Solid Electrolyte Interphase for Dendrite‐Free Lithium‐Metal Batteries Gao, Chunhui; Dong, Qingyuan; Zhang, Gang ChemElectroChem, Vol. 6, Issue 4 https://doi.org/10.1002/celc.201801410	journal	January 2019
High Ion Conducting Solid Composite Electrolytes with Enhanced Interfacial Compatibility for Lithium Metal Batteries Feng, Haoyu; Ma, Cheng; Dai, Kuan ChemElectroChem, Vol. 6, Issue 3 https://doi.org/10.1002/celc.201801894	journal	February 2019
Reducing the Interfacial Resistance in All‐Solid‐State Lithium Batteries Based on Oxide Ceramic Electrolytes Jiang, Zhouyang; Han, Qingyue; Wang, Suqing ChemElectroChem, Vol. 6, Issue 12 https://doi.org/10.1002/celc.201801898	journal	April 2019
Construction of Ag/WS ₂ Zero/Two‐Dimensional Hybrid Architectures by Self‐Assembly for High‐Rate Lithium Storage Mao, Ya‐Chun; Zhu, Xiao‐Dong; Fan, Xiu‐Hua ChemElectroChem, Vol. 6, Issue 17 https://doi.org/10.1002/celc.201901288	journal	August 2019
Recent Progress of Hybrid Solid‐State Electrolytes for Lithium Batteries Liu, Xiaoyan; Li, Xinru; Li, Hexing Chemistry – A European Journal, Vol. 24, Issue 69 https://doi.org/10.1002/chem.201803616	journal	June 2018
Interface-Engineered Li ₇ La ₃ Zr ₂ O ₁₂ -Based Garnet Solid Electrolytes with Suppressed Li-Dendrite Formation and Enhanced Electrochemical Performance Zhang, Zhaoshuai; Zhang, Long; Liu, Yanyan ChemSusChem, Vol. 11, Issue 21 https://doi.org/10.1002/cssc.201801756	journal	October 2018
Synergistically Suppressing Lithium Dendrite Growth by Coating Poly‐ l ‐Lactic Acid on Sustainable Gel Polymer Electrolyte Li, Lei; Yu, Miao; Wang, Feijun Energy Technology, Vol. 7, Issue 5 https://doi.org/10.1002/ente.201800768	journal	April 2019
Heat‐Resistant Trilayer Separators for High‐Performance Lithium‐Ion Batteries Feng, Chao; Wang, Xuchang; Zeng, Guangfeng physica status solidi (RRL) – Rapid Research Letters, Vol. 14, Issue 1 https://doi.org/10.1002/pssr.201900504	journal	October 2019
Design Principles of Functional Polymer Separators for High-Energy, Metal-Based Batteries Zhang, Weidong; Tu, Zhengyuan; Qian, Jiawei Small, Vol. 14, Issue 11 https://doi.org/10.1002/smll.201703001	journal	December 2017
Dendrite-Free Lithium Deposition via Flexible-Rigid Coupling Composite Network for LiNi _0.5 Mn _1.5 O ₄ /Li Metal Batteries Chai, Jingchao; Chen, Bingbing; Xian, Fang Small, Vol. 14, Issue 37 https://doi.org/10.1002/smll.201802244	journal	August 2018
Regulating Lithium Nucleation via CNTs Modifying Carbon Cloth Film for Stable Li Metal Anode Liu, Fanfan; Xu, Rui; Hu, Zexun Small, Vol. 15, Issue 5 https://doi.org/10.1002/smll.201803734	journal	December 2018
Plasma Treatment for Nitrogen-Doped 3D Graphene Framework by a Conductive Matrix with Sulfur for High-Performance Li-S Batteries Duan, Lianfeng; Zhao, Lijuan; Cong, Hui Small, Vol. 15, Issue 7 https://doi.org/10.1002/smll.201804347	journal	January 2019
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Compactly Coupled Nitrogen‐Doped Carbon Nanosheets/Molybdenum Phosphide Nanocrystal Hollow Nanospheres as Polysulfide Reservoirs for High‐Performance Lithium–Sulfur Chemistry Sun, Zhonghui; Wu, Xing‐Long; Peng, Zhangquan Small, Vol. 15, Issue 40 https://doi.org/10.1002/smll.201902491	journal	August 2019
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Li _0.33 La _0.557 TiO ₃ ceramic nanofiber-enhanced polyethylene oxide-based composite polymer electrolytes for all-solid-state lithium batteries Zhu, Pei; Yan, Chaoyi; Dirican, Mahmut Journal of Materials Chemistry A, Vol. 6, Issue 10 https://doi.org/10.1039/c7ta10517g	journal	January 2018
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Recent developments and insights into the understanding of Na metal anodes for Na-metal batteries Zhao, Yang; Adair, Keegan R.; Sun, Xueliang Energy & Environmental Science, Vol. 11, Issue 10 https://doi.org/10.1039/c8ee01373j	journal	January 2018
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One-step in situ growth of ZnS nanoparticles on reduced graphene oxides and their improved lithium storage performance using sodium carboxymethyl cellulose binder Lu, Lun; Jing, Liwei; Yang, Zhizheng RSC Advances, Vol. 8, Issue 17 https://doi.org/10.1039/c8ra00470f	journal	January 2018
Reliable seawater battery anode: controlled sodium nucleation via deactivation of the current collector surface Kim, Do Hyeong; Choi, Hongkyw; Hwang, Dae Yeon Journal of Materials Chemistry A, Vol. 6, Issue 40 https://doi.org/10.1039/c8ta07610c	journal	January 2018
Revisiting polymeric single lithium-ion conductors as an organic route for all-solid-state lithium ion and metal batteries Jeong, Kihun; Park, Sodam; Lee, Sang-Young Journal of Materials Chemistry A, Vol. 7, Issue 5 https://doi.org/10.1039/c8ta09056d	journal	January 2019
Li ₇ La ₃ Zr ₂ O ₁₂ ceramic nanofiber-incorporated composite polymer electrolytes for lithium metal batteries Li, Yang; Zhang, Wei; Dou, Qianqian Journal of Materials Chemistry A, Vol. 7, Issue 7 https://doi.org/10.1039/c8ta11449h	journal	January 2019
Chemically exfoliated boron nitride nanosheets form robust interfacial layers for stable solid-state Li metal batteries Shen, Bao; Zhang, Tian-Wen; Yin, Yi-Chen Chemical Communications, Vol. 55, Issue 53 https://doi.org/10.1039/c9cc02124h	journal	January 2019
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A versatile single-ion electrolyte with a Grotthuss-like Li conduction mechanism for dendrite-free Li metal batteries Yuan, Shouyi; Bao, Junwei Lucas; Wei, Jishi Energy & Environmental Science, Vol. 12, Issue 9 https://doi.org/10.1039/c9ee01473j	journal	January 2019
Dendrite formation in Li-metal anodes: an atomistic molecular dynamics study Selis, Luis A.; Seminario, Jorge M. RSC Advances, Vol. 9, Issue 48 https://doi.org/10.1039/c9ra05067a	journal	January 2019
Nonflammable quasi-solid-state electrolyte for stable lithium-metal batteries Sun, Qiushi; Chen, Xiao; Xie, Jian RSC Advances, Vol. 9, Issue 72 https://doi.org/10.1039/c9ra08677c	journal	January 2019
Towards high energy density lithium battery anodes: silicon and lithium Zhu, Bin; Wang, Xinyu; Yao, Pengcheng Chemical Science, Vol. 10, Issue 30 https://doi.org/10.1039/c9sc01201j	journal	January 2019
ZnO nanoarray-modified nickel foam as a lithiophilic skeleton to regulate lithium deposition for lithium-metal batteries Sun, Changzhi; Li, Yanpei; Jin, Jun Journal of Materials Chemistry A, Vol. 7, Issue 13 https://doi.org/10.1039/c9ta00862d	journal	January 2019
Single-cluster Au as an usher for deeply cyclable Li metal anodes Yang, Tingzhou; Qian, Tao; Shen, Xiaowei Journal of Materials Chemistry A, Vol. 7, Issue 24 https://doi.org/10.1039/c9ta02640a	journal	January 2019
A borate decorated anion-immobilized solid polymer electrolyte for dendrite-free, long-life Li metal batteries Ma, Cheng; Feng, Yiming; Xing, Fangzhou Journal of Materials Chemistry A, Vol. 7, Issue 34 https://doi.org/10.1039/c9ta07551h	journal	January 2019
Dendrite-free lithium–metal batteries at high rate realized using a composite solid electrolyte with an ester–PO ₄ complex and stable interphase Zhang, Zhaoshuai; Zhang, Long; Liu, Yanyan Journal of Materials Chemistry A, Vol. 7, Issue 40 https://doi.org/10.1039/c9ta08415k	journal	January 2019
Confinement effect and air tolerance of Li plating by lithiophilic poly(vinyl alcohol) coating for dendrite-free Li metal batteries Wu, Han; Yao, Zhenguo; Wu, Qingping Journal of Materials Chemistry A, Vol. 7, Issue 39 https://doi.org/10.1039/c9ta09146g	journal	January 2019
3D lithiophilic–lithiophobic–lithiophilic dual-gradient porous skeleton for highly stable lithium metal anode Zheng, Hongfei; Zhang, Qingfei; Chen, Qiulin Journal of Materials Chemistry A, Vol. 8, Issue 1 https://doi.org/10.1039/c9ta09505e	journal	January 2020
Nitrogen-doped graphdiyne nanowall stabilized dendrite-free lithium metal anodes Jiang, Tao; Chen, Ke; Wang, Jingjing Journal of Materials Chemistry A, Vol. 7, Issue 48 https://doi.org/10.1039/c9ta09551a	journal	January 2019
Continuous plating/stripping behavior of solid-state lithium metal anode in a 3D ion-conductive framework Yang, Chunpeng; Zhang, Lei; Liu, Boyang Proceedings of the National Academy of Sciences, Vol. 115, Issue 15 https://doi.org/10.1073/pnas.1719758115	journal	March 2018
High-capacity rechargeable batteries based on deeply cyclable lithium metal anodes Shi, Qiuwei; Zhong, Yiren; Wu, Min Proceedings of the National Academy of Sciences, Vol. 115, Issue 22 https://doi.org/10.1073/pnas.1803634115	journal	May 2018
Review—Li Metal Anode in Working Lithium-Sulfur Batteries Cheng, Xin-Bing; Huang, Jia-Qi; Zhang, Qiang Journal of The Electrochemical Society, Vol. 165, Issue 1 https://doi.org/10.1149/2.0111801jes	journal	June 2017

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