Materials for the Recovery of Uranium from Seawater

Abney, Carter W.; Mayes, Richard T.; Saito, Tomonori; Dai, Sheng

doi:10.1021/acs.chemrev.7b00355

Materials for the Recovery of Uranium from Seawater

Journal Article · Wed Nov 22 00:00:00 EST 2017 · Chemical Reviews

DOI:https://doi.org/10.1021/acs.chemrev.7b00355· OSTI ID:1412046

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Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

More than 1000× uranium exists in the oceans than exists in terrestrial ores. With nuclear power generation expected to increase over the coming decades, access to this unconventional reserve is a matter of energy security. With origins in the mid-1950’s, materials have been developed for the selective recovery of seawater uranium for more than six decades, with a renewed interest in particular since 2010. This review comprehensively surveys materials developed from 2000 – 2016 for recovery of seawater uranium, in particular including recent developments in inorganic materials, polymer adsorbents and related research pertaining to amidoxime, and nanostructured materials such as metal-organic frameworks, porous-organic polymers, and mesoporous carbons. In conclusion, challenges of performing reliable and reproducible uranium adsorption studies are also discussed, as well as the standardization of parameters necessary to ensure valid comparisons between different adsorbents.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Nuclear Energy (NE), Fuel Cycle Technologies (NE-5)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1412046

Journal Information:: Chemical Reviews, Journal Name: Chemical Reviews Journal Issue: 23 Vol. 117; ISSN 0009-2665

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Detailed characterization of dioxouranium( vi ) complexes with a symmetrical tetradentate N ₂ O ₂ -benzil bis(isonicotinoyl hydrazone) ligand Sethi, Sipun; Panigrahi, Rachita; Paul, Avijit Kumar Dalton Transactions, Vol. 49, Issue 30 https://doi.org/10.1039/d0dt02014a	journal	January 2020
A water-stable cyano-functionalized metal-organic framework as an efficient adsorbent of uranyl ion Peng, Ying; Zhang, Xiaowen; Wu, Xiaoyan Materials Research Express, Vol. 6, Issue 12 https://doi.org/10.1088/2053-1591/ab5415	journal	November 2019

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