Continuous‐Wave Lasing in Cesium Lead Bromide Perovskite Nanowires

Evans, Tyler J. S.; Schlaus, Andrew; Fu, Yongping; Zhong, Xinjue; Atallah, Timothy L.; Spencer, Michael S.; Brus, Louis E.; Jin, Song; Zhu, X. ‐Y.

doi:10.1002/adom.201700982

Title: Continuous‐Wave Lasing in Cesium Lead Bromide Perovskite Nanowires

Journal Article · Mon Dec 18 00:00:00 EST 2017 · Advanced Optical Materials

DOI:https://doi.org/10.1002/adom.201700982· OSTI ID:1413827

Evans, Tyler J. S. ^[1]; Schlaus, Andrew ^[1]; Fu, Yongping ^[2]; Zhong, Xinjue ^[1]; Atallah, Timothy L. ^[1]; Spencer, Michael S. ^[1]; Brus, Louis E. ^[1]; Jin, Song ^[2];

^[1]

Department of Chemistry Columbia University New York NY 10027 USA
Department of Chemistry University of Wisconsin‐Madison Madison WI 53706 USA

Abstract Lead halide perovskite nanowires (NWs) have been demonstrated in pulsed lasing with high quantum yields, low thresholds, and broad tunability. However, continuous‐wave (CW) lasing, necessary for many optoelectronic applications, has not been achieved to date. This is thought to be due to many‐body screening, which reduces the excitonic resonance enhancement of the oscillator strength at high excitation densities necessary for population inversion. Here CW lasing in CsPbBr ₃ perovskite NWs is reported. Analysis of the cavity modes and their temperature dependence reveals that both CW and pulsed lasing originate from polariton modes near the bottleneck region on the lower polariton branch, with a vacuum Rabi splitting of 0.20 ± 0.03 eV. These findings suggest that lead halide perovskite NWs may serve as low‐power CW coherent light sources and as model systems for polaritonics in the strong‐coupling regime.

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Sponsoring Organization:: USDOE

Grant/Contract Number:: SC0010692

OSTI ID:: 1413827

Journal Information:: Advanced Optical Materials, Journal Name: Advanced Optical Materials Vol. 6 Journal Issue: 2; ISSN 2195-1071

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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Cited by: 148 works

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