Re Doping in 2D Transition Metal Dichalcogenides as a New Route to Tailor Structural Phases and Induced Magnetism

Kochat, Vidya; Apte, Amey; Hachtel, Jordan A.; Kumazoe, Hiroyuki; Krishnamoorthy, Aravind; Susarla, Sandhya; Idrobo, Juan Carlos; Shimojo, Fuyuki; Vashishta, Priya; Kalia, Rajiv; Nakano, Aiichiro; Tiwary, Chandra Sekhar; Ajayan, Pulickel M.

doi:10.1002/adma.201703754

Title: Re Doping in 2D Transition Metal Dichalcogenides as a New Route to Tailor Structural Phases and Induced Magnetism

Journal Article · Mon Oct 09 00:00:00 EDT 2017 · Advanced Materials

DOI:https://doi.org/10.1002/adma.201703754· OSTI ID:1423052

Kochat, Vidya ^[1]; Apte, Amey ^[1]; Hachtel, Jordan A. ^[2]; Kumazoe, Hiroyuki ^[3]; Krishnamoorthy, Aravind ^[4]; Susarla, Sandhya ^[1]; Idrobo, Juan Carlos ^[2]; Shimojo, Fuyuki ^[5]; Vashishta, Priya ^[4]; Kalia, Rajiv ^[4]; Nakano, Aiichiro ^[4];

^[1]; Ajayan, Pulickel M. ^[1]

Rice Univ., Houston, TX (United States). Materials Science and Nano Engineering
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences
Univ. of Southern California, Los Angeles, CA (United States). Collaboratory for Advanced Computing and Simulations; Kumamoto Univ. (Japan). Dept. of Physics
Univ. of Southern California, Los Angeles, CA (United States). Collaboratory for Advanced Computing and Simulations
Kumamoto Univ. (Japan). Dept. of Physics

Alloying in 2D results in the development of new, diverse, and versatile systems with prospects in bandgap engineering, catalysis, and energy storage. Tailoring structural phase transitions using alloying is a novel idea with implications in designing all 2D device architecture as the structural phases in 2D materials such as transition metal dichalcogenides are correlated with electronic phases. In this paper, this study develops a new growth strategy employing chemical vapor deposition to grow monolayer 2D alloys of Re-doped MoSe₂ with show composition tunable structural phase variations. The compositions where the phase transition is observed agree well with the theoretical predictions for these 2D systems. Finally, it is also shown that in addition to the predicted new electronic phases, these systems also provide opportunities to study novel phenomena such as magnetism which broadens the range of their applications.

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Research Organization:: Univ. of Southern California, Los Angeles, CA (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States); Rice Univ., Houston, TX (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725; SC0014607

OSTI ID:: 1423052

Alternate ID(s):: OSTI ID: 1398722

Journal Information:: Advanced Materials, Vol. 29, Issue 43; ISSN 0935-9648

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 150 works

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Title: Re Doping in 2D Transition Metal Dichalcogenides as a New Route to Tailor Structural Phases and Induced Magnetism

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