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Fullerene-fullerene collisions: Fragmentation and electron capture

Journal Article · · Physical Review A
; ;  [1]; ; ;  [2];  [3]
  1. Institute of Physics and Astronomy, University of Aarhus, DK-8000 Aarhus C (Denmark)
  2. Stockholm University, S-104 05 Stockholm (Sweden)
  3. SRI International, Menlo Park, California 94025 (United States)
In this paper, we describe collisions between high-energy (100-keV) fullerene ions (C{sub 60}{sup +}, C{sub 60}{sup 2+}, C{sub 70}{sup 2+}, and C{sub 70}{sup 3+}) and C{sub 60}. The fast, forward-directed charged collision products are identified, leading to information on electron capture and loss as well as fragmentation. Similar studies are performed on rare-gas targets (He and Xe), and the fragmentation patterns and charge-exchange cross sections are compared and discussed. The electron-capture cross sections are two orders of magnitude larger for collisions with C{sub 60} as compared to Xe, while the smaller cluster-ion fragment peaks are only 3--6 times more intense. These observations are discussed in the light of the low ionization energy and the large mass and size of C{sub 60}.
OSTI ID:
132904
Journal Information:
Physical Review A, Journal Name: Physical Review A Journal Issue: 5 Vol. 52; ISSN 1050-2947; ISSN PLRAAN
Country of Publication:
United States
Language:
English

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