Stable low-bandgap Pb-Sn binary perovskites for tandem solar cells

Yang, Zhibin; Rajagopal, Adharsh; Chueh, Chu -Chen; Jo, Sae Byeok; Liu, Bo; Zhao, Ting; Jen, Alex K. -Y.

doi:10.1002/adma.201602696

Title: Stable low-bandgap Pb-Sn binary perovskites for tandem solar cells

Journal Article · Mon Aug 22 00:00:00 EDT 2016 · Advanced Materials

DOI:https://doi.org/10.1002/adma.201602696· OSTI ID:1343608

Yang, Zhibin ^[1]; Rajagopal, Adharsh ^[1]; Chueh, Chu -Chen ^[1]; Jo, Sae Byeok ^[1]; Liu, Bo ^[1]; Zhao, Ting ^[1]; Jen, Alex K. -Y. ^[1]

Univ. of Washington, Seattle, WA (United States)

A low-bandgap (1.33 eV) Sn-based MA_0.5FA_0.5Pb_0.75Sn_0.25I₃ perovskite is developed via combined compositional, process, and interfacial engineering. It can deliver a high power conversion efficiency (PCE) of 14.19%. Lastly, a four-terminal all-perovskite tandem solar cell is demonstrated by combining this low-bandgap cell with a semitransparent MAPbI₃ cell to achieve a high efficiency of 19.08%.

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Research Organization:: Univ. of Washington, Seattle, WA (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE)

Contributing Organization:: This work was supported by the Office of Naval Research (N00014-14-1-0246), the Asian Office of Aerospace R&D (FA2386-15-1-4106), and the Department of Energy SunShot (DE-EE0006710). A.K.-Y.J. thanks the Boeing-Johnson Foundation for financial support. Z.Y. thanks the financial support from Washington Research Foundation Innovation Fellowship. Part of this work was conducted at UW NNCI Washington Nanofabrication Facility and Molecular Analysis Facility (Supported in part by the National Science Foundation, Grant No. ECC-1542101) at University of Washington. The authors thank the material synthesis from Francis Lin. The authors also thank Chun-Chih Huang for the steady state PL measurement.

Grant/Contract Number:: EE0006710

OSTI ID:: 1343608

Report Number(s):: DOE-UW-Jen-33

Journal Information:: Advanced Materials, Vol. 28, Issue 40; ISSN 0935-9648

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 271 works

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Low‐Bandgap Mixed Tin‐Lead Perovskites and Their Applications in All‐Perovskite Tandem Solar Cells Wang, Changlei; Song, Zhaoning; Li, Chongwen Advanced Functional Materials, Vol. 29, Issue 47 https://doi.org/10.1002/adfm.201808801	journal	February 2019
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Polyelemental, Multicomponent Perovskite Semiconductor Libraries through Combinatorial Screening Saliba, Michael nanoGe Fall Meeting 2019, Proceedings of the nanoGe Fall Meeting19 https://doi.org/10.29363/nanoge.nfm.2019.264	conference	November 2021
Perovskite solar cells: must lead be replaced – and can it be done? Zhang, Qi; Hao, Feng; Li, Jianbao Science and Technology of Advanced Materials, Vol. 19, Issue 1 https://doi.org/10.1080/14686996.2018.1460176	journal	May 2018

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