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Impact of Stoichiometry on Structural and Optical Properties of Sputter Deposited Multicomponent Tellurite Glass Films

Journal Article · · Journal of the American Ceramic Society
DOI:https://doi.org/10.1111/jace.13534· OSTI ID:1400906
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  1. Department of Materials Science &, Engineering University of Delaware Newark Delaware 19716
  2. College of Optics and Photonics CREOL Department of Materials Science and Engineering University of Central Florida Orlando Florida 32816

Multicomponent TeO 2 –Bi 2 O 3 –ZnO ( TBZ ) glass thin films were prepared using RF magnetron sputtering under different oxygen flow rates. The influences of oxygen flow rate on the structural and optical properties of the resulting thin films were investigated. We observed that thin films sputtered in an oxygen‐rich environment are optically transparent while those sputtered in an oxygen‐deficient environment exhibit broadband absorption. The structural origin of the optical property variation was studied using X‐ray diffraction, X‐ray photoelectron spectroscopy, Raman Spectroscopy, and transmission electron microscopy which revealed that the presence of under‐coordinated Te leads to the observed optical absorption in oxygen‐deficient films.

Sponsoring Organization:
USDOE
Grant/Contract Number:
EE0005327
OSTI ID:
1400906
Journal Information:
Journal of the American Ceramic Society, Journal Name: Journal of the American Ceramic Society Journal Issue: 6 Vol. 98; ISSN 0002-7820
Publisher:
Wiley-BlackwellCopyright Statement
Country of Publication:
United States
Language:
English

References (51)

Diamond in Tellurite Glass: a New Medium for Quantum Information journal April 2011
Tellurite glass lasers operating close to 2 μ m journal March 2010
Optical Absorption of Tellurium Suboxide Thin Films journal April 1993
Glass Structure and Optical Nonlinearities in Thallium(I) Tellurium(IV) Oxide Glasses journal September 1999
Spectroscopic Properties of Rare Earth Metal Ion Doped Tellurium Oxide Glasses and Fibres journal September 2004
Raman spectra of TeO2-based glasses and glassy liquids: local structure change with temperature in relation to fragility of liquid journal November 1994
Optical second harmonic generation in poled MgOZnOTeO2 and B2O3TeO2 glasses journal August 1996
Optical absorption and structural characterization of reactively sputtered tellurium suboxide thin films journal March 1993
Tellurite glass: a new candidate for fiber devices journal August 1994
Intrinsic defects and glass stability in Er 3+ doped TeO 2 glasses and the implications for Er 3+ -doped tellurite fiber amplifiers journal October 2003
EXAFS of tellurium in the glasses of the B2O3TeO2 system journal January 1992
Raman spectra of MO1/2TeO2 (M = Li, Na, K, Rb, Cs and Tl) glasses journal January 1992
Dynamics and structure of TeO 2 polymorphs: model treatment of paratellurite and tellurite; Raman scattering evidence for new γ- and δ-phases journal April 2000
Optical waveguiding in amorphous tellurium oxide thin films journal November 2003
X-Ray photoelectron spectroscopy (XPS) studies of copper–sodium tellurite glasses journal January 2003
Impact of tellurite-based glass structure on Raman gain journal December 2012
Local structure and redox state of copper in tellurite glasses journal July 2004
Effect of ZnO and Bi2O3 addition on linear and non-linear optical properties of tellurite glasses journal March 2007
Remark on the optical gap in ZnO–Bi2O3–TeO2 glasses journal September 2007
Bridging, non-bridging and free (O2–) oxygen in Na2O-SiO2 glasses: An X-ray Photoelectron Spectroscopic (XPS) and Nuclear Magnetic Resonance (NMR) study journal January 2011
Influence of Bi2O3 content on the crystallization behavior of TeO2–Bi2O3–ZnO glass system journal March 2012
Structural and optical properties of Er3+-Yb3+ codoped multicomposition TeO2-ZnO-PbO-TiO2-Na2O glass journal February 2013
Er3+-doped tellurite waveguides deposited by excimer laser ablation journal December 2003
Processing and characterization of core–clad tellurite glass preforms and fibers fabricated by rotational casting journal March 2010
Optical, structural and photoelectron spectroscopic studies on amorphous and crystalline molybdenum oxide thin films journal May 2004
Deposition of TiO2 thin films using RF magnetron sputtering method and study of their surface characteristics journal March 2005
δ-Bi2O3 thin films prepared by reactive sputtering: Fabrication and characterization journal August 2006
Tungsten–tellurite glasses and thin films doped with rare-earth elements produced by radio frequency magnetron deposition journal April 2008
Inner-orbital binding-energy shifts of antimony and bismuth compounds journal April 1973
Preparation of TeO2-TiO2 thin films by sol-gel process journal January 1999
Integrated flexible chalcogenide glass photonic devices journal June 2014
UV-IR spectra of new tellurite glasses journal September 2002
Parameterization of the optical functions of amorphous materials in the interband region journal July 1996
Sputtered stoichiometric TeO2 glass films: Dispersion of linear and nonlinear optical properties journal August 2003
Enhanced Raman gain coefficients and bandwidths in P2O5 and WO3 added tellurite glasses for Raman gain media journal September 2006
Influence of modifier oxides on the structural and optical properties of binary TeO2 glasses journal January 2007
Growth of amorphous TeOx (2≤x≤3) thin film by radio frequency sputtering journal April 2007
Higher nonlinear indices, Raman gain coefficients, and bandwidths in the TeO2–ZnO–Nb2O5–MoO3 quaternary glass system journal May 2007
B-spline parametrization of the dielectric function applied to spectroscopic ellipsometry on amorphous carbon journal December 2009
Pulsed Laser Deposition of Er doped tellurite films on large area journal April 2007
Spectroscopic Analysis of the Structure and Properties of Alkali Tellurite Glasses journal February 1992
Nonlinear Optical Properties of TeO2-Based Glasses: MOx-TeO2 (M = Sc, Ti, V, Nb, Mo, Ta, and W) Binary Glasses journal April 1995
Processing of Tellurite-Based Glass with Low OH Content: Processing of Tellurite-Based Glass journal September 2010
X‐ray photoelectron and Auger electron spectroscopic study of the CdTe surface resulting from various surface pretreatments: Correlation of photoelectrochemical and capacitance‐potential behavior with surface chemical composition
  • Ricco, Antonio J.; White, Henry S.; Wrighton, Mark S.
  • Journal of Vacuum Science & Technology A: Vacuum, Surfaces, and Films, Vol. 2, Issue 2 https://doi.org/10.1116/1.572547
journal April 1984
Estimation of peak Raman gain coefficients for Barium-Bismuth-Tellurite glasses from spontaneous Raman cross-section experiments journal January 2009
Index matching between passive and active tellurite glasses for use in microstructured fiber lasers: Erbium doped lanthanum-tellurite glass journal January 2009
Very low loss reactively ion etched Tellurium Dioxide planar rib waveguides for linear and non-linear optics journal January 2009
Engineering broadband and anisotropic photoluminescence emission from rare earth doped tellurite thin film photonic crystals journal January 2012
Tellurite microspheres for nanoparticle sensing and novel light sources journal January 2014
Large second-order nonlinearity in poled fused silica journal January 1991
Flexible integrated photonics: where materials, mechanics and optics meet [Invited] journal January 2013

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