Resonantly enhanced second-harmonic generation using III–V semiconductor all-dielectric metasurfaces

Liu, Sheng; Sinclair, Michael B.; Saravi, Sina; Keeler, Gordon A.; Yang, Yuanmu; Reno, John; Peake, Gregory M.; Setzpfandt, Frank; Staude, Isabelle; Pertsch, Thomas; Brener, Igal

doi:10.1021/acs.nanolett.6b01816

Resonantly enhanced second-harmonic generation using III–V semiconductor all-dielectric metasurfaces

Journal Article · Mon Aug 08 00:00:00 EDT 2016 · Nano Letters

DOI:https://doi.org/10.1021/acs.nanolett.6b01816· OSTI ID:1326369

Liu, Sheng ^[1]; Sinclair, Michael B. ^[1]; Saravi, Sina ^[2]; Keeler, Gordon A. ^[1]; Yang, Yuanmu ^[1]; Reno, John ^[1]; Peake, Gregory M. ^[1]; Setzpfandt, Frank ^[2]; Staude, Isabelle ^[2]; Pertsch, Thomas ^[2]; Brener, Igal ^[1]

Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
Friedrich-Schiller-Univ. Jena, Jena (Germany)

Nonlinear optical phenomena in nanostructured materials have been challenging our perceptions of nonlinear optical processes that have been explored since the invention of lasers. For example, the ability to control optical field confinement, enhancement, and scattering almost independently allows nonlinear frequency conversion efficiencies to be enhanced by many orders of magnitude compared to bulk materials. Also, the subwavelength length scale renders phase matching issues irrelevant. Compared with plasmonic nanostructures, dielectric resonator metamaterials show great promise for enhanced nonlinear optical processes due to their larger mode volumes. Here, we present, for the first time, resonantly enhanced second-harmonic generation (SHG) using gallium arsenide (GaAs) based dielectric metasurfaces. Using arrays of cylindrical resonators we observe SHG enhancement factors as large as 10⁴ relative to unpatterned GaAs. At the magnetic dipole resonance, we measure an absolute nonlinear conversion efficiency of ~2 × 10^–5 with ~3.4 GW/cm² pump intensity. In conclusion, the polarization properties of the SHG reveal that both bulk and surface nonlinearities play important roles in the observed nonlinear process.

View Accepted Manuscript (DOE)

Research Organization:: Sandia National Laboratories (SNL-NM), Albuquerque, NM (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC04-94AL85000

OSTI ID:: 1326369

Report Number(s):: SAND--2016-9155J; 647439

Journal Information:: Nano Letters, Journal Name: Nano Letters Journal Issue: 9 Vol. 16; ISSN 1530-6984

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Inverse-designed photonic fibers and metasurfaces for nonlinear frequency conversion [Invited] Sitawarin, Chawin; Jin, Weiliang; Lin, Zin Photonics Research, Vol. 6, Issue 5 https://doi.org/10.1364/prj.6.000b82	journal	January 2018
A review of dielectric optical metasurfaces for wavefront control Kamali, Seyedeh Mahsa; Arbabi, Ehsan; Arbabi, Amir Nanophotonics, Vol. 7, Issue 6 https://doi.org/10.1515/nanoph-2017-0129	journal	June 2018
Lattice effect influence on the electric and magnetic dipole resonance overlap in a disk array Babicheva, Viktoriia E.; Moloney, Jerome V. Nanophotonics, Vol. 7, Issue 10 https://doi.org/10.1515/nanoph-2018-0107	journal	September 2018
Thermal tuning capabilities of semiconductor metasurface resonators Lewi, Tomer; Butakov, Nikita A.; Schuller, Jon A. Nanophotonics, Vol. 8, Issue 2 https://doi.org/10.1515/nanoph-2018-0178	journal	November 2018
Highly-efficient longitudinal second-harmonic generation from doubly-resonant AlGaAs nanoantennas Xu, Lei; Rahmani, Mohsen; Smirnova, Daria https://doi.org/10.20944/preprints201808.0414.v1	preprint	August 2018
All-Dielectric Nanoresonators for χ(2) Nonlinear Optics Gigli, Carlo; Marino, Giuseppe; Borne, Adrien Frontiers in Physics, Vol. 7 https://doi.org/10.3389/fphy.2019.00221	journal	December 2019
Boosting Second Harmonic Radiation from AlGaAs Nanoantennas with Epsilon-Near-Zero Materials Rocco, Davide; Vincenti, Maria; De Angelis, Costantino Applied Sciences, Vol. 8, Issue 11 https://doi.org/10.3390/app8112212	journal	November 2018
Second-Harmonic Generation in Mie-Resonant GaAs Nanowires de Ceglia, Domenico; Carletti, Luca; Vincenti, Maria Antonietta Applied Sciences, Vol. 9, Issue 16 https://doi.org/10.3390/app9163381	journal	August 2019
Fano Resonance on Nanostructured Lithium Niobate for Highly Efficient and Tunable Second Harmonic Generation Huang, Zhijin; Lu, Huihui; Xiong, Hanqing Nanomaterials, Vol. 9, Issue 1 https://doi.org/10.3390/nano9010069	journal	January 2019
Highly-Efficient Longitudinal Second-Harmonic Generation from Doubly-Resonant AlGaAs Nanoantennas Xu, Lei; Rahmani, Mohsen; Smirnova, Daria Photonics, Vol. 5, Issue 3 https://doi.org/10.3390/photonics5030029	journal	September 2018
Enhanced Nonlinear Yield from Barium Titanate Metasurface Down to the Near Ultraviolet Timpu, Flavia; Reig Escalé, Marc; Timofeeva, Maria ETH Zurich https://doi.org/10.3929/ethz-b-000366859	text	January 2019
All-dielectric nanophotonics: the quest for better materials and fabrication techniques Baranov, Denis G.; Zuev, Dmitry A.; Lepeshov, Sergey I. arXiv https://doi.org/10.48550/arxiv.1702.00677	preprint	January 2017
Gradient metasurfaces: a review of fundamentals and applications Ding, Fei; Pors, Anders; Bozhevolnyi, Sergey I. arXiv https://doi.org/10.48550/arxiv.1704.03032	text	January 2017
Thermal tuning capabilities of semiconductor metasurface resonators Lewi, Tomer; Butakov, Nikita A.; Schuller, Jon A. arXiv https://doi.org/10.48550/arxiv.1802.09664	preprint	January 2018
Giant nonlinear response at the nanoscale driven by bound states in the continuum Carletti, Luca; Koshelev, Kirill; De Angelis, Costantino arXiv https://doi.org/10.48550/arxiv.1804.02947	text	January 2018
Reconfiguring structured light beams using nonlinear metasurfaces Xu, Yun; Sun, Jingbo; Frantz, Jesse arXiv https://doi.org/10.48550/arxiv.1805.07327	text	January 2018
All-dielectric metasurfaces with trapped modes: group-theoretical description Yu, Pengchao; Kupriianov, Anton S.; Dmitriev, Victor arXiv https://doi.org/10.48550/arxiv.1812.10817	text	January 2018
Coherent Control of the Non-instantaneous Nonlinear Power-law Response in Resonant Nanostructures Bahar, Eyal; Arieli, Uri; Mrejen, Michael arXiv https://doi.org/10.48550/arxiv.1909.06126	text	January 2019

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