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Nematicity, magnetism and superconductivity in FeSe

Journal Article · · Journal of Physics. Condensed Matter
Iron-based superconductors are well known for their complex interplay between structure, magnetism and superconductivity. FeSe offers a particularly fascinating example. This material has been intensely discussed because of its extended nematic phase, whose relationship with magnetism is not obvious. Superconductivity in FeSe is highly tunable, with the superconducting transition temperature, T c, ranging from 8 K in bulk single crystals at ambient pressure to almost 40 K under pressure or in intercalated systems, and to even higher temperatures in thin films. In this topical review, we present an overview of nematicity, magnetism and superconductivity, and discuss the interplay of these phases in FeSe. We focus on bulk FeSe and the effects of physical pressure and chemical substitutions as tuning parameters. In conclusion, the experimental results are discussed in the context of the well-studied iron-pnictide superconductors and interpretations from theoretical approaches are presented.
Research Organization:
Ames Laboratory (AMES), Ames, IA (United States)
Sponsoring Organization:
USDOE
Grant/Contract Number:
AC02-07CH11358
OSTI ID:
1415833
Report Number(s):
IS-J--9539
Journal Information:
Journal of Physics. Condensed Matter, Journal Name: Journal of Physics. Condensed Matter Journal Issue: 2 Vol. 30; ISSN 0953-8984
Publisher:
IOP PublishingCopyright Statement
Country of Publication:
United States
Language:
English

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Spin Ferroquadrupolar Order in the Nematic Phase of FeSe journal June 2016
Thermal Conductivity of the Iron-Based Superconductor FeSe: Nodeless Gap with a Strong Two-Band Character journal August 2016
Origin of the Resistivity Anisotropy in the Nematic Phase of FeSe journal September 2016
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Evidence for Time-Reversal Symmetry Breaking of the Superconducting State near Twin-Boundary Interfaces in FeSe Revealed by Scanning Tunneling Spectroscopy journal August 2015
Nematicity and Magnetism in FeSe and Other Families of Fe-Based Superconductors journal June 2016
Magnetism, Superconductivity, and Spontaneous Orbital Order in Iron-Based Superconductors: Which Comes First and Why? journal December 2016
Prominent Role of Spin-Orbit Coupling in FeSe Revealed by Inelastic Neutron Scattering journal May 2017
Superconductivity in iron compounds journal December 2011
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Character of the structural and magnetic phase transitions in the parent and electron-doped BaFe 2 As 2 compounds journal April 2011
Magnetoelastic coupling in the phase diagram of Ba 1 − x K x Fe 2 As 2 as seen via neutron diffraction journal May 2011
Molecular-beam epitaxy and robust superconductivity of stoichiometric FeSe crystalline films on bilayer graphene journal July 2011
Coexistence of isotropic and extended s -wave order parameters in FeSe as revealed by low-temperature specific heat journal December 2011
Coexistence of superconductivity and magnetism in FeSe 1 − x under pressure journal February 2012
Anisotropic vortex lattice structures in the FeSe superconductor journal March 2012
Low-temperature phase diagram of Fe 1 + y Te studied using x-ray diffraction journal September 2013
Anomalous Fermi surface in FeSe seen by Shubnikov–de Haas oscillation measurements journal October 2014
Emergence of the nematic electronic state in FeSe journal April 2015
Resistivity and magnetoresistance of FeSe single crystals under helium-gas pressure journal May 2015
Origin of nematic order in FeSe journal May 2015
Observation of two distinct d x z / d y z band splittings in FeSe journal June 2015
Enhanced superconducting transition temperature in hyper-interlayer-expanded FeSe despite the suppressed electronic nematic order and spin fluctuations journal September 2015
Robust determination of the superconducting gap sign structure via quasiparticle interference journal November 2015
Momentum-dependent sign inversion of orbital order in superconducting FeSe journal November 2015
Superconductivity pairing mechanism from cobalt impurity doping in FeSe: Spin ( s ± ) or orbital ( s + + ) fluctuation journal January 2016
Nodal superconducting gap in tetragonal FeS journal March 2016
Interatomic Coulomb interaction and electron nematic bond order in FeSe journal March 2016
Coexistence of low-moment magnetism and superconductivity in tetragonal FeS and suppression of T c under pressure journal April 2016
Multiband superconductivity and large anisotropy in FeS crystals journal April 2016
Magnetotransport study of the pressure-induced antiferromagnetic phase in FeSe journal May 2016
Nematic antiferromagnetic states in bulk FeSe journal May 2016
Impurity scattering effects on the superconducting properties and the tetragonal-to-orthorhombic phase transition in FeSe journal June 2016
Enhancement of superconducting transition temperature by pointlike disorder and anisotropic energy gap in FeSe single crystals journal August 2016
Structural-transition-induced quasi-two-dimensional Fermi surface in FeSe journal October 2016
Orbital-dependent Fermi surface shrinking as a fingerprint of nematicity in FeSe journal October 2016
Interplay of nematic and magnetic orders in FeSe under pressure journal March 2017
Orbital selective pairing and gap structures of iron-based superconductors journal May 2017
Pressure-induced magnetic order in FeSe: A muon spin rotation study journal May 2017
Possible nematic spin liquid in spin-1 antiferromagnetic system on the square lattice: Implications for the nematic paramagnetic state of FeSe journal May 2017
Complex biphase nature of the superconducting dome of the FeSe phase diagram journal July 2017
Dome of magnetic order inside the nematic phase of sulfur-substituted FeSe under pressure journal July 2017
Superconducting gaps in FeSe studied by soft point-contact Andreev reflection spectroscopy journal September 2017
Optical anisotropy in the electronic nematic phase of FeSe journal September 2017
Tunable ( δ π , δ π )-Type Antiferromagnetic Order in α -Fe(Te,Se) Superconductors journal June 2009
Tetragonal-to-Orthorhombic Structural Phase Transition at 90 K in the Superconductor Fe 1.01 Se journal July 2009
Pressure Induced Static Magnetic Order in Superconducting FeSe 1 − x journal February 2010
Effects of Nematic Fluctuations on the Elastic Properties of Iron Arsenide Superconductors journal October 2010
Anisotropy of the In-Plane Resistivity of Underdoped Ba ( Fe 1 − x Co x ) 2 As 2 Superconductors Induced by Impurity Scattering in the Antiferromagnetic Orthorhombic Phase journal May 2013
Observation of Incipient Charge Nematicity in Ba ( Fe 1 − X Co X ) 2 As 2 journal December 2013
Nematic Susceptibility of Hole-Doped and Electron-Doped Ba F e 2 As 2 Iron-Based Superconductors from Shear Modulus Measurements journal January 2014
Model of Electronic Structure and Superconductivity in Orbitally Ordered FeSe journal July 2015
Dichotomy between the Hole and Electron Behavior in Multiband Superconductor FeSe Probed by Ultrahigh Magnetic Fields journal July 2015
Observation of Double-Dome Superconductivity in Potassium-Doped FeSe Thin Films journal April 2016
Sign-Reversing Orbital Polarization in the Nematic Phase of FeSe due to the C 2 Symmetry Breaking in the Self-Energy journal June 2016
Thermal Conductivity of the Iron-Based Superconductor FeSe: Nodeless Gap with a Strong Two-Band Character journal August 2016
Origin of the Resistivity Anisotropy in the Nematic Phase of FeSe journal September 2016
Coexistence of Replica Bands and Superconductivity in FeSe Monolayer Films journal February 2017
Magnetism, Superconductivity, and Spontaneous Orbital Order in Iron-Based Superconductors: Which Comes First and Why? journal December 2016
Prominent Role of Spin-Orbit Coupling in FeSe Revealed by Inelastic Neutron Scattering journal May 2017
Superconductivity in iron compounds journal December 2011
Nematic Electronic Structure in the “Parent” State of the Iron-Based Superconductor Ca(Fe 1– x Co x ) 2 As 2 journal January 2010
In-Plane Resistivity Anisotropy in an Underdoped Iron Arsenide Superconductor journal August 2010
Direct Observation of Nodes and Twofold Symmetry in FeSe Superconductor journal June 2011
Divergent Nematic Susceptibility in an Iron Arsenide Superconductor journal August 2012
Nematic spin correlations in the tetragonal state of uniaxial-strained BaFe2-xNixAs2 journal July 2014
Ubiquitous signatures of nematic quantum criticality in optimally doped Fe-based superconductors journal May 2016
Femtosecond electron-phonon lock-in by photoemission and x-ray free-electron laser journal July 2017
Discovery of orbital-selective Cooper pairing in FeSe journal July 2017
Evidence for Unconventional Superconductivity in Arsenic-Free Iron-Based Superconductor FeSe: A 77 Se-NMR Study journal November 2008
Precise Pressure Dependence of the Superconducting Transition Temperature of FeSe: Resistivity and 77 Se-NMR Study journal June 2009
Substitution Effects on FeSe Superconductor journal July 2009
Comparison of Ab initio Low-Energy Models for LaFePO, LaFeAsO, BaFe 2 As 2 , LiFeAs, FeSe, and FeTe: Electron Correlation and Covalency journal April 2010
Review of Fe Chalcogenides as the Simplest Fe-Based Superconductor journal October 2010
Orbital-Selective Superconductivity and the Effect of Lattice Distortion in Iron-Based Superconductors journal July 2011
Evidence for Unconventional Superconductivity in Arsenic-Free Iron-Based Superconductor FeSe: A 77 Se-NMR Study journal November 2008
Review of Fe Chalcogenides as the Simplest Fe-Based Superconductor journal October 2010
Monolayer FeSe on SrTiO 3 journal March 2017
FeAs-Based Superconductivity: A Case Study of the Effects of Transition Metal Doping on BaFe 2 As 2 journal August 2010
Acoustic characteristics of FeSe single crystals journal March 2013
Quantum oscillations and upper critical magnetic field of the iron-based superconductor FeSe journal January 2015
High-temperature superconductivity (T c onset at 34 K) in the high-pressure orthorhombic phase of FeSe journal April 2009
Anisotropic charge dynamics in detwinned Ba(Fe 1-x Co x ) 2 As 2 journal February 2011
High-temperature superconductivity in FeSe monolayers journal October 2016
High-temperature superconductivity in FeSe monolayers journal October 2016
Evidence for Time-Reversal Symmetry Breaking of the Superconducting State near Twin-Boundary Interfaces in FeSe Revealed by Scanning Tunneling Spectroscopy text January 2015
Substitution Effects on FeSe Superconductor text January 2008
Pairing Symmetry and Pairing State in Ferropnictides: Theoretical Overview text January 2009
Anion height dependence of Tc for the Fe-based superconductor text January 2010
High-temperature superconductivity in iron-based materials text January 2010
Shallow pockets and very strong coupling superconductivity in FeSe_xTe_1-x text January 2011
Anisotropic vortex lattice structures in the FeSe superconductor text January 2011
Manifestations of nematic degrees of freedom in the magnetic, elastic, and superconducting properties of the iron pnictides text January 2012
Anomalous superfluid density in quantum critical superconductors text January 2013
Lack of coupling between superconductivity and orthorhombic distortion in stoichiometric single-crystalline FeSe text January 2013
Direct observation of spin-orbit coupling in iron-based superconductors text January 2014
Neutron-scattering measurements of the spin excitations in LaFeAsO and Ba(Fe$_{0.953}$Co$_{0.047}$)$_{2}$As$_{2}$: Evidence for a sharp enhancement of spin fluctuations by nematic order text January 2014
Field-induced superconducting phase of FeSe in the BCS-BEC cross-over text January 2014
Antiferroquadrupolar and Ising-Nematic Orders of a Frustrated Bilinear-Biquadratic Heisenberg Model and Implications for the Magnetism of FeSe text January 2015
Strong Interplay between Stripe Spin Fluctuations, Nematicity and Superconductivity in FeSe text January 2015
Charge Nematicity and Electronic Raman Scattering in Iron-based Superconductors text January 2015
Structural transition and superconductivity in hydrothermally synthesized FeX (X = S, Se) text January 2015
Spin excitations in a model of FeSe with orbital ordering text January 2015
Strong anisotropy in nearly ideal-tetrahedral superconducting FeS single crystals text January 2015
Unveiling the hidden nematicity and spin subsystem in FeSe text January 2016
Nematic quantum critical point without magnetism in FeSe1-xSx superconductors text January 2016
High Temperature Superconductivity in FeSe Monolayers text January 2016
Interplay of nematic and magnetic orders in FeSe under pressure text January 2016
Interplay between magnetism, superconductivity, and orbital order in a 5-pocket model for iron-based superconductors - a parquet renormalization group study text January 2016
In-plane anisotropy of transport coefficients in the electronic nematic states: Universal origin of the nematicity in Fe-based superconductors text January 2016
Anomalous temperature evolution of the electronic structure of FeSe text January 2017
Strongly enhanced temperature dependence of the chemical potential in FeSe text January 2017
Monolayer FeSe on SrTiO$_3$ text January 2017
Suppression of electronic correlations by chemical pressure from FeSe to FeS text January 2017
NMR evidence for static local nematicity and its cooperative interplay with low-energy magnetic fluctuations in FeSe under pressure text January 2017
Pressure induced static magnetic order in superconducting FeSe_{1-x} text January 2010
Giant superconducting fluctuations in the compensated semimetal FeSe at the BCS-BEC crossover text January 2016
Effect of nematic ordering on electronic structure of FeSe text January 2016
Evidence for time-reversal symmetry breaking of the superconducting state near twin-boundary interfaces in FeSe revealed by scanning tunneling spectroscopy text January 2015
Enhanced Superconductivity on the Tetragonal Lattice in FeSe under Hydrostatic Pressure journal January 2014
Pressure-Induced Antiferromagnetic Transition and Phase Diagram in FeSe journal June 2015
Quasiparticle Excitations in the Superconducting State of FeSe Probed by Thermal Hall Conductivity in the Vicinity of the BCS–BEC Crossover journal January 2017
Shifts and Splittings of the Hole Bands in the Nematic Phase of FeSe journal May 2017
Enhanced Superconductivity on the Tetragonal Lattice in FeSe under Hydrostatic Pressure journal January 2014
Quasiparticle Excitations in the Superconducting State of FeSe Probed by Thermal Hall Conductivity in the Vicinity of the BCS–BEC Crossover journal January 2017

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Tuning the interplay between nematicity and spin fluctuations in Na1−xLi x FeAs superconductors journal May 2018
Measurements of elastoresistance under pressure by combining in-situ tunable quasi-uniaxial stress with hydrostatic pressure journal February 2020
Magnetoelastoresistance in WTe 2 : Exploring electronic structure and extremely large magnetoresistance under strain journal December 2019
A novel metastable state magnetic phase of monolayer FeSe journal March 2018
Intertwined spin-orbital coupled orders in the iron-based superconductors journal July 2019
Room temperature local nematicity in FeSe superconductor journal July 2019
Imaging anisotropic vortex dynamics in FeSe journal July 2019
Role of the Fermi surface for the pressure-tuned nematic transition in the BaFe 2 As 2 family journal August 2019
Distinct pressure evolution of coupled nematic and magnetic orders in FeSe journal August 2019
Disorder-induced electronic nematicity journal August 2019
Theory of two-fluid metallicity in superconducting FeSe at high pressure journal September 2019
Spin fluctuation anisotropy as a probe of orbital-selective hole-electron quasiparticle excitations in detwinned Ba ( Fe 1 − x Co x ) 2 As 2 journal October 2019
Lattice dynamics in FeSe via inelastic x-ray scattering and first-principles calculations journal January 2020
Evidence for short-range magnetic order in the nematic phase of FeSe from anisotropic in-plane magnetostriction and susceptibility measurements journal March 2018
Persistent correlation between superconductivity and antiferromagnetic fluctuations near a nematic quantum critical point in FeSe 1 − x S x journal July 2018
Itinerant approach to magnetic neutron scattering of FeSe: Effect of orbital selectivity journal December 2018
Superconductivity in FeSe: The Role of Nematic Order journal June 2018
Quantum Vortex Core and Missing Pseudogap in the Multiband BCS-BEC Crossover Superconductor FeSe journal February 2019
Evidence for an Fulde-Ferrell-Larkin-Ovchinnikov State with Segmented Vortices in the BCS-BEC-Crossover Superconductor FeSe journal March 2020
Nematicity and superconductivity in orthorhombic superconductor N a 0.35 ( C 3 N 2 H 10 ) 0.426 F e 2 S e 2 journal November 2018
Orbital transmutation and the electronic spectrum of FeSe in the nematic phase journal January 2020
Orbital Origin of Extremely Anisotropic Superconducting Gap in Nematic Phase of FeSe Superconductor journal August 2018
Probing the reconstructed Fermi surface of antiferromagnetic $BaFe_{2}As_{2}$ in one domain text January 2019
Nematicity of correlated systems driven by anisotropic chemical phase separation text January 2018
Orbital transmutation and the electronic spectrum of FeSe in the nematic phase text January 2019

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