A Water-Based Silver-Nanowire Screen-Print Ink for the Fabrication of Stretchable Conductors and Wearable Thin-Film Transistors

Liang, Jiajie; Tong, Kwing; Pei, Qibing

doi:10.1002/adma.201600772

Title: A Water-Based Silver-Nanowire Screen-Print Ink for the Fabrication of Stretchable Conductors and Wearable Thin-Film Transistors

Journal Article · Mon May 09 00:00:00 EDT 2016 · Advanced Materials

DOI:https://doi.org/10.1002/adma.201600772· OSTI ID:1429112

Liang, Jiajie ^[1]; Tong, Kwing ^[1]; Pei, Qibing ^[1]

Univ. of California, Los Angeles, CA (United States). Henry Samuli School of Engineering and Applied Science and Dept. of Materials Science and Engineering

Silver nanowire is a very promising material for fabricating compliant conductors which are essential for stretchable/wearable electronic devices. Screen printing is a cost-effective and scalable technology to fabricate large-area thin film coatings with modest pattern resolution. The biggest challenge to prepare a screen printable silver nanowire ink stems from the low viscosity of silver nanowire dispersions and that the addition of a thickening agent could dramatically increase the inter-nanowire contact resistance in the resulting coating. Herein, we report the synthesis of a water-based silver nanowire ink, which was formulated with low solid contents, high viscosity at 0.1 s^-1 shear rate, and appropriate rheological behavior suitable for screen printing. Silver nanowire coating patterns were screen printed with uniform sharp edges, ~50 μm resolution, and electrical conductivity as high as 4.67 × 10⁴ S cm^-1. The screen printed silver nanowires were then used to fabricate a composite conductor that retained a conductivity greater than 10,000 S cm^-1 under 70% tensile strain. Fully printed and stretchable/wearable thin-film transistor arrays were also fabricated by employing the screen printed composite conductor as the source, drain, and gate, drop cast semiconducting carbon nanotubes as the channel, and a dielectric elastomer. The 10 × 6 thin-film transistor arrays had a fabrication yield of 91.7%, average mobility of 33.8 ± 3.7 cm²V^-1s^-1, ON/OFF ratio ~1000, and remained stable during 1,000 cycles of wearing on and peeling off a glass tube with 5 mm diameter.

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Research Organization:: Univ. of California, Los Angeles, CA (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE)

Grant/Contract Number:: EE0006674; FA9550‐12‐1‐0074

OSTI ID:: 1429112

Journal Information:: Advanced Materials, Vol. 28, Issue 28; ISSN 0935-9648

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 372 works

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Screen printing of silver nanowires: balancing conductivity with transparency while maintaining flexibility and stretchability Li, Weiwei; Yang, Shuai; Shamim, Atif npj Flexible Electronics, Vol. 3, Issue 1 https://doi.org/10.1038/s41528-019-0057-1	journal	July 2019
High-Throughput Fabrication of Flexible and Transparent All-Carbon Nanotube Electronics Chen, Yong-Yang; Sun, Yun; Zhu, Qian-Bing Advanced Science, Vol. 5, Issue 5 https://doi.org/10.1002/advs.201700965	journal	February 2018
Highly reliable mulberry paper (Hanji)-based electrode with printed silver nanowire/zinc oxide hybrid for soft electronics Go, Myeongjong; Hwang, Byungil; Lim, Sooman Materials and Manufacturing Processes, Vol. 34, Issue 14 https://doi.org/10.1080/10426914.2019.1594266	journal	March 2019
Silver Nanoparticles Based Ink with Moderate Sintering in Flexible and Printed Electronics Mo, Lixin; Guo, Zhenxin; Yang, Li International Journal of Molecular Sciences, Vol. 20, Issue 9 https://doi.org/10.3390/ijms20092124	journal	April 2019
Copper nanomaterials and assemblies for soft electronics Feng, Yang; Zhu, Jian Science China Materials, Vol. 62, Issue 11 https://doi.org/10.1007/s40843-019-9468-5	journal	August 2019
Stretchable electronics: functional materials, fabrication strategies and applications Wu, Wei Science and Technology of Advanced Materials, Vol. 20, Issue 1 https://doi.org/10.1080/14686996.2018.1549460	journal	March 2019
Stretchable Organometal‐Halide‐Perovskite Quantum‐Dot Light‐Emitting Diodes Li, Yun‐Fei; Chou, Shu‐Yu; Huang, Peng Advanced Materials, Vol. 31, Issue 22 https://doi.org/10.1002/adma.201807516	journal	January 2019
Printing Conductive Nanomaterials for Flexible and Stretchable Electronics: A Review of Materials, Processes, and Applications Huang, Qijin; Zhu, Yong Advanced Materials Technologies, Vol. 4, Issue 5 https://doi.org/10.1002/admt.201800546	journal	January 2019
A Room-Temperature High-Conductivity Metal Printing Paradigm with Visible-Light Projection Lithography Yang, Xingyun; Sun, Mo; Bian, Yinxu Advanced Functional Materials, Vol. 29, Issue 1 https://doi.org/10.1002/adfm.201807615	journal	November 2018
Self-healing and superstretchable conductors from hierarchical nanowire assemblies Song, Pin; Qin, Haili; Gao, Huai-Ling Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-05238-w	journal	July 2018
Wireless Monitoring Using a Stretchable and Transparent Sensor Sheet Containing Metal Nanowires Araki, Teppei; Uemura, Takafumi; Yoshimoto, Shusuke Advanced Materials, Vol. 32, Issue 15 https://doi.org/10.1002/adma.201902684	journal	November 2019
Bistable and Reconfigurable Photonic Crystals-Electroactive Shape Memory Polymer Nanocomposite for Ink-Free Rewritable Paper Xie, Yu; Meng, Yuan; Wang, Wenxin Advanced Functional Materials, Vol. 28, Issue 34 https://doi.org/10.1002/adfm.201802430	journal	June 2018
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Highly Stretchable Metallic Nanowire Networks Reinforced by the Underlying Randomly Distributed Elastic Polymer Nanofibers via Interfacial Adhesion Improvement Jiang, Zhi; Nayeem, Md Osman Goni; Fukuda, Kenjiro Advanced Materials, Vol. 31, Issue 37 https://doi.org/10.1002/adma.201903446	journal	July 2019
A Metal‐Like Conductive Elastomer with a Hierarchical Wrinkled Structure Lee, Seokmin; Song, Yongkwon; Ko, Yongmin Advanced Materials, Vol. 32, Issue 7 https://doi.org/10.1002/adma.201906460	journal	November 2019
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Fabrication and Evaluation of a Novel Non-Invasive Stretchable and Wearable Respiratory Rate Sensor Based on Silver Nanoparticles Using Inkjet Printing Technology Al-Halhouli, Ala’aldeen; Al-Ghussain, Loiy; El Bouri, Saleem Polymers, Vol. 11, Issue 9 https://doi.org/10.3390/polym11091518	journal	September 2019
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Hydrous RuO ₂ ‐Decorated MXene Coordinating with Silver Nanowire Inks Enabling Fully Printed Micro‐Supercapacitors with Extraordinary Volumetric Performance Li, Hongpeng; Li, Xiran; Liang, Jiajie Advanced Energy Materials, Vol. 9, Issue 15 https://doi.org/10.1002/aenm.201803987	journal	February 2019
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Electric Field Assisted Self-Healing of Open Circuits with Conductive Particle-Insulating Fluid Dispersions: Optimizing Dispersion Concentration. Parab, Virendra; Prasad, Oppili; Pillai, Sreelal Apollo - University of Cambridge Repository https://doi.org/10.17863/cam.48551	text	January 2019
Water-Borne Perovskite Quantum Dot-Loaded, Polystyrene Latex Ink Huang, Keke; Peng, Lucheng; Liu, Baijun Frontiers in Chemistry, Vol. 6 https://doi.org/10.3389/fchem.2018.00453	journal	October 2018
Mechanisms and Materials of Flexible and Stretchable Skin Sensors Zhao, Yicong; Huang, Xian Micromachines, Vol. 8, Issue 3 https://doi.org/10.3390/mi8030069	journal	February 2017
Preparation of Nano Silver Paste and Applications in Transparent Electrodes via Electric-Field Driven Micro-Scale 3D Printing Li, Hongke; Zhu, Xiaoyang; Li, Zhenghao Nanomaterials, Vol. 10, Issue 1 https://doi.org/10.3390/nano10010107	journal	January 2020

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Title: A Water-Based Silver-Nanowire Screen-Print Ink for the Fabrication of Stretchable Conductors and Wearable Thin-Film Transistors

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