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Title: Spin dynamics in the stripe-ordered buckled honeycomb lattice antiferromagnet Ba 2 NiTeO 6

Abstract

We carried out inelastic neutron scattering experiments on a buckled honeycomb lattice antiferromagnet Ba 2NiTeO 6 exhibiting a stripe structure at a low temperature. Magnetic excitations are observed in the energy range of ℏω≲10 meV having an anisotropy gap of 2 meV at 2 K. We perform spin-wave calculations to identify the spin model. The obtained microscopic parameters are consistent with the location of the stripe structure in the classical phase diagram. Furthermore, the Weiss temperature independently estimated from a bulk magnetic susceptibility is consistent with the microscopic parameters. The results reveal that a competition between the nearest-neighbor and next-nearest-neighbor interactions that together with a relatively large single-ion magnetic anisotropy stabilize the stripe magnetic structure.

Authors:
 [1];  [1];  [2];  [2]; ORCiD logo [3]; ORCiD logo [3];  [1]
  1. Univ. of Tokyo (Japan). Inst. for Solid State Physics
  2. Osaka Prefecture Univ., Sakai, Osaka, (Japan). Dept. of Physical Science
  3. Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Quantum Condensed Matter Division
Publication Date:
Research Org.:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Org.:
USDOE Office of Science (SC)
OSTI Identifier:
1394594
Alternate Identifier(s):
OSTI ID: 1389672
Grant/Contract Number:  
AC05-00OR22725; IPTS-13701.1
Resource Type:
Journal Article: Accepted Manuscript
Journal Name:
Physical Review B
Additional Journal Information:
Journal Volume: 96; Journal Issue: 10; Journal ID: ISSN 2469-9950
Publisher:
American Physical Society (APS)
Country of Publication:
United States
Language:
English
Subject:
72 PHYSICS OF ELEMENTARY PARTICLES AND FIELDS

Citation Formats

Asai, Shinichiro, Soda, Minoru, Kasatani, Kazuhiro, Ono, Toshio, Garlea, Vasile Ovidiu, Winn, Barry L., and Masuda, Takatsugu. Spin dynamics in the stripe-ordered buckled honeycomb lattice antiferromagnet Ba2NiTeO6. United States: N. p., 2017. Web. doi:10.1103/PhysRevB.96.104414.
Asai, Shinichiro, Soda, Minoru, Kasatani, Kazuhiro, Ono, Toshio, Garlea, Vasile Ovidiu, Winn, Barry L., & Masuda, Takatsugu. Spin dynamics in the stripe-ordered buckled honeycomb lattice antiferromagnet Ba2NiTeO6. United States. doi:10.1103/PhysRevB.96.104414.
Asai, Shinichiro, Soda, Minoru, Kasatani, Kazuhiro, Ono, Toshio, Garlea, Vasile Ovidiu, Winn, Barry L., and Masuda, Takatsugu. Fri . "Spin dynamics in the stripe-ordered buckled honeycomb lattice antiferromagnet Ba2NiTeO6". United States. doi:10.1103/PhysRevB.96.104414. https://www.osti.gov/servlets/purl/1394594.
@article{osti_1394594,
title = {Spin dynamics in the stripe-ordered buckled honeycomb lattice antiferromagnet Ba2NiTeO6},
author = {Asai, Shinichiro and Soda, Minoru and Kasatani, Kazuhiro and Ono, Toshio and Garlea, Vasile Ovidiu and Winn, Barry L. and Masuda, Takatsugu},
abstractNote = {We carried out inelastic neutron scattering experiments on a buckled honeycomb lattice antiferromagnet Ba2NiTeO6 exhibiting a stripe structure at a low temperature. Magnetic excitations are observed in the energy range of ℏω≲10 meV having an anisotropy gap of 2 meV at 2 K. We perform spin-wave calculations to identify the spin model. The obtained microscopic parameters are consistent with the location of the stripe structure in the classical phase diagram. Furthermore, the Weiss temperature independently estimated from a bulk magnetic susceptibility is consistent with the microscopic parameters. The results reveal that a competition between the nearest-neighbor and next-nearest-neighbor interactions that together with a relatively large single-ion magnetic anisotropy stabilize the stripe magnetic structure.},
doi = {10.1103/PhysRevB.96.104414},
journal = {Physical Review B},
number = 10,
volume = 96,
place = {United States},
year = {Fri Sep 01 00:00:00 EDT 2017},
month = {Fri Sep 01 00:00:00 EDT 2017}
}

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