Chapter 19: Catalysis by Metal Carbides and Nitrides

Schaidle, Joshua A; Nash, Connor P; Yung, Matthew M; Chen, Yuan; Carl, Sarah; Thompson, Levi

doi:10.1002/9783527691036.hsscvol6031

Chapter 19: Catalysis by Metal Carbides and Nitrides

Book · Wed Aug 09 04:00:00 EDT 2017

DOI:https://doi.org/10.1002/9783527691036.hsscvol6031· OSTI ID:1405917

Schaidle, Joshua A ^[1]; Nash, Connor P ^[1]; Yung, Matthew M ^[1]; Chen, Yuan ^[2]; Carl, Sarah ^[3]; Thompson, Levi ^[3]

National Renewable Energy Laboratory (NREL), Golden, CO (United States)
Pacific Northwest National Laboratory
University of Michigan

Early transition metal carbides and nitrides (ETMCNs), materials in which carbon or nitrogen occupies interstitial sites within a parent metal lattice, possess unique physical and chemical properties that motivate their use as catalysts. Specifically, these materials possess multiple types of catalytic sites, including metallic, acidic, and basic sites, and as such, exhibit reactivities that differ from their parent metals. Moreover, their surfaces are dynamic under reaction conditions. This chapter reviews recent (since 2010) experimental and computational investigations into the catalytic properties of ETMCN materials for applications including biomass conversion, syngas and CO2 upgrading, petroleum and natural gas refining, and electrocatalytic energy conversion, energy storage, and chemicals production, and attempts to link catalyst performance to active site identity/surface structure in order to elucidate the present level of understanding of structure-function relationships for these materials. The chapter concludes with a perspective on leveraging the unique properties of these materials to design and develop improved catalysts through a dedicated, multidisciplinary effort.

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Research Organization:: National Renewable Energy Laboratory (NREL), Golden, CO (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Bioenergy Technologies Office (EE-3B)

DOE Contract Number:: AC36-08GO28308

OSTI ID:: 1405917

Report Number(s):: NREL/CH-5100-67481

Country of Publication:: United States

Language:: English

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