Synthesis of Two-Dimensional Materials for Capacitive Energy Storage

Mendoza-Sánchez, Beatriz; Gogotsi, Yury

doi:10.1002/adma.201506133

Synthesis of Two-Dimensional Materials for Capacitive Energy Storage

Journal Article · Thu Jun 02 00:00:00 EDT 2016 · Advanced Materials

DOI:https://doi.org/10.1002/adma.201506133· OSTI ID:1286986

Mendoza-Sánchez, Beatriz ^[1]; Gogotsi, Yury ^[2]

FranÃ§ois Rabelais Univ., Tours (France)
Drexel Univ., Philadelphia, PA (United States)

The unique properties and great variety of two-dimensional (2D) nanomaterials make them highly attractive for energy storage applications. Here, an insight into the progress made towards the application of 2D nanomaterials for capacitive energy storage is provided. Moreover, synthesis methods, and electrochemical performance of various classes of 2D nanomaterials, particularly based on graphene, transition metal oxides, dichalcogenides, and carbides, are presented. Some factors that directly influence capacitive performance are discussed throughout the text and include nanosheet composition, morphology and texture, electrode architecture, and device configuration. Recent progress in the fabrication of 2D-nanomaterials-based microsupercapacitors and flexible and free-standing supercapacitors is presented. The main electrode manufacturing techniques with emphasis on scalability and cost-effectiveness are discussed, and include laser scribing, printing, and roll-to-roll manufacture. Some various issues that prevent the use of the full energy-storage potential of 2D nanomaterials and how they have been tackled are discussed, and include nanosheet aggregation and the low electrical conductivity of some 2D nanomaterials. In particular, the design of hybrid and hierarchical 2D and 3D structures based on 2D nanomaterials is presented. Other challenges and opportunities are discussed and include: control of nanosheets size and thickness, chemical and electrochemical instability, and scale-up of electrode films.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1286986

Alternate ID(s):: OSTI ID: 1371399
OSTI ID: 1387684

Journal Information:: Advanced Materials, Journal Name: Advanced Materials Journal Issue: 29 Vol. 28; ISSN 0935-9648

Publisher:: WileyCopyright Statement

Country of Publication:: United States

Language:: English

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The Synthesis of NiCo2O4–MnO2 Core–Shell Nanowires by Electrodeposition and Its Supercapacitive Properties Yan, Ai-Lan; Wang, Wei-Dong; Chen, Wen-Qiang Nanomaterials, Vol. 9, Issue 10 https://doi.org/10.3390/nano9101398	journal	October 2019

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Flexible MXene/Graphene Films for Ultrafast Supercapacitors with Outstanding Volumetric Capacitance

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