Design of radiation resistant metallic multilayers for advanced nuclear systems

Zhernenkov, Mikhail; Gill, Simerjeet; Stanic, Vesna; DiMasi, Elaine; Kisslinger, Kim; Baldwin, J. Kevin; Misra, Amit; Demkowicz, M. J.; Ecker, Lynne

doi:10.1063/1.4883481

Design of radiation resistant metallic multilayers for advanced nuclear systems

Journal Article · Tue Jun 17 00:00:00 EDT 2014 · Applied Physics Letters

DOI:https://doi.org/10.1063/1.4883481· OSTI ID:1384372

Zhernenkov, Mikhail ^[1]; Gill, Simerjeet ^[1]; Stanic, Vesna ^[1]; DiMasi, Elaine ^[1]; Kisslinger, Kim ^[1]; Baldwin, J. Kevin ^[2]; Misra, Amit ^[2]; Demkowicz, M. J. ^[3]; Ecker, Lynne ^[1]

Brookhaven National Lab. (BNL), Upton, NY (United States)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Massachusetts Inst. of Technology (MIT), Cambridge, MA (United States)

Helium implantation from transmutation reactions is a major cause of embrittlement and dimensional instability of structural components in nuclear energy systems. Development of novel materials with improved radiation resistance, which is of the utmost importance for progress in nuclear energy, requires guidelines to arrive at favorable parameters more efficiently. Here, we present a methodology that can be used for the design of radiation tolerant materials. We used synchrotron X-ray reflectivity to nondestructively study radiation effects at buried interfaces and measure swelling induced by He implantation in Cu/Nb multilayers. The results, supported by transmission electron microscopy, show a direct correlation between reduced swelling in nanoscale multilayers and increased interface area per unit volume, consistent with helium storage in Cu/Nb interfaces in forms that minimize dimensional changes. In addition, for Cu/Nb layers, a linear relationship is demonstrated between the measured depth-dependent swelling and implanted He density from simulations, making the reflectivity technique a powerful tool for heuristic material design.

View Accepted Manuscript (DOE)

Research Organization:: Energy Frontier Research Centers (EFRC) (United States). Center for Materials at Irradiation and Mechanical Extremes (CMIME)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

OSTI ID:: 1384372

Journal Information:: Applied Physics Letters, Journal Name: Applied Physics Letters Journal Issue: 24 Vol. 104; ISSN 0003-6951

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

References (28)

Design of Radiation Tolerant Materials Via Interface Engineering Han, Weizhong; Demkowicz, Michael J.; Mara, Nathan A. Advanced Materials, Vol. 25, Issue 48 https://doi.org/10.1002/adma.201303400	journal	September 2013
Neutron irradiation effects on copper at 327° C Adamson, R. B.; Bell, W. L.; Kelly, P. C. Journal of Nuclear Materials, Vol. 92, Issue 1 https://doi.org/10.1016/0022-3115(80)90153-1	journal	August 1980
Nucleation of helium bubbles on dislocations, dislocation networks and dislocations in grain boundaries during 600 MeV proton irradiation of aluminium Singh, B. N.; Leffers, T.; Green, W. V. Journal of Nuclear Materials, Vol. 125, Issue 3 https://doi.org/10.1016/0022-3115(84)90556-7	journal	August 1984
Void swelling and defect cluster formation in reactor-irradiated copper Zinkle, S. J.; Farrell, K. Journal of Nuclear Materials, Vol. 168, Issue 3 https://doi.org/10.1016/0022-3115(89)90591-6	journal	December 1989
Nuclear reactor materials at the atomic scale Marquis, Emmanuelle A.; Hyde, Jonathan M.; Saxey, David W. Materials Today, Vol. 12, Issue 11 https://doi.org/10.1016/S1369-7021(09)70296-2	journal	November 2009
Effect of grain boundary character on sink efficiency Han, W. Z.; Demkowicz, M. J.; Fu, E. G. Acta Materialia, Vol. 60, Issue 18 https://doi.org/10.1016/j.actamat.2012.08.009	journal	October 2012
The role of interface structure in controlling high helium concentrations Demkowicz, M. J.; Misra, A.; Caro, A. Current Opinion in Solid State and Materials Science, Vol. 16, Issue 3 https://doi.org/10.1016/j.cossms.2011.10.003	journal	June 2012
Defect structures and hardening mechanisms in high dose helium ion implanted Cu and Cu/Nb multilayer thin films Li, N.; Nastasi, M.; Misra, A. International Journal of Plasticity, Vol. 32-33 https://doi.org/10.1016/j.ijplas.2011.12.007	journal	May 2012
Helium transport, fate and management in nanostructured ferritic alloys: In situ helium implanter studies Odette, G. R.; Miao, P.; Edwards, D. J. Journal of Nuclear Materials, Vol. 417, Issue 1-3 https://doi.org/10.1016/j.jnucmat.2011.01.064	journal	October 2011
Radiation damage tolerant nanomaterials Beyerlein, I. J.; Caro, A.; Demkowicz, M. J. Materials Today, Vol. 16, Issue 11 https://doi.org/10.1016/j.mattod.2013.10.019	journal	November 2013
Nanostructured Cu/Nb multilayers subjected to helium ion-irradiation Zhang, X.; Li, Nan; Anderoglu, O. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 261, Issue 1-2 https://doi.org/10.1016/j.nimb.2007.03.098	journal	August 2007
Bubble formation at grain boundaries in helium implanted copper Thorsen, P. A.; Bilde-Sørensen, J. B.; Singh, B. N. Scripta Materialia, Vol. 51, Issue 6 https://doi.org/10.1016/j.scriptamat.2004.05.038	journal	September 2004
A Transmission Electron Microscopy Study of the Effect of Interfaces on Bubble Formation in He-Implanted Cu-Nb Multilayers Bhattacharyya, D.; Demkowicz, M. J.; Wang, Y. -Q. Microscopy and Microanalysis, Vol. 18, Issue 1 https://doi.org/10.1017/S1431927611012219	journal	January 2012
Are Nanoporous Materials Radiation Resistant? Bringa, E. M.; Monk, J. D.; Caro, A. Nano Letters, Vol. 12, Issue 7 https://doi.org/10.1021/nl201383u	journal	June 2011
Removal of stacking-fault tetrahedra by twin boundaries in nanotwinned metals Yu, K. Y.; Bufford, D.; Sun, C. Nature Communications, Vol. 4, Issue 1 https://doi.org/10.1038/ncomms2382	journal	January 2013
Influence of interfaces on the storage of ion-implanted He in multilayered metallic composites Höchbauer, T.; Misra, A.; Hattar, K. Journal of Applied Physics, Vol. 98, Issue 12 https://doi.org/10.1063/1.2149168	journal	December 2005
The effect of excess atomic volume on He bubble formation at fcc–bcc interfaces Demkowicz, M. J.; Bhattacharyya, D.; Usov, I. Applied Physics Letters, Vol. 97, Issue 16 https://doi.org/10.1063/1.3502594	journal	October 2010
A first-principles study of helium storage in oxides and at oxide–iron interfaces Erhart, Paul Journal of Applied Physics, Vol. 111, Issue 11 https://doi.org/10.1063/1.4707944	journal	June 2012
Detection of helium bubble formation at fcc-bcc interfaces using neutron reflectometry Kashinath, A.; Wang, P.; Majewski, J. Journal of Applied Physics, Vol. 114, Issue 4 https://doi.org/10.1063/1.4813780	journal	July 2013
Modification of radiation damage microstructure by helium Farrell, K.; Maziasz, P. J.; Lee, E. H. Radiation Effects, Vol. 78, Issue 1-4 https://doi.org/10.1080/00337578308207378	journal	January 1983
Helium bubble nucleation at grain boundaries Lane, P. L.; Goodhew, P. J. Philosophical Magazine A, Vol. 48, Issue 6 https://doi.org/10.1080/01418618308244330	journal	December 1983
Nucleation and growth of bubbles in He ion-implanted V/Ag multilayers Wei, Q. M.; Wang, Y. Q.; Nastasi, M. Philosophical Magazine, Vol. 91, Issue 4 https://doi.org/10.1080/14786435.2010.526647	journal	February 2011
Effect of grain size on void formation during high-energy electron irradiation of austenitic stainless steel Singh, B. N. The Philosophical Magazine: A Journal of Theoretical Experimental and Applied Physics, Vol. 29, Issue 1 https://doi.org/10.1080/14786437408213551	journal	January 1974
Tunable helium bubble superlattice ordered by screw dislocation network Di, Zengfeng; Bai, Xian-Ming; Wei, Qiangmin Physical Review B, Vol. 84, Issue 5 https://doi.org/10.1103/PhysRevB.84.052101	journal	August 2011
Stable Storage of Helium in Nanoscale Platelets at Semicoherent Interfaces Kashinath, A.; Misra, A.; Demkowicz, M. J. Physical Review Letters, Vol. 110, Issue 8 https://doi.org/10.1103/PhysRevLett.110.086101	journal	February 2013
One-Dimensional Fast Migration of Vacancy Clusters in Metals Matsukawa, Y.; Zinkle, S. J. Science, Vol. 318, Issue 5852 https://doi.org/10.1126/science.1148336	journal	November 2007
Recent Developments in Irradiation-Resistant Steels Odette, G. R.; Alinger, M. J.; Wirth, B. D. Annual Review of Materials Research, Vol. 38, Issue 1, p. 471-503 https://doi.org/10.1146/annurev.matsci.38.060407.130315	journal	August 2008
A first-principles study of helium storage in oxides and at oxide--iron interfaces Erhart, Paul arXiv https://doi.org/10.48550/arxiv.1109.0433	text	January 2011

Cited By (2)

Carbon Nanotubes Enhance the Radiation Resistance of bcc Iron Revealed by Atomistic Study Liu, Shuzhuang; Xie, Lu; Peng, Qing Materials, Vol. 12, Issue 2 https://doi.org/10.3390/ma12020217	journal	January 2019
Helium Irradiation and Implantation Effects on the Structure of Amorphous Silicon Oxycarbide Su, Qing; Inoue, Shinsuke; Ishimaru, Manabu Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/s41598-017-04247-x	journal	June 2017

Similar Records

Design of radiation resistant metallic multilayers for advanced nuclear systems

Journal Article · Mon Jun 16 00:00:00 EDT 2014 · Applied Physics Letters · OSTI ID:22299885

Influence of interfaces on the storage of ion-implanted He in multilayered metallic composites

Journal Article · Wed Dec 14 23:00:00 EST 2005 · Journal of Applied Physics · OSTI ID:20787724

A Transmission Electron Microscopy Study of the Effect of Interfaces on Bubble Formation in He-Implanted Cu-Nb Multilayers

Journal Article · Tue Jan 17 23:00:00 EST 2012 · Microscopy and Microanalysis · OSTI ID:1387016

Related Subjects

36 MATERIALS SCIENCE
defects
materials and chemistry by design
mechanical behavior
nuclear (including radiation effects)
synthesis (novel materials)
synthesis (scalable processing)

Design of radiation resistant metallic multilayers for advanced nuclear systems

Citation Formats

References (28)

Cited By (2)

Similar Records

Related Subjects