Nonlinear Fano-Resonant Dielectric Metasurfaces

Yang, Yuanmu; Wang, Wenyi; Boulesbaa, Abdelaziz; Kravchenko, Ivan I.; Briggs, Dayrl P.; Puretzky, Alexander; Geohegan, David; Valentine, Jason

doi:10.1021/acs.nanolett.5b02802

Nonlinear Fano-Resonant Dielectric Metasurfaces

Journal Article · Mon Oct 26 00:00:00 EDT 2015 · Nano Letters

DOI:https://doi.org/10.1021/acs.nanolett.5b02802· OSTI ID:1265873

Yang, Yuanmu ^[1]; Wang, Wenyi ^[1]; Boulesbaa, Abdelaziz ^[2]; Kravchenko, Ivan I. ^[2]; Briggs, Dayrl P. ^[2]; Puretzky, Alexander ^[2]; Geohegan, David ^[2]; Valentine, Jason ^[1]

Vanderbilt Univ., Nashville, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

Strong nonlinear light matter interaction is highly sought-after for a variety of applications including lasing and all-optical light modulation. Recently, resonant plasmonic structures have been considered promising candidates for enhancing nonlinear optical processes due to their ability to greatly enhance the optical near-field; however, their small mode volumes prevent the inherently large nonlinear susceptibility of the metal from being efficiently exploited. We present an alternative approach that utilizes a Fano-resonant silicon metasurface. The metasurface results in strong near-field enhancement within the volume of the silicon resonator while minimizing two photon absorption. Here, we measure a third harmonic generation enhancement factor of 1.5 105 with respect to an unpatterned silicon film and an absolute conversion efficiency of 1.2 10 6 with a peak pump intensity of 3.2 GW cm 2. The enhanced nonlinearity, combined with a sharp linear transmittance spectrum, results in transmission modulation with a modulation depth of 36%. Finally, the modulation mechanism is studied by pump probe experiments

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States). Center for Nanophase Materials Sciences (CNMS)

Sponsoring Organization:: USDOE Office of Science (SC); National Science Foundation (NSF)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1265873

Journal Information:: Nano Letters, Journal Name: Nano Letters Journal Issue: 11 Vol. 15; ISSN 1530-6984

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Overcoming the efficiency-bandwidth tradeoff for optical harmonics generation using nonlinear time-variant resonators Shcherbakov, Maxim R.; Shafirin, Pavel; Shvets, Gennady Physical Review A, Vol. 100, Issue 6 https://doi.org/10.1103/physreva.100.063847	journal	December 2019
Generalized Optical Signal Processing Based on Multioperator Metasurfaces Synthesized by Susceptibility Tensors Momeni, Ali; Rajabalipanah, Hamid; Abdolali, Ali Physical Review Applied, Vol. 11, Issue 6 https://doi.org/10.1103/physrevapplied.11.064042	journal	June 2019
Enhancement and Inhibition of Spontaneous Photon Emission by Resonant Silicon Nanoantennas Bouchet, Dorian; Mivelle, Mathieu; Proust, Julien Physical Review Applied, Vol. 6, Issue 6 https://doi.org/10.1103/physrevapplied.6.064016	journal	December 2016
Momentum Analysis for Metasurfaces Liu, Wenwei; Li, Zhancheng; Cheng, Hua Physical Review Applied, Vol. 8, Issue 1 https://doi.org/10.1103/physrevapplied.8.014012	journal	July 2017
Probing the Combined Electromagnetic Local Density of Optical States with Quantum Emitters Supporting Strong Electric and Magnetic Transitions Li, Dongfang; Karaveli, Sinan; Cueff, Sébastien Physical Review Letters, Vol. 121, Issue 22 https://doi.org/10.1103/physrevlett.121.227403	journal	November 2018
High- Q Quasibound States in the Continuum for Nonlinear Metasurfaces Liu, Zhuojun; Xu, Yi; Lin, Ye Physical Review Letters, Vol. 123, Issue 25 https://doi.org/10.1103/physrevlett.123.253901	journal	December 2019
Nonlinear optics in all-dielectric nanoantennas and metasurfaces: a review Sain, Basudeb; Meier, Cedrik; Zentgraf, Thomas Advanced Photonics, Vol. 1, Issue 02 https://doi.org/10.1117/1.ap.1.2.024002	journal	March 2019
Complex dewetting scenarios of ultrathin silicon films for large-scale nanoarchitectures Naffouti, Meher; Backofen, Rainer; Salvalaglio, Marco Science Advances, Vol. 3, Issue 11 https://doi.org/10.1126/sciadv.aao1472	journal	November 2017
Optically resonant dielectric nanostructures Kuznetsov, Arseniy I.; Miroshnichenko, Andrey E.; Brongersma, Mark L. Science, Vol. 354, Issue 6314 https://doi.org/10.1126/science.aag2472	journal	November 2016
Ultrafast optical pulse shaping using dielectric metasurfaces Divitt, Shawn; Zhu, Wenqi; Zhang, Cheng Science, Vol. 364, Issue 6443 https://doi.org/10.1126/science.aav9632	journal	May 2019
Generalized Optical Signal Processing Based on Multi-Operator Metasurfaces Synthesized by Susceptibility Tensors Momeni, Ali; Rajabalipanah, Hamid; Abdolali, Ali Unpublished https://doi.org/10.13140/rg.2.2.26553.62566	text	January 2018
High Q-factor with the excitation of anapole modes in dielectric split nanodisk arrays Liu, Shao-Ding; Wang, Zhi-Xing; Wang, Wen-Jie Optics Express, Vol. 25, Issue 19 https://doi.org/10.1364/OE.25.022375	journal	January 2017
Near-field probing the magnetic field vector of visible light with a silicon nanoparticle probe and nanopolarimetry Sun, Lin; Bai, Benfeng; Meng, Xiaoxia Optics Express, Vol. 26, Issue 19 https://doi.org/10.1364/OE.26.024637	journal	January 2018
Design and modeling of third-harmonic plasmonic metasurfaces coupled to multi-quantum well structures Zahedi, Taher; Firouzeh, Zaker Hossein; Nezhad, Abolghasem Zeidaabadi Journal of the Optical Society of America B, Vol. 36, Issue 9 https://doi.org/10.1364/josab.36.002429	journal	January 2019
Monolithic AlGaAs second-harmonic nanoantennas Gili, V. F.; Carletti, L.; Locatelli, A. Optics Express, Vol. 24, Issue 14, p. 15965-15971 https://doi.org/10.1364/oe.24.015965	journal	January 2016
Enhanced third harmonic generation in a silicon metasurface using trapped mode Tong, Wenyuan; Gong, Cheng; Liu, Xiaojun Optics Express, Vol. 24, Issue 17 https://doi.org/10.1364/oe.24.019661	journal	January 2016
Anticrossing double Fano resonances generated in metallic/dielectric hybrid nanostructures using nonradiative anapole modes for enhanced nonlinear optical effects Zhai, Wu-Chao; Qiao, Tie-Zhu; Cai, Dong-Jin Optics Express, Vol. 24, Issue 24 https://doi.org/10.1364/oe.24.027858	journal	January 2016
Vectorial control of nonlinear emission via chiral butterfly nanoantennas: generation of pure high order nonlinear vortex beams Lesina, Antonino Cala’; Berini, Pierre; Ramunno, Lora Optics Express, Vol. 25, Issue 3 https://doi.org/10.1364/oe.25.002569	journal	January 2017
Giant enhancement of reflectance due to the interplay between surface confined wave modes and nonlinear gain in dielectric media Kim, Sangbum; Kim, Kihong Optics Express, Vol. 25, Issue 25 https://doi.org/10.1364/oe.25.031816	journal	January 2017
Ultrahigh-quality factor resonant dielectric metasurfaces based on hollow nanocuboids Algorri, J. F.; Zografopoulos, D. C.; Ferraro, A. Optics Express, Vol. 27, Issue 5 https://doi.org/10.1364/oe.27.006320	journal	January 2019
Investigation of terahertz all-dielectric metamaterials He, Xiaoyong; Liu, Feng; Lin, Fangting Optics Express, Vol. 27, Issue 10 https://doi.org/10.1364/oe.27.013831	journal	January 2019
Ultra-thin transmissive crystalline silicon high-contrast grating metasurfaces Li, He; Stellinga, Daan P.; Qiu, Yunmin Optics Express, Vol. 27, Issue 21 https://doi.org/10.1364/oe.27.030931	journal	January 2019
Self-tuning of second-harmonic generation in GaAs nanowires enabled by nonlinear absorption Carletti, L.; de Ceglia, D.; Vincenti, M. A. Optics Express, Vol. 27, Issue 22 https://doi.org/10.1364/oe.27.032480	journal	January 2019
Dual-functional dielectric metasurface doublets Bian, Kai; Lu, Daquan; Hu, Wei Optics Express, Vol. 27, Issue 23 https://doi.org/10.1364/oe.27.034258	journal	January 2019
Polarization properties of second-harmonic generation in AlGaAs optical nanoantennas Ghirardini, L.; Carletti, L.; Gili, V. Optics Letters, Vol. 42, Issue 3 https://doi.org/10.1364/ol.42.000559	journal	January 2017
Fano-resonance-based mode-matching hybrid metasurface for enhanced second-harmonic generation Li, Zhi; Liu, Wenwei; Li, Zhancheng Optics Letters, Vol. 42, Issue 16 https://doi.org/10.1364/ol.42.003117	journal	January 2017
Microscopic study of resonant third-harmonic generation from amorphous silicon nanodisk arrays Deka, Jayanta; Jha, Keshav Kumar; Menon, Sruti Optics Letters, Vol. 43, Issue 21 https://doi.org/10.1364/ol.43.005242	journal	January 2018
Fano-resonant silicon photonic crystal slab for efficient third-harmonic generation Ban, Guoxun; Gong, Cheng; Zhou, Chaobiao Optics Letters, Vol. 44, Issue 1 https://doi.org/10.1364/ol.44.000126	journal	December 2018
Near-infrared modulation by means of GeTe/SOI-based metamaterial Petronijevic, E.; Leahu, G.; Di Meo, V. Optics Letters, Vol. 44, Issue 6 https://doi.org/10.1364/ol.44.001508	journal	January 2019
Analog of electromagnetically induced transparency in an E-shaped all-dielectric metasurface based on toroidal dipolar response Han, Bingxin; Li, Xiangjun; Sui, Chuanshuai Optical Materials Express, Vol. 8, Issue 8 https://doi.org/10.1364/ome.8.002197	journal	January 2018
Multipolar nonlinear nanophotonics Smirnova, Daria; Kivshar, Yuri S. Optica, Vol. 3, Issue 11 https://doi.org/10.1364/optica.3.001241	journal	January 2016
Accelerating light with metasurfaces Henstridge, Meredith; Pfeiffer, Carl; Wang, Di Optica, Vol. 5, Issue 6 https://doi.org/10.1364/optica.5.000678	journal	January 2018
Spontaneous photon-pair generation from a dielectric nanoantenna Marino, Giuseppe; Solntsev, Alexander S.; Xu, Lei Optica, Vol. 6, Issue 11 https://doi.org/10.1364/optica.6.001416	journal	January 2019
Broken symmetry theta-shaped dielectric arrays for a high Q-factor Fano resonance with anapole excitation and magnetic field tunability Wang, Wudeng; Zhao, Xin; Xiong, Li OSA Continuum, Vol. 2, Issue 2 https://doi.org/10.1364/osac.2.000507	journal	January 2019
Resonant four-wave mixing microscopy on silicon-on-insulator based zero-contrast gratings Biswas, Rabindra; Deka, Jayanta; Jha, Keshav kumar OSA Continuum, Vol. 2, Issue 10 https://doi.org/10.1364/osac.2.002864	journal	January 2019
Inverse-designed photonic fibers and metasurfaces for nonlinear frequency conversion [Invited] Sitawarin, Chawin; Jin, Weiliang; Lin, Zin Photonics Research, Vol. 6, Issue 5 https://doi.org/10.1364/prj.6.000b82	journal	January 2018
Interference-enhanced optical magnetism in surface high-index resonators: a pathway toward high-performance ultracompact linear and nonlinear meta-optics Kang, Lei; Bao, Huaguang; Werner, Douglas H. Photonics Research, Vol. 7, Issue 11 https://doi.org/10.1364/prj.7.001296	journal	January 2019
Material platforms for optical metasurfaces Choudhury, Sajid M.; Wang, Di; Chaudhuri, Krishnakali Nanophotonics, Vol. 7, Issue 6 https://doi.org/10.1515/nanoph-2017-0130	journal	June 2018
Thermal tuning capabilities of semiconductor metasurface resonators Lewi, Tomer; Butakov, Nikita A.; Schuller, Jon A. Nanophotonics, Vol. 8, Issue 2 https://doi.org/10.1515/nanoph-2018-0178	journal	November 2018
Plasmon-induced transparency effect for ultracompact on-chip devices Niu, Xinxiang; Hu, Xiaoyong; Yan, Qiuchen Nanophotonics, Vol. 8, Issue 7 https://doi.org/10.1515/nanoph-2019-0093	journal	June 2019
Highly-efficient longitudinal second-harmonic generation from doubly-resonant AlGaAs nanoantennas Xu, Lei; Rahmani, Mohsen; Smirnova, Daria https://doi.org/10.20944/preprints201808.0414.v1	preprint	August 2018
All-Dielectric Nanoresonators for χ(2) Nonlinear Optics Gigli, Carlo; Marino, Giuseppe; Borne, Adrien Frontiers in Physics, Vol. 7 https://doi.org/10.3389/fphy.2019.00221	journal	December 2019
Highly-Efficient Longitudinal Second-Harmonic Generation from Doubly-Resonant AlGaAs Nanoantennas Xu, Lei; Rahmani, Mohsen; Smirnova, Daria Photonics, Vol. 5, Issue 3 https://doi.org/10.3390/photonics5030029	journal	September 2018
Enhanced Nonlinear Yield from Barium Titanate Metasurface Down to the Near Ultraviolet Timpu, Flavia; Reig Escalé, Marc; Timofeeva, Maria ETH Zurich https://doi.org/10.3929/ethz-b-000366859	text	January 2019
Fano Resonance in a Subwavelength Mie-based Metamolecule with Split Ring Resonator Wang, Xiaobo; Zhou, Ji arXiv https://doi.org/10.48550/arxiv.1704.02758	text	January 2017
Thermal tuning capabilities of semiconductor metasurface resonators Lewi, Tomer; Butakov, Nikita A.; Schuller, Jon A. arXiv https://doi.org/10.48550/arxiv.1802.09664	preprint	January 2018
Accelerating Light with Metasurfaces Henstridge, Meredith; Pfeiffer, Carl; Wang, Di arXiv https://doi.org/10.48550/arxiv.1803.01769	preprint	January 2018
All-dielectric metasurfaces with trapped modes: group-theoretical description Yu, Pengchao; Kupriianov, Anton S.; Dmitriev, Victor arXiv https://doi.org/10.48550/arxiv.1812.10817	text	January 2018

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