Probing 5f -state configurations in URu2Si2 with U LIII -edge resonant x-ray emission spectroscopy

Booth, Corwin H.; Medling, S. A.; Tobin, J. G.; Baumbach, Ryan E.; Bauer, Eric Dietzgen; Sokaras, D.; Nordlund, D.; Weng, T. -C.

doi:10.1103/PhysRevB.94.045121

Title: Probing $5 f$ -state configurations in ${URu}_{2} {Si}_{2}$ with U $L_{III}$ -edge resonant x-ray emission spectroscopy

Journal Article · Fri Jul 15 00:00:00 EDT 2016 · Physical Review B

DOI:https://doi.org/10.1103/PhysRevB.94.045121· OSTI ID:1379516

Booth, Corwin H. ^[1]; Medling, S. A. ^[2]; Tobin, J. G. ^[3]; Baumbach, Ryan E. ^[4];

^[5]; Sokaras, D. ^[6]; Nordlund, D. ^[6]; Weng, T. -C. ^[7]

Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Australian National Univ., Canberra (Australia)
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States); Univ. of Wisconsin-Oshkosh, WI (United States)
National High Magnetic Field Lab., Tallahassee, FL (United States); Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
SLAC National Accelerator Lab., Menlo Park, CA (United States)
SLAC National Accelerator Lab., Menlo Park, CA (United States); Center for High Pressure Science & Technology Advanced Research, Shanghai (People's Republic of China)

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Research Organization:: Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States); Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC). Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC02-05CH11231; AC52-07NA27344; AC02-76SF00515; AC52-06NA25396

OSTI ID:: 1379516

Alternate ID(s):: OSTI ID: 1263696; OSTI ID: 1407893

Report Number(s):: LA-UR-17-24462; PRBMDO; ark:/13030/qt2xm6690f; TRN: US1702696

Journal Information:: Physical Review B, Vol. 94, Issue 4; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 23 works

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References (73)

The crystal structure of UF ₄ Larson, A. C.; Roof, R. B.; Cromer, D. T. Acta Crystallographica, Vol. 17, Issue 5 https://doi.org/10.1107/S0365110X64001293	journal	May 1964
Imaging the Three-Dimensional Fermi-Surface Pairing near the Hidden-Order Transition in ${URu}_{2} {Si}_{2}$ Using Angle-Resolved Photoemission Spectroscopy Meng, Jian-Qiao; Oppeneer, Peter M.; Mydosh, John A. Physical Review Letters, Vol. 111, Issue 12 https://doi.org/10.1103/PhysRevLett.111.127002	journal	September 2013
Delocalization and occupancy effects of 5f orbitals in plutonium intermetallics using L3-edge resonant X-ray emission spectroscopy Booth, C. H.; Medling, S. A.; Jiang, Yu Journal of Electron Spectroscopy and Related Phenomena, Vol. 194 https://doi.org/10.1016/j.elspec.2014.03.004	journal	June 2014
Coherence Scale of the Kondo Lattice Burdin, S.; Georges, A.; Grempel, D. R. Physical Review Letters, Vol. 85, Issue 5 https://doi.org/10.1103/PhysRevLett.85.1048	journal	July 2000
Hastatic order in the heavy-fermion compound URu2Si2 Chandra, Premala; Coleman, Piers; Flint, Rebecca Nature, Vol. 493, Issue 7434 https://doi.org/10.1038/nature11820	journal	January 2013
Total and partial atomic-level widths Keski-Rahkonen, Olavi; Krause, Manfred O. Atomic Data and Nuclear Data Tables, Vol. 14, Issue 2 https://doi.org/10.1016/S0092-640X(74)80020-3	journal	August 1974
Magnetic excitations and ordering in the heavy-electron superconductor ${URu}_{2}$ ${Si}_{2}$ Broholm, C.; Kjems, J. K.; Buyers, W. J. L. Physical Review Letters, Vol. 58, Issue 14 https://doi.org/10.1103/PhysRevLett.58.1467	journal	April 1987
Electronic Structure of Heavy Fermion Uranium Compounds Studied by Core-Level Photoelectron Spectroscopy Fujimori, Shin-ichi; Ohkochi, Takuo; Kawasaki, Ikuto Journal of the Physical Society of Japan, Vol. 81, Issue 1 https://doi.org/10.1143/JPSJ.81.014703	journal	January 2012
Partially gapped Fermi surface in the heavy-electron superconductor ${URu}_{2}$ ${Si}_{2}$ Maple, M. B.; Chen, J. W.; Dalichaouch, Y. Physical Review Letters, Vol. 56, Issue 2 https://doi.org/10.1103/PhysRevLett.56.185	journal	January 1986
High energy resolution x-ray absorption spectroscopy study of uranium in varying valence states Vitova, T.; Kvashnina, K. O.; Nocton, G. Physical Review B, Vol. 82, Issue 23 https://doi.org/10.1103/PhysRevB.82.235118	journal	December 2010
Two Fluid Description of the Kondo Lattice Nakatsuji, Satoru; Pines, David; Fisk, Zachary Physical Review Letters, Vol. 92, Issue 1 https://doi.org/10.1103/PhysRevLett.92.016401	journal	January 2004
Oxidation and crystal field effects in uranium Tobin, J. G.; Yu, S. -W.; Booth, C. H. Physical Review B, Vol. 92, Issue 3 https://doi.org/10.1103/PhysRevB.92.035111	journal	July 2015
Spectroscopic Determination of the Atomic $f$ -Electron Symmetry Underlying Hidden Order in ${URu}_{2} {Si}_{2}$ Wray, L. Andrew; Denlinger, Jonathan; Huang, Shih-Wen Physical Review Letters, Vol. 114, Issue 23 https://doi.org/10.1103/PhysRevLett.114.236401	journal	June 2015
Slow crossover in $Yb X {Cu}_{4}$ ( X =Ag, Cd, In, Mg, Tl, Zn) intermediate-valence compounds Lawrence, J. M.; Riseborough, P. S.; Booth, C. H. Physical Review B, Vol. 63, Issue 5 https://doi.org/10.1103/PhysRevB.63.054427	journal	January 2001
Parameter-free calculations of X-ray spectra with FEFF9 Rehr, John J.; Kas, Joshua J.; Vila, Fernando D. Physical Chemistry Chemical Physics, Vol. 12, Issue 21 https://doi.org/10.1039/b926434e	journal	January 2010
Multiconfigurational nature of 5f orbitals in uranium and plutonium intermetallics Booth, C. H.; Jiang, Y.; Wang, D. L. Proceedings of the National Academy of Sciences, Vol. 109, Issue 26 https://doi.org/10.1073/pnas.1200725109	journal	June 2012
Thermal Transport in the Hidden-Order State of ${URu}_{2} {Si}_{2}$ Behnia, K.; Bel, R.; Kasahara, Y. Physical Review Letters, Vol. 94, Issue 15 https://doi.org/10.1103/PhysRevLett.94.156405	journal	April 2005
On the valence fluctuation in the early actinide metals Söderlind, P.; Landa, A.; Tobin, J. G. Journal of Electron Spectroscopy and Related Phenomena, Vol. 207 https://doi.org/10.1016/j.elspec.2015.11.014	journal	February 2016
Hexadecapolar Kondo Effect in $U {Ru}_{2} S i_{2}$ ? Tóth, Anna I.; Kotliar, Gabriel Physical Review Letters, Vol. 107, Issue 26 https://doi.org/10.1103/PhysRevLett.107.266405	journal	December 2011
Evolution from first-order valence transition to heavy-fermion behavior in ${YbIn}_{1 - x}$ ${Ag}_{x}$ ${Cu}_{4}$ Sarrao, J. L.; Immer, C. D.; Benton, C. L. Physical Review B, Vol. 54, Issue 17 https://doi.org/10.1103/PhysRevB.54.12207	journal	November 1996
Colloquium : Hidden order, superconductivity, and magnetism: The unsolved case of ${URu}_{2} {Si}_{2}$ Mydosh, J. A.; Oppeneer, P. M. Reviews of Modern Physics, Vol. 83, Issue 4 https://doi.org/10.1103/RevModPhys.83.1301	journal	November 2011
Photoemission investigations of URu ₂ Si ₂ Durakiewicz, Tomasz Philosophical Magazine, Vol. 94, Issue 32-33 https://doi.org/10.1080/14786435.2014.937783	journal	July 2014
Inflection Point in the Magnetic Field Dependence of the Ordered Moment of ${U R u}_{2} {S i}_{2}$ Observed by Neutron Scattering in Fields up to 17 T Bourdarot, F.; Fåk, B.; Habicht, K. Physical Review Letters, Vol. 90, Issue 6 https://doi.org/10.1103/PhysRevLett.90.067203	journal	February 2003
Fluctuation effects in mixed-valence systems at zero temperature Kohn, W.; Lee, T. K. Philosophical Magazine A, Vol. 45, Issue 2 https://doi.org/10.1080/01418618208244303	journal	February 1982
Hidden order behaviour in URu ₂ Si ₂ (A critical review of the status of hidden order in 2014) Mydosh, J. A.; Oppeneer, P. M. Philosophical Magazine, Vol. 94, Issue 32-33 https://doi.org/10.1080/14786435.2014.916428	journal	May 2014
Effect of Mott-Hubbard correlations on the electronic structure and structural stability of uranium dioxide Dudarev, S. L.; Manh, D. Nguyen; Sutton, A. P. Philosophical Magazine B, Vol. 75, Issue 5 https://doi.org/10.1080/13642819708202343	journal	May 1997
High-resolution photoemission study of UNi2Al3 and URu2Si2 Yang, S. -H.; Kumigashira, H.; Yokoya, T. Journal of Electron Spectroscopy and Related Phenomena, Vol. 78 https://doi.org/10.1016/S0368-2048(96)80047-8	journal	May 1996
Hastatic order in ${URu}_{2} {Si}_{2}$ : Hybridization with a twist Chandra, Premala; Coleman, Piers; Flint, Rebecca Physical Review B, Vol. 91, Issue 20 https://doi.org/10.1103/PhysRevB.91.205103	journal	May 2015
Fermi-surface instability at the ‘hidden-order’ transition of URu2Si2 Santander-Syro, Andrés F.; Klein, Markus; Boariu, Florin L. Nature Physics, Vol. 5, Issue 9 https://doi.org/10.1038/nphys1361	journal	July 2009
Anderson lattice behavior in ${Yb}_{1 - x} {Lu}_{x} {Al}_{3}$ Bauer, E. D.; Booth, C. H.; Lawrence, J. M. Physical Review B, Vol. 69, Issue 12 https://doi.org/10.1103/PhysRevB.69.125102	journal	March 2004
Electronic structure theory of the hidden-order material ${URu}_{2} {Si}_{2}$ Oppeneer, P. M.; Rusz, J.; Elgazzar, S. Physical Review B, Vol. 82, Issue 20 https://doi.org/10.1103/PhysRevB.82.205103	journal	November 2010
Investigation of Aquo and Chloro Complexes of UO ₂ ²⁺ , NpO ₂ ⁺ , Np ⁴⁺ , and Pu ³⁺ by X-ray Absorption Fine Structure Spectroscopy Allen, P. G.; Bucher, J. J.; Shuh, D. K. Inorganic Chemistry, Vol. 36, Issue 21 https://doi.org/10.1021/ic970502m	journal	October 1997
Long range order and two-fluid behavior in heavy electron materials Shirer, K. R.; Shockley, A. C.; Dioguardi, A. P. Proceedings of the National Academy of Sciences, Vol. 109, Issue 45 https://doi.org/10.1073/pnas.1209609109	journal	September 2012
Gapped itinerant spin excitations account for missing entropy in the hidden-order state of URu2Si2 Wiebe, C. R.; Janik, J. A.; MacDougall, G. J. Nature Physics, Vol. 3, Issue 2 https://doi.org/10.1038/nphys522	journal	January 2007
Higher Order Speciation Effects on Plutonium L ₃ X-ray Absorption Near Edge Spectra Conradson, Steven D.; Abney, Kent D.; Begg, Bruce D. Inorganic Chemistry, Vol. 43, Issue 1 https://doi.org/10.1021/ic0346477	journal	January 2004
Self-consistent large- $N$ expansion for normal-state properties of dilute magnetic alloys Bickers, N. E.; Cox, D. L.; Wilkins, J. W. Physical Review B, Vol. 36, Issue 4 https://doi.org/10.1103/PhysRevB.36.2036	journal	August 1987
Why the Hidden Order in URu ₂ Si ₂ Is Still Hidden–One Simple Answer Harima, Hisatomo; Miyake, Kazumasa; Flouquet, Jacques Journal of the Physical Society of Japan, Vol. 79, Issue 3 https://doi.org/10.1143/JPSJ.79.033705	journal	March 2010
A charge density wave in the hidden order state of URu ₂ Si ₂ Su, Jung-Jung; Dubi, Yonatan; Wölfle, Peter Journal of Physics: Condensed Matter, Vol. 23, Issue 9 https://doi.org/10.1088/0953-8984/23/9/094214	journal	February 2011
Variation of f -electron localization in diluted US and UTe Schoenes, J.; Vogt, O.; Löhle, J. Physical Review B, Vol. 53, Issue 22 https://doi.org/10.1103/PhysRevB.53.14987	journal	June 1996
The dual nature of 5f electrons and the origin of heavy fermions in U compounds Zwicknagl, G.; Fulde, P. Journal of Physics: Condensed Matter, Vol. 15, Issue 28 https://doi.org/10.1088/0953-8984/15/28/302	journal	July 2003
Induced-Moment Weak Antiferromagnetism and Orbital Order on the Itinerant-Localized Duality Model with Nested Fermi Surface : A Possible Origin of Exotic Magnetism in URu ₂ Si ₂ Okuno, Yukihiro; Miyake, Kazumasa Journal of the Physical Society of Japan, Vol. 67, Issue 7 https://doi.org/10.1143/JPSJ.67.2469	journal	July 1998
Arrested Kondo effect and hidden order in URu2Si2 Haule, Kristjan; Kotliar, Gabriel Nature Physics, Vol. 5, Issue 11 https://doi.org/10.1038/nphys1392	journal	September 2009
Intermediate-Valence Tautomerism in Decamethylytterbocene Complexes of Methyl-Substituted Bipyridines Booth, Corwin H.; Kazhdan, Daniel; Werkema, Evan L. Journal of the American Chemical Society, Vol. 132, Issue 49 https://doi.org/10.1021/ja106902s	journal	December 2010
Emergent states in heavy-electron materials Yang, Y. -f.; Pines, D. Proceedings of the National Academy of Sciences, Vol. 109, Issue 45 https://doi.org/10.1073/pnas.1211186109	journal	September 2012
The Kondo Problem to Heavy Fermions Hewson, Alexander Cyril https://doi.org/10.1017/CBO9780511470752	book	January 1993
The two-channel Kondo route to non-Fermi-liquid metals Cox, D. L.; Jarrell, M. Journal of Physics: Condensed Matter, Vol. 8, Issue 48 https://doi.org/10.1088/0953-8984/8/48/012	journal	November 1996
Full correction of the self-absorption in soft-fluorescence extended x-ray-absorption fine structure Tröger, L.; Arvanitis, D.; Baberschke, K. Physical Review B, Vol. 46, Issue 6 https://doi.org/10.1103/PhysRevB.46.3283	journal	August 1992
Band structure and Fermi surface of URu $_{2}$ Si $_{2}$ studied by soft x-ray angle-resolved photoemission spectroscopy Kawasaki, Ikuto; Fujimori, Shin-ichi; Takeda, Yukiharu Physical Review B, Vol. 83, Issue 23 https://doi.org/10.1103/PhysRevB.83.235121	journal	June 2011
Cyclotron Resonance in the Hidden-Order Phase of ${URu}_{2} {Si}_{2}$ Tonegawa, S.; Hashimoto, K.; Ikada, K. Physical Review Letters, Vol. 109, Issue 3 https://doi.org/10.1103/PhysRevLett.109.036401	journal	July 2012
Are heavy-fermion metals Fermi liquids? Steglich, F.; Gegenwart, P.; Helfrich, R. Zeitschrift für Physik B Condensed Matter, Vol. 103, Issue 2 https://doi.org/10.1007/s002570050366	journal	June 1996
Inelastic x-ray scattering by electronic excitations under high pressure Rueff, Jean-Pascal; Shukla, Abhay Reviews of Modern Physics, Vol. 82, Issue 1 https://doi.org/10.1103/RevModPhys.82.847	journal	March 2010
Symmetry and correlations underlying hidden order in ${URu}_{2} {Si}_{2}$ Butch, Nicholas P.; Manley, Michael E.; Jeffries, Jason R. Physical Review B, Vol. 91, Issue 3 https://doi.org/10.1103/PhysRevB.91.035128	journal	January 2015
Degree of $5 f$ electron localization in ${URu}_{2} {Si}_{2}$ : Electron energy-loss spectroscopy and spin-orbit sum rule analysis Jeffries, J. R.; Moore, K. T.; Butch, N. P. Physical Review B, Vol. 82, Issue 3 https://doi.org/10.1103/PhysRevB.82.033103	journal	July 2010
Tetravalency and magnetic phase diagram in the heavy-fermion superconductor ${UPd}_{2}$ ${Al}_{3}$ Grauel, A.; Böhm, A.; Fischer, H. Physical Review B, Vol. 46, Issue 9 https://doi.org/10.1103/PhysRevB.46.5818	journal	September 1992
$f$ - $f$ origin of the insulating state in uranium dioxide: X-ray absorption experiments and first-principles calculations Yu, S. -W.; Tobin, J. G.; Crowhurst, J. C. Physical Review B, Vol. 83, Issue 16 https://doi.org/10.1103/PhysRevB.83.165102	journal	April 2011
A seven-crystal Johann-type hard x-ray spectrometer at the Stanford Synchrotron Radiation Lightsource Sokaras, D.; Weng, T. -C.; Nordlund, D. Review of Scientific Instruments, Vol. 84, Issue 5 https://doi.org/10.1063/1.4803669	journal	May 2013
Chirality density wave of the "hidden order" phase in URu2Si2 Kung, H. - H.; Baumbach, R. E.; Bauer, E. D. Science, Vol. 347, Issue 6228 https://doi.org/10.1126/science.1259729	journal	February 2015
Spin and orbital hybridization at specifically nested Fermi surfaces in URu $_{2}$ Si $_{2}$ Oppeneer, P. M.; Elgazzar, S.; Rusz, J. Physical Review B, Vol. 84, Issue 24 https://doi.org/10.1103/PhysRevB.84.241102	journal	December 2011
Direct observation of lattice symmetry breaking at the hidden-order transition in URu2Si2 Tonegawa, S.; Kasahara, S.; Fukuda, T. Nature Communications, Vol. 5, Issue 1 https://doi.org/10.1038/ncomms5188	journal	June 2014
Hall-effect and resistivity study of the heavy-fermion system ${URu}_{2}$ ${Si}_{2}$ Schoenes, J.; Schönenberger, C.; Franse, J. J. M. Physical Review B, Vol. 35, Issue 10 https://doi.org/10.1103/PhysRevB.35.5375	journal	April 1987
Gapped itinerant spin excitations account for missing entropy in the hidden order state of URu$_2$Si$_2$ Wiebe, C. R.; Janik, J. A.; Macdougall, G. J. arXiv https://doi.org/10.48550/arxiv.0710.0896	text	January 2007
Arrested Kondo effect and hidden order in URu_2Si_2 Haule, Kristjan; Kotliar, Gabriel arXiv https://doi.org/10.48550/arxiv.0907.3889	text	January 2009
Why the hidden order in URu2Si2 is still hidden - one simple answer Harima, Hisatomo; Miyake, Kazumasa; Flouquet, Jacques arXiv https://doi.org/10.48550/arxiv.1001.2369	text	January 2010
Spin and orbital hybridization at specifically nested Fermi surfaces in URu$_2$Si$_2$ Oppeneer, Peter M.; Elgazzar, Saad; Rusz, Jan arXiv https://doi.org/10.48550/arxiv.1110.0981	text	January 2011
Electronic Structure of Heavy Fermion Uranium Compounds Studied by Core-Level Photoelectron Spectroscopy Fujimori, Shin-ichi; Ohkochi, Takuo; Kawasaki, Ikuto arXiv https://doi.org/10.48550/arxiv.1110.6689	text	January 2011
Emergent states in heavy electron materials Yang, Yi-feng; Pines, David arXiv https://doi.org/10.48550/arxiv.1206.1115	text	January 2012
Long range order and two-fluid behavior in heavy electron materials Shirer, K. R.; Shockley, A. C.; Dioguardi, A. P. arXiv https://doi.org/10.48550/arxiv.1206.1879	text	January 2012
Multiconfigurational nature of 5f orbitals in uranium and plutonium intermetallics Booth, C. H.; Jiang, Yu; Wang, D. L. arXiv https://doi.org/10.48550/arxiv.1208.2234	text	January 2012
Hidden Order Behaviour in URu2Si2 (A Critical Review of the Status of Hidden Order in 2014) Mydosh, John A.; Oppeneer, Peter M. arXiv https://doi.org/10.48550/arxiv.1405.1625	text	January 2014
Direct observation of lattice symmetry breaking at the hidden-order transition in URu2Si2 Tonegawa, S.; Kasahara, S.; Fukuda, T. arXiv https://doi.org/10.48550/arxiv.1406.5040	text	January 2014
Chirality density wave of the 'hidden order' phase in URu$_2$Si$_2$ Kung, H. -H.; Baumbach, R. E.; Bauer, E. D. arXiv https://doi.org/10.48550/arxiv.1410.6398	text	January 2014
The dual nature of 5f electrons and origin of heavy fermions in U compounds Zwicknagl, G.; Fulde, P. arXiv https://doi.org/10.48550/arxiv.cond-mat/0211706	text	January 2002
Induced-Moment Weak Antiferromagnetism and Orbital Order on the Itinerant-Localized Duality Model with Nested Fermi Surface: A Possible Origin of Exotic Magnetism in URu${}_{2}$Si$_{2}$ Okuno, Yukihiro; Miyake, Kazumasa arXiv https://doi.org/10.48550/arxiv.cond-mat/9804127	text	January 1998

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