Synthesis of Two-Dimensional Materials for Capacitive Energy Storage
Abstract
The unique properties and great variety of two-dimensional (2D) nanomaterials make them highly attractive for energy storage applications. Here, an insight into the progress made towards the application of 2D nanomaterials for capacitive energy storage is provided. Moreover, synthesis methods, and electrochemical performance of various classes of 2D nanomaterials, particularly based on graphene, transition metal oxides, dichalcogenides, and carbides, are presented. Some factors that directly influence capacitive performance are discussed throughout the text and include nanosheet composition, morphology and texture, electrode architecture, and device configuration. Recent progress in the fabrication of 2D-nanomaterials-based microsupercapacitors and flexible and free-standing supercapacitors is presented. The main electrode manufacturing techniques with emphasis on scalability and cost-effectiveness are discussed, and include laser scribing, printing, and roll-to-roll manufacture. Some various issues that prevent the use of the full energy-storage potential of 2D nanomaterials and how they have been tackled are discussed, and include nanosheet aggregation and the low electrical conductivity of some 2D nanomaterials. In particular, the design of hybrid and hierarchical 2D and 3D structures based on 2D nanomaterials is presented. Other challenges and opportunities are discussed and include: control of nanosheets size and thickness, chemical and electrochemical instability, and scale-up of electrode films.
- Authors:
-
- François Rabelais Univ., Tours (France)
- Drexel Univ., Philadelphia, PA (United States)
- Publication Date:
- Research Org.:
- Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
- Sponsoring Org.:
- USDOE Office of Science (SC), Basic Energy Sciences (BES)
- OSTI Identifier:
- 1286986
- Grant/Contract Number:
- AC05-00OR22725
- Resource Type:
- Journal Article: Accepted Manuscript
- Journal Name:
- Advanced Materials
- Additional Journal Information:
- Journal Volume: 28; Journal Issue: 29; Journal ID: ISSN 0935-9648
- Publisher:
- Wiley
- Country of Publication:
- United States
- Language:
- English
- Subject:
- 25 ENERGY STORAGE; 2D materials; electrode architecture; hierarchical structure; hybrid devices; supercapacitors
Citation Formats
Mendoza-Sánchez, Beatriz, and Gogotsi, Yury. Synthesis of Two-Dimensional Materials for Capacitive Energy Storage. United States: N. p., 2016.
Web. doi:10.1002/adma.201506133.
Mendoza-Sánchez, Beatriz, & Gogotsi, Yury. Synthesis of Two-Dimensional Materials for Capacitive Energy Storage. United States. https://doi.org/10.1002/adma.201506133
Mendoza-Sánchez, Beatriz, and Gogotsi, Yury. 2016.
"Synthesis of Two-Dimensional Materials for Capacitive Energy Storage". United States. https://doi.org/10.1002/adma.201506133. https://www.osti.gov/servlets/purl/1286986.
@article{osti_1286986,
title = {Synthesis of Two-Dimensional Materials for Capacitive Energy Storage},
author = {Mendoza-Sánchez, Beatriz and Gogotsi, Yury},
abstractNote = {The unique properties and great variety of two-dimensional (2D) nanomaterials make them highly attractive for energy storage applications. Here, an insight into the progress made towards the application of 2D nanomaterials for capacitive energy storage is provided. Moreover, synthesis methods, and electrochemical performance of various classes of 2D nanomaterials, particularly based on graphene, transition metal oxides, dichalcogenides, and carbides, are presented. Some factors that directly influence capacitive performance are discussed throughout the text and include nanosheet composition, morphology and texture, electrode architecture, and device configuration. Recent progress in the fabrication of 2D-nanomaterials-based microsupercapacitors and flexible and free-standing supercapacitors is presented. The main electrode manufacturing techniques with emphasis on scalability and cost-effectiveness are discussed, and include laser scribing, printing, and roll-to-roll manufacture. Some various issues that prevent the use of the full energy-storage potential of 2D nanomaterials and how they have been tackled are discussed, and include nanosheet aggregation and the low electrical conductivity of some 2D nanomaterials. In particular, the design of hybrid and hierarchical 2D and 3D structures based on 2D nanomaterials is presented. Other challenges and opportunities are discussed and include: control of nanosheets size and thickness, chemical and electrochemical instability, and scale-up of electrode films.},
doi = {10.1002/adma.201506133},
url = {https://www.osti.gov/biblio/1286986},
journal = {Advanced Materials},
issn = {0935-9648},
number = 29,
volume = 28,
place = {United States},
year = {Thu Jun 02 00:00:00 EDT 2016},
month = {Thu Jun 02 00:00:00 EDT 2016}
}
Web of Science
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Supercapacitor electrode materials with hierarchically structured pores from carbonization of MWCNTs and ZIF-8 composites
journal, January 2017
- Li, Xueqin; Hao, Changlong; Tang, Bochong
- Nanoscale, Vol. 9, Issue 6
Highly negative Poisson's ratio in a flexible two-dimensional tungsten carbide monolayer
journal, January 2018
- Wu, Donghai; Wang, Shuaiwei; Zhang, Shouren
- Physical Chemistry Chemical Physics, Vol. 20, Issue 28
Rationally designing S/Ti 3 C 2 T x as a cathode material with an interlayer for high-rate and long-cycle lithium–sulfur batteries
journal, January 2018
- Jin, Q.; Zhang, N.; Zhu, C. C.
- Nanoscale, Vol. 10, Issue 35
Heteroatom-doped porous carbons derived from moxa floss of different storage years for supercapacitors
journal, January 2018
- Zhang, Xuelin; Niu, Qingyuan; Guo, Yaqing
- RSC Advances, Vol. 8, Issue 30
Oxygen-vacancy Bi 2 O 3 nanosheet arrays with excellent rate capability and CoNi 2 S 4 nanoparticles immobilized on N-doped graphene nanotubes as robust electrode materials for high-energy asymmetric supercapacitors
journal, January 2019
- Zhao, Jian; Li, Zhenjiang; Shen, Tong
- Journal of Materials Chemistry A, Vol. 7, Issue 13
B 3 S monolayer: prediction of a high-performance anode material for lithium-ion batteries
journal, January 2019
- Jana, Saibal; Thomas, Siby; Lee, Chi Ho
- Journal of Materials Chemistry A, Vol. 7, Issue 20
A super-thermostable, flexible supercapacitor for ultralight and high performance devices
journal, January 2020
- Kim, Dong Won; Jung, Sung Mi; Jung, Hyun Young
- Journal of Materials Chemistry A, Vol. 8, Issue 2
The development of 2D materials for electrochemical energy applications: A mechanistic approach
journal, March 2019
- Hynek, David J.; Pondick, Joshua V.; Cha, Judy J.
- APL Materials, Vol. 7, Issue 3
Novel mesoporous electrode materials for symmetric, asymmetric and hybrid supercapacitors
journal, March 2019
- Cherusseri, Jayesh; Sambath Kumar, Kowsik; Choudhary, Nitin
- Nanotechnology, Vol. 30, Issue 20
Strategies for improving the lithium-storage performance of 2D nanomaterials
journal, July 2017
- Mei, Jun; Zhang, Yuanwen; Liao, Ting
- National Science Review, Vol. 5, Issue 3
Flocculant-Assisted Synthesis of Graphene-Like Carbon Nanosheets for Oxygen Reduction Reaction and Supercapacitor
journal, August 2019
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- Nanomaterials, Vol. 9, Issue 8
The Synthesis of NiCo2O4–MnO2 Core–Shell Nanowires by Electrodeposition and Its Supercapacitive Properties
journal, October 2019
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- Nanomaterials, Vol. 9, Issue 10
Molecularly Coupled Two‐Dimensional Titanium Oxide and Carbide Sheets for Wearable and High‐Rate Quasi‐Solid‐State Rechargeable Batteries
journal, April 2019
- Wu, Jinli; Jiang, Kun; Li, Guohui
- Advanced Functional Materials, Vol. 29, Issue 30
Recent Development of Printed Micro‐Supercapacitors: Printable Materials, Printing Technologies, and Perspectives
journal, April 2019
- Li, Hongpeng; Liang, Jiajie
- Advanced Materials, Vol. 32, Issue 3
The Road Towards Planar Microbatteries and Micro‐Supercapacitors: From 2D to 3D Device Geometries
journal, June 2019
- Zheng, Shuanghao; Shi, Xiaoyu; Das, Pratteek
- Advanced Materials
Dreidimensionale Architekturen aus Übergangsmetall‐Dichalkogenid‐Nanomaterialien zur elektrochemischen Energiespeicherung und ‐umwandlung
journal, December 2017
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- Angewandte Chemie, Vol. 130, Issue 3
Confined Self-Assembly in Two-Dimensional Interlayer Space: Monolayered Mesoporous Carbon Nanosheets with In-Plane Orderly Arranged Mesopores and a Highly Graphitized Framework
journal, February 2018
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- Angewandte Chemie International Edition, Vol. 57, Issue 11
Ultrathin Two‐Dimensional Semiconductors for Photocatalysis in Energy and Environment Applications
journal, October 2019
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- ChemCatChem, Vol. 11, Issue 24
Tracking Ionic Rearrangements and Interpreting Dynamic Volumetric Changes in Two‐Dimensional Metal Carbide Supercapacitors: A Molecular Dynamics Simulation Study
journal, January 2018
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- ChemSusChem, Vol. 11, Issue 12
Facile synthesis and electrochemical performance of TiO2 nanowires/Ti3C2 composite
journal, January 2018
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- Journal of Materials Science: Materials in Electronics, Vol. 29, Issue 6
Flexible and integrated supercapacitor with tunable energy storage
journal, January 2017
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- Nanoscale, Vol. 9, Issue 34
Sb 2 O 3 /MXene(Ti 3 C 2 T x ) hybrid anode materials with enhanced performance for sodium-ion batteries
journal, January 2017
- Guo, Xin; Xie, Xiuqiang; Choi, Sinho
- Journal of Materials Chemistry A, Vol. 5, Issue 24
An easily manipulated protocol for patterning of MXenes on paper for planar micro-supercapacitors
journal, January 2017
- Hu, Haibo; Hua, Tao
- Journal of Materials Chemistry A, Vol. 5, Issue 37
Edge-oriented SnS 2 nanosheet arrays on carbon paper as advanced binder-free anodes for Li-ion and Na-ion batteries
journal, January 2017
- Wang, Jian-Gan; Sun, Huanhuan; Liu, Huanyan
- Journal of Materials Chemistry A, Vol. 5, Issue 44
A stepwise crosslinking strategy toward lamellar carbon frameworks with covalently connected alternate layers of porous carbon nanosheets and porous carbon spacers
journal, January 2018
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- Chemical Communications, Vol. 54, Issue 73
Electronic Properties of Armchair Black Phosphorene Nanoribbons Edge-Modified by Transition Elements V, Cr, and Mn
journal, April 2019
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- Nanoscale Research Letters, Vol. 14, Issue 1
Optically Sintered 2D RuO 2 Nanosheets: Temperature-Controlled NO 2 Reaction
journal, February 2017
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- Advanced Functional Materials, Vol. 27, Issue 13
Functionalized Hybridization of 2D Nanomaterials
journal, September 2019
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- Advanced Science, Vol. 6, Issue 23
Fluorine-free preparation of titanium carbide MXene quantum dots with high near-infrared photothermal performances for cancer therapy
journal, January 2017
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- Nanoscale, Vol. 9, Issue 45
Photochemical and oxidative cyclisation of tetraphenylpyrroles
journal, January 2017
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- Organic & Biomolecular Chemistry, Vol. 15, Issue 44
Scalable transfer of vertical graphene nanosheets for flexible supercapacitor applications
journal, September 2017
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- Nanotechnology, Vol. 28, Issue 41
Synthesis of Nitrogen-Doped Two-Dimensional Ti 3 C 2 with Enhanced Electrochemical Performance
journal, January 2017
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- Journal of The Electrochemical Society, Vol. 164, Issue 4
Vanadium‐Based Nanomaterials: A Promising Family for Emerging Metal‐Ion Batteries
journal, January 2020
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- Advanced Functional Materials, Vol. 30, Issue 10
Extraordinary Areal and Volumetric Performance of Flexible Solid-State Micro-Supercapacitors Based on Highly Conductive Freestanding Ti 3 C 2 T x Films
journal, June 2018
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- Advanced Electronic Materials, Vol. 4, Issue 8
Emergent Pseudocapacitance of 2D Nanomaterials
journal, February 2018
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- Advanced Energy Materials, Vol. 8, Issue 13
Automated Scalpel Patterning of Solution Processed Thin Films for Fabrication of Transparent MXene Microsupercapacitors
journal, October 2018
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- Small, Vol. 14, Issue 44
Amorphous 2D materials containing a conjugated-polymer network
journal, August 2019
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- Communications Chemistry, Vol. 2, Issue 1
Recent advances in inorganic 2D materials and their applications in lithium and sodium batteries
journal, January 2017
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- Journal of Materials Chemistry A, Vol. 5, Issue 8
Two dimensional oxygen-vacancy-rich Co 3 O 4 nanosheets with excellent supercapacitor performances
journal, January 2017
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- Chemical Communications, Vol. 53, Issue 92
Ultrathin VO 2 nanosheets self-assembled into 3D micro/nano-structured hierarchical porous sponge-like micro-bundles for long-life and high-rate Li-ion batteries
journal, January 2017
- Liu, Pengcheng; Xu, Yuan; Zhu, Kongjun
- Journal of Materials Chemistry A, Vol. 5, Issue 18
Self-assembled two-dimensional copper oxide nanosheet bundles as an efficient oxygen evolution reaction (OER) electrocatalyst for water splitting applications
journal, January 2017
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- Journal of Materials Chemistry A, Vol. 5, Issue 25
Silicon quantum dot-assisted synthesis of MoS 2 /rGO sandwich structures with excellent supercapacitive performance
journal, January 2019
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- New Journal of Chemistry, Vol. 43, Issue 22
Modulation of the electronic properties of pristine and AlP-codoped stanene monolayers by the adsorption of CH 2 O and CH 4 molecules: a DFT study
journal, April 2019
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- Materials Research Express, Vol. 6, Issue 7
2D Black Phosphorus: from Preparation to Applications for Electrochemical Energy Storage
journal, February 2018
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- Advanced Science, Vol. 5, Issue 5
Electronic Properties of Armchair Black Phosphorene Nanoribbons Edge-Modified by Transition Elements V, Cr, and Mn
journal, April 2019
- Huang, Jiong-Hua; Wang, Xue-Feng; Liu, Yu-Shen
- Nanoscale Research Letters, Vol. 14, Issue 1
A Review on Flexible and Transparent Energy Storage System
journal, November 2018
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- Materials, Vol. 11, Issue 11
Flocculant-Assisted Synthesis of Graphene-Like Carbon Nanosheets for Oxygen Reduction Reaction and Supercapacitor
journal, August 2019
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- Nanomaterials, Vol. 9, Issue 8