Negative thermal expansion in functional materials: controllable thermal expansion by chemical modifications

Chen, Jun; Hu, Lei; Deng, Jinxia; Xing, Xianran

doi:10.1039/c4cs00461b

Title: Negative thermal expansion in functional materials: controllable thermal expansion by chemical modifications

Journal Article · Mon Apr 13 00:00:00 EDT 2015 · Chemical Society Reviews

DOI:https://doi.org/10.1039/c4cs00461b· OSTI ID:1353243

Chen, Jun ^[1]; Hu, Lei ^[1]; Deng, Jinxia ^[1]; Xing, Xianran ^[1]

Univ. of Science and Technology Beijing (China)

Negative thermal expansion (NTE) is an intriguing physical property of solids, which is a consequence of a complex interplay among the lattice, phonons, and electrons. Interestingly, a large number of NTE materials have been found in various types of functional materials. In the last two decades good progress has been achieved to discover new phenomena and mechanisms of NTE. In the present review article, NTE is reviewed in functional materials of ferroelectrics, magnetics, multiferroics, superconductors, temperature-induced electron configuration change and so forth. Zero thermal expansion (ZTE) of functional materials is emphasized due to the importance for practical applications. The NTE functional materials present a general physical picture to reveal a strong coupling role between physical properties and NTE. There is a general nature of NTE for both ferroelectrics and magnetics, in which NTE is determined by either ferroelectric order or magnetic one. In NTE functional materials, a multi-way to control thermal expansion can be established through the coupling roles of ferroelectricity-NTE, magnetism-NTE, change of electron configuration-NTE, open-framework-NTE, and so on. Chemical modification has been proved to be an effective method to control thermal expansion. Finally, challenges and questions are discussed for the development of NTE materials. There remains a challenge to discover a “perfect” NTE material for each specific application for chemists. The future studies on NTE functional materials will definitely promote the development of NTE materials.

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Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States). Advanced Photon Source (APS)

Sponsoring Organization:: National Natural Science Foundation of China (NSFC); Fundamental Research Funds for the Central Universities

Grant/Contract Number:: 21322102; 91422301; 21231001

OSTI ID:: 1353243

Journal Information:: Chemical Society Reviews, Vol. 44, Issue 11; ISSN 0306-0012

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: ENGLISH

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Cited by: 462 works

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