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Title: Nonlinear Wavefront Control with All-Dielectric Metasurfaces

Journal Article · · Nano Letters

Metasurfaces, two-dimensional lattices of nanoscale resonators, offer unique opportunities for functional flat optics and allow the control of the transmission, reflection, and polarization of a wavefront of light. Recently, all-dielectric metasurfaces reached remarkable efficiencies, often matching or out-performing conventional optical elements. The exploitation of the nonlinear optical response of metasurfaces offers a paradigm shift in nonlinear optics, and dielectric nonlinear metasurfaces are expected to enrich subwavelength photonics by enhancing substantially nonlinear response of natural materials combined with the efficient control of the phase of nonlinear waves. Here, we suggest a novel and rather general approach for engineering the wavefront of parametric waves of arbitrary complexity generated by a nonlinear metasurface. We design all-dielectric nonlinear metasurfaces, achieve a highly efficient wavefront control of a third-harmonic field, and demonstrate the generation of nonlinear beams at a designed angle and the generation of nonlinear focusing vortex beams. Lastly, our nonlinear metasurfaces produce phase gradients over a full 0–2π phase range with a 92% diffraction efficiency.

Research Organization:
Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES)
Grant/Contract Number:
AC05-00OR22725
OSTI ID:
1456796
Journal Information:
Nano Letters, Vol. 18, Issue 6; ISSN 1530-6984
Publisher:
American Chemical SocietyCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 132 works
Citation information provided by
Web of Science

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Cited By (27)

Corrugated silicon metasurface optimized within the Rayleigh hypothesis for anomalous refraction at large angles journal January 2019
Recent Progress in Active Optical Metasurfaces journal April 2019
Resonant dielectric metasurfaces: active tuning and nonlinear effects journal July 2019
Controlling second-harmonic diffraction by nano-patterning MoS 2 monolayers journal January 2019
Twofold Polarization‐Selective All‐Dielectric Trifoci Metalens for Linearly Polarized Visible Light journal July 2019
CMOS-compatible all-Si metasurface polarizing bandpass filters on 12-inch wafers journal January 2019
Exact Multipolar Decompositions with Applications in Nanophotonics journal December 2018
All-dielectric metamirror for independent and asymmetric wave-front control journal November 2019
Third‐Harmonic Generation from Plasmonic Metasurfaces Coupled to Intersubband Transitions journal February 2019
Tailored Nonlinear Anisotropy in Mie‐Resonant Dielectric Oligomers journal July 2019
A Dynamically Modulated All‐Dielectric Metasurface Doublet for Directional Harmonic Generation and Manipulation in Transmission journal September 2019
Ultrafast optical pulse shaping using dielectric metasurfaces journal May 2019
Nonlinear wavefront shaping with optically induced three-dimensional nonlinear photonic crystals journal July 2019
High conversion efficiency second-harmonic beam shaping via amplitude-type nonlinear photonic crystals journal December 2019
Interaction of semiconductor metasurfaces with short laser pulses: From nonlinear-optical response toward spatiotemporal shaping journal August 2019
Polarization- and diffraction-controlled second-harmonic generation from semiconductor metasurfaces journal January 2019
Self-assembly of nanostructured glass metasurfaces via templated fluid instabilities journal February 2019
Nonlinear optics in all-dielectric nanoantennas and metasurfaces: a review journal March 2019
Photosensitive chalcogenide metasurfaces supporting bound states in the continuum journal January 2019
Broadband visible-near infrared and deep ultraviolet generation by four-wave mixing and high-order stimulated Raman scattering from the hybrid metasurfaces of plasmonic nanoantennae and Raman-active nanoparticles journal January 2019
When metasurface meets hologram: principle and advances journal January 2019
Resonance-enhanced three-photon luminesce via lead halide perovskite metasurfaces for optical encoding journal May 2019
Interference-enhanced optical magnetism in surface high-index resonators: a pathway toward high-performance ultracompact linear and nonlinear meta-optics journal January 2019
Third-Harmonic Generation in Photonic Topological Metasurfaces journal September 2019
Corrugated silicon metasurface optimized within the Rayleigh hypothesis for anomalous refraction at large angles text January 2019
Photosensitive chalcogenide metasurfaces supporting bound states in the continuum text January 2019
Silicon metasurfaces for third harmonic geometric phase manipulation and multiplexed holography text January 2019

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