Successive field-induced transitions in BiFeO3 around room temperature

Kawachi, Shiro; Miyake, Atsushi; Ito, Toshimitsu; Dissanayake, Sachith E.; Matsuda, Masaaki; Ratcliff, William; Xu, Zhijun; Zhao, Yang; Miyahara, Shin; Furukawa, Nobuo; Tokunaga, Masashi

doi:10.1103/PhysRevMaterials.1.024408

Successive field-induced transitions in ${BiFeO}_{3}$ around room temperature

Journal Article · Fri Jul 21 00:00:00 EDT 2017 · Physical Review Materials

DOI:https://doi.org/10.1103/PhysRevMaterials.1.024408· OSTI ID:1376426

Kawachi, Shiro ^[1]; Miyake, Atsushi ^[1]; Ito, Toshimitsu ^[2]; Dissanayake, Sachith E. ^[3]; Matsuda, Masaaki ^[3]; Ratcliff, William ^[4]; Xu, Zhijun ^[5]; Zhao, Yang ^[5]; Miyahara, Shin ^[6]; Furukawa, Nobuo ^[7]; Tokunaga, Masashi ^[1]

Univ. of Tokyo, Kashiwa (Japan). The Inst. for Solid State Physics (ISSP)
National Inst. of Advanced Industrial Science and Technology (AIST), Tsukuba (Japan)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Quantum Condensed Matter Division
National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States). NIST Center for Neutron Research
National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States). NIST Center for Neutron Research; Univ. of Maryland, College Park, MD (United States). Dept. of Materials Science and Engineering
Fukuoka Univ. (Japan). Dept. of Applied Physics
Aoyama Gakuin Univ., Sagamihara (Japan). Dept. of Physics and Mathematics

The effects of high magnetic fields applied perpendicular to the spontaneous ferroelectric polarization on single crystals of BiFeO₃ were investigated in this paper through magnetization, magnetostriction, and neutron diffraction measurements. The magnetostriction measurements revealed lattice distortion of 2 x 10^-5 during the reorientation process of the cycloidal spin order by applied magnetic fields. Furthermore, anomalous changes in magnetostriction and electric polarization at a larger field demonstrate an intermediate phase between cycloidal and canted antiferromagnetic states, where a large magnetoelectric effect was observed. Neutron diffraction measurements clarified that incommensurate spin modulation along the [110]_hex direction in the cycloidal phase becomes Q = 0 commensurate along this direction in the intermediate phase. Finally, theoretical calculations based on the standard spin Hamiltonian of this material suggest an antiferromagnetic cone-type spin order in the intermediate phase.

View Accepted Manuscript (DOE)

Research Organization:: National Inst. of Advanced Industrial Science and Technology (AIST), Tsukuba (Japan); National Inst. of Standards and Technology (NIST), Gaithersburg, MD (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tokyo, Kashiwa (Japan)

Sponsoring Organization:: Dept. of Commerce (United States); Japan Society for the Promotion of Science (JSPS) (Japan); Murata Science Foundation (Japan); USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Contributing Organization:: Aoyama Gakuin Univ., Sagamihara (Japan); Fukuoka Univ. (Japan); Univ. of Maryland, College Park, MD (United States)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1376426

Alternate ID(s):: OSTI ID: 1372421

Journal Information:: Physical Review Materials, Journal Name: Physical Review Materials Journal Issue: 2 Vol. 1; ISSN 2475-9953

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited By (3)

The structural origin of composition-driven magnetic transformation in BiFeO ₃ -based multiferroics: a neutron diffraction study Khomchenko, V. A.; Karpinsky, D. V.; Latushka, S. I. Journal of Materials Chemistry C, Vol. 7, Issue 20 https://doi.org/10.1039/c9tc01521c	journal	January 2019
Multiferroic behavior from synergetic response of multiple ordering parameters in BiFeO ₃ single crystal under high magnetic field up to 50 Tesla Huang, Sha; Hong, Fang; Xia, Zhengcai Journal of Applied Physics, Vol. 127, Issue 4 https://doi.org/10.1063/1.5131411	journal	January 2020
Direct coupling of ferromagnetic moment and ferroelectric polarization in BiFeO 3 Kawachi, Shiro; Miyahara, Shin; Ito, Toshimitsu Physical Review B, Vol. 100, Issue 14 https://doi.org/10.1103/physrevb.100.140412	journal	October 2019

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