Prediction of an arc-tunable Weyl Fermion metallic state in MoxW1-xTe2

Chang, Tay-Rong; Xu, Su-Yang; Chang, Guoqing; Lee, Chi-Cheng; Huang, Shin-Ming; Wang, BaoKai; Bian, Guang; Zheng, Hao; Sanchez, Daniel S.; Belopolski, Ilya; Alidoust, Nasser; Neupane, Madhab; Bansil, Arun; Jeng, Horng-Tay; Lin, Hsin; Zahid Hasan, M.

doi:10.1038/ncomms10639

Prediction of an arc-tunable Weyl Fermion metallic state in Mo_xW_1-xTe₂

Journal Article · Mon Feb 15 00:00:00 EST 2016 · Nature Communications

DOI:https://doi.org/10.1038/ncomms10639· OSTI ID:1259283

Chang, Tay-Rong ^[1]; Xu, Su-Yang ^[2]; ^[3]; Lee, Chi-Cheng ^[3]; ^[3]; ^[4]; Bian, Guang ^[2]; ^[2]; Sanchez, Daniel S. ^[2]; Belopolski, Ilya ^[2]; Alidoust, Nasser ^[2]; Neupane, Madhab ^[5]; Bansil, Arun ^[6]; Jeng, Horng-Tay ^[7]; Lin, Hsin ^[3]; ^[8]

National Tsing Hua Univ., Hsinchu (Taiwan)
Princeton Univ., NJ (United States). Dept.of Physics
National Univ. of Singapore (Singapore)
National Univ. of Singapore (Singapore); Northeastern Univ., Boston, MA (United States)
Princeton Univ., NJ (United States). Dept.of Physics; Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Northeastern Univ., Boston, MA (United States)
National Tsing Hua Univ., Hsinchu (Taiwan); Academia Sinica, Taipei (Taiwan)
Princeton Univ., NJ (United States). Dept.of Physics; Princeton Univ., NJ (United States). Princeton Institute for the Science and Technology of Materials

A Weyl semimetal is a new state of matter that hosts Weyl fermions as emergent quasiparticles. The Weyl fermions correspond to isolated points of bulk band degeneracy, Weyl nodes, which are connected only through the crystal’s boundary by exotic Fermi arcs. The length of the Fermi arc gives a measure of the topological strength, because the only way to destroy the Weyl nodes is to annihilate them in pairs in the reciprocal space. To date, Weyl semimetals are only realized in the TaAs class. Here, we propose a tunable Weyl state in Mo_xW_1₋xTe₂ where Weyl nodes are formed by touching points between metallic pockets. We show that the Fermi arc length can be changed as a function of Mo concentration, thus tuning the topological strength. Lastly,our results provide an experimentally feasible route to realizing Weyl physics in the layered compound Mo_xW_1₋xTe₂, where non-saturating magneto-resistance and pressure-driven superconductivity have been observed.

View Accepted Manuscript (DOE)

Research Organization:: Los Alamos National Lab. (LANL), Los Alamos, NM (United States); Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: National Research Foundation (NRF) Singapore; USDOE; USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22)

Grant/Contract Number:: AC02-05CH11231; AC52-06NA25396; FG02-05ER46200; FG02-07ER46352

OSTI ID:: 1259283

Alternate ID(s):: OSTI ID: 1409766

Report Number(s):: LA-UR--17-22173; ncomms10639

Journal Information:: Nature Communications, Journal Name: Nature Communications Vol. 7; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United States

Language:: English

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Dirac–Weyl semimetal phase in noncentrosymmetric transition metal monochalcogenides MoTe and WTe Meng, Lijun; Wu, Jiafang; Li, Yizhi Journal of Materials Chemistry C, Vol. 7, Issue 39 https://doi.org/10.1039/c9tc03339d	journal	January 2019
Highly anisotropic type-II nodal line state in pure titanium metal Zhang, Xiaoming; Jin, Lei; Dai, Xuefang Applied Physics Letters, Vol. 112, Issue 12 https://doi.org/10.1063/1.5023320	journal	March 2018
Magneto-conductivity of tilted type-I Weyl semimetals with different types of impurities Shao, Jianmei; Yan, Lijuan AIP Advances, Vol. 9, Issue 4 https://doi.org/10.1063/1.5091852	journal	April 2019
Quantum transport in Dirac and Weyl semimetals: a review Wang, Shuo; Lin, Ben-Chuan; Wang, An-Qi Advances in Physics: X, Vol. 2, Issue 3 https://doi.org/10.1080/23746149.2017.1327329	journal	May 2017
Quasiparticle interference on type-I and type-II Weyl semimetal surfaces: a review Zheng, Hao; Zahid Hasan, M. Advances in Physics: X, Vol. 3, Issue 1 https://doi.org/10.1080/23746149.2018.1466661	journal	January 2018
Broken cubic symmetry driven co-emergence of type-I and type-II Dirac points in topological crystalline insulator ThTaN ₃ Tian, Xin; Shi, Xianbiao; He, Peng Journal of Physics: Condensed Matter, Vol. 31, Issue 29 https://doi.org/10.1088/1361-648x/ab17a2	journal	May 2019
Interplay between magnetic, metal/insulator and topological phases in Hg _{1− x} Mn _x Te alloys: prediction of a ferromagnetic Weyl semimetal at x = 0.25 Silveira, Orlando J.; de Carvalho, Luiz C.; Alves, Horacio W. L. Journal of Physics: Condensed Matter, Vol. 31, Issue 43 https://doi.org/10.1088/1361-648x/ab3270	journal	July 2019
Tuning the electrical transport of type II Weyl semimetal WTe ₂ nanodevices by Mo doping Fu, Dongzhi; Pan, Xingchen; Bai, Zhanbin Nanotechnology, Vol. 29, Issue 13 https://doi.org/10.1088/1361-6528/aaa811	journal	February 2018
Type-II nodal line semimetal He, Jing; Kong, Xiao; Wang, Wei New Journal of Physics, Vol. 20, Issue 5 https://doi.org/10.1088/1367-2630/aabdf8	journal	May 2018
Giant enhancement of superconductivity in few layers MoTe ₂ Gan, Yuan; Cho, Chang-Woo; Li, Alei Chinese Physics B, Vol. 28, Issue 11 https://doi.org/10.1088/1674-1056/ab457f	journal	October 2019
Effect of aging-induced disorder on the quantum transport properties of few-layer WTe ₂ Liu, Wei Lai; Chen, Mao Lin; Li, Xiao Xi 2D Materials, Vol. 4, Issue 1 https://doi.org/10.1088/2053-1583/4/1/011011	journal	December 2016
The structural phases and vibrational properties of Mo _1−x W _x Te ₂ alloys Oliver, Sean M.; Beams, Ryan; Krylyuk, Sergiy 2D Materials, Vol. 4, Issue 4 https://doi.org/10.1088/2053-1583/aa7a32	journal	August 2017
Type-II Weyl points in three-dimensional cold-atom optical lattices Xu, Yong; Duan, L. -M. Physical Review A, Vol. 94, Issue 5 https://doi.org/10.1103/physreva.94.053619	journal	November 2016
Ideal type-II Weyl phonons in wurtzite CuI Liu, Jian; Hou, Wenjie; Wang, En Physical Review B, Vol. 100, Issue 8 https://doi.org/10.1103/physrevb.100.081204	journal	August 2019
Berry curvature induced thermopower in type-I and type-II Weyl semimetals Das, Kamal; Agarwal, Amit Physical Review B, Vol. 100, Issue 8 https://doi.org/10.1103/physrevb.100.085406	journal	August 2019
Giant optical activity and Kerr effect in type-I and type-II Weyl semimetals Sonowal, Kabyashree; Singh, Ashutosh; Agarwal, Amit Physical Review B, Vol. 100, Issue 8 https://doi.org/10.1103/physrevb.100.085436	journal	August 2019
Weyl semimetal phase in the noncentrosymmetric superlattice W 2 X Y ( X , Y = S , Se , Te , X ≠ Y ) Meng, Lijun; Wu, Jiafang; Li, Yizhi Physical Review B, Vol. 100, Issue 15 https://doi.org/10.1103/physrevb.100.155151	journal	October 2019
Asymmetric mass acquisition in LaBi: Topological semimetal candidate Wu, Yun; Kong, Tai; Wang, Lin-Lin Physical Review B, Vol. 94, Issue 8 https://doi.org/10.1103/physrevb.94.081108	journal	August 2016
Electronic excitation-induced semiconductor-to-metal transition in monolayer MoTe 2 Kolobov, A. V.; Fons, P.; Tominaga, J. Physical Review B, Vol. 94, Issue 9 https://doi.org/10.1103/physrevb.94.094114	journal	September 2016
Hall effect within the colossal magnetoresistive semimetallic state of MoTe 2 Zhou, Qiong; Rhodes, D.; Zhang, Q. R. Physical Review B, Vol. 94, Issue 12 https://doi.org/10.1103/physrevb.94.121101	journal	September 2016
Type-II Weyl cone transitions in driven semimetals Chan, Ching-Kit; Oh, Yun-Tak; Han, Jung Hoon Physical Review B, Vol. 94, Issue 12 https://doi.org/10.1103/physrevb.94.121106	journal	September 2016
Observation of Fermi arcs in the type-II Weyl semimetal candidate WTe 2 Wu, Yun; Mou, Daixiang; Jo, Na Hyun Physical Review B, Vol. 94, Issue 12 https://doi.org/10.1103/physrevb.94.121113	journal	September 2016
Type-II Dirac fermions in the PtSe 2 class of transition metal dichalcogenides Huang, Huaqing; Zhou, Shuyun; Duan, Wenhui Physical Review B, Vol. 94, Issue 12 https://doi.org/10.1103/physrevb.94.121117	journal	September 2016
Observation of Fermi arc and its connection with bulk states in the candidate type-II Weyl semimetal WTe 2 Wang, Chenlu; Zhang, Yan; Huang, Jianwei Physical Review B, Vol. 94, Issue 24 https://doi.org/10.1103/physrevb.94.241119	journal	December 2016
Persistence of a surface state arc in the topologically trivial phase of MoTe 2 Crepaldi, A.; Autès, G.; Sterzi, A. Physical Review B, Vol. 95, Issue 4 https://doi.org/10.1103/physrevb.95.041408	journal	January 2017
Minimal models for topological Weyl semimetals McCormick, Timothy M.; Kimchi, Itamar; Trivedi, Nandini Physical Review B, Vol. 95, Issue 7 https://doi.org/10.1103/physrevb.95.075133	journal	February 2017
Anticorrelation between polar lattice instability and superconductivity in the Weyl semimetal candidate MoTe 2 Takahashi, H.; Akiba, T.; Imura, K. Physical Review B, Vol. 95, Issue 10 https://doi.org/10.1103/physrevb.95.100501	journal	March 2017
Observation of spin-polarized bands and domain-dependent Fermi arcs in polar Weyl semimetal MoT e 2 Sakano, M.; Bahramy, M. S.; Tsuji, H. Physical Review B, Vol. 95, Issue 12 https://doi.org/10.1103/physrevb.95.121101	journal	March 2017
Origins of the structural phase transitions in MoTe 2 and WTe 2 Kim, Hyun-Jung; Kang, Seoung-Hun; Hamada, Ikutaro Physical Review B, Vol. 95, Issue 18 https://doi.org/10.1103/physrevb.95.180101	journal	May 2017
Experimental evidence for type-II Dirac semimetal in PtSe 2 Zhang, Kenan; Yan, Mingzhe; Zhang, Haoxiong Physical Review B, Vol. 96, Issue 12 https://doi.org/10.1103/physrevb.96.125102	journal	September 2017
Quasiparticle interference of surface states in the type-II Weyl semimetal WTe 2 Zhang, Wenhan; Wu, Quansheng; Zhang, Lunyong Physical Review B, Vol. 96, Issue 16 https://doi.org/10.1103/physrevb.96.165125	journal	October 2017
Bulk Fermi surface of the Weyl type-II semimetallic candidate γ − MoTe 2 Rhodes, D.; Schönemann, R.; Aryal, N. Physical Review B, Vol. 96, Issue 16 https://doi.org/10.1103/physrevb.96.165134	journal	October 2017
Nodal-knot semimetals Bi, Ren; Yan, Zhongbo; Lu, Ling Physical Review B, Vol. 96, Issue 20 https://doi.org/10.1103/physrevb.96.201305	journal	November 2017
Enhanced ultrafast relaxation rate in the Weyl semimetal phase of MoTe 2 measured by time- and angle-resolved photoelectron spectroscopy Crepaldi, A.; Autès, G.; Gatti, G. Physical Review B, Vol. 96, Issue 24 https://doi.org/10.1103/physrevb.96.241408	journal	December 2017
Magnetic and noncentrosymmetric Weyl fermion semimetals in the R AlGe family of compounds ( R = rare earth ) Chang, Guoqing; Singh, Bahadur; Xu, Su-Yang Physical Review B, Vol. 97, Issue 4 https://doi.org/10.1103/physrevb.97.041104	journal	January 2018
Universal scattering response across the type-II Weyl semimetal phase diagram Rüßmann, P.; Weber, A. P.; Glott, F. Physical Review B, Vol. 97, Issue 7 https://doi.org/10.1103/physrevb.97.075106	journal	February 2018
Dynamics of out-of-equilibrium electron and hole pockets in the type-II Weyl semimetal candidate WTe 2 Caputo, M.; Khalil, L.; Papalazarou, E. Physical Review B, Vol. 97, Issue 11 https://doi.org/10.1103/physrevb.97.115115	journal	March 2018
Klein tunneling and electron optics in Dirac-Weyl fermion systems with tilted energy dispersion Nguyen, V. Hung; Charlier, J. -C. Physical Review B, Vol. 97, Issue 23 https://doi.org/10.1103/physrevb.97.235113	journal	June 2018
Topological surface Fermi arcs in the magnetic Weyl semimetal Co 3 Sn 2 S 2 Xu, Qiunan; Liu, Enke; Shi, Wujun Physical Review B, Vol. 97, Issue 23 https://doi.org/10.1103/physrevb.97.235416	journal	June 2018
Quantum oscillations in type-II Dirac semimetal PtTe 2 Fu, Dongzhi; Bo, Xiangyan; Fei, Fucong Physical Review B, Vol. 97, Issue 24 https://doi.org/10.1103/physrevb.97.245109	journal	June 2018
Topological phase with a critical-type nodal line state in intermetallic CaPd Liu, Guodong; Jin, Lei; Dai, Xuefang Physical Review B, Vol. 98, Issue 7 https://doi.org/10.1103/physrevb.98.075157	journal	August 2018
Phase transition and electronic structure evolution of MoTe 2 induced by W substitution Jin, Wencan; Schiros, Theanne; Lin, Yi Physical Review B, Vol. 98, Issue 14 https://doi.org/10.1103/physrevb.98.144114	journal	October 2018
Importance of electron correlations in understanding photoelectron spectroscopy and Weyl character of MoTe 2 Aryal, Niraj; Manousakis, Efstratios Physical Review B, Vol. 99, Issue 3 https://doi.org/10.1103/physrevb.99.035123	journal	January 2019
MoTe 2 : A Type-II Weyl Topological Metal Wang, Zhijun; Gresch, Dominik; Soluyanov, Alexey A. Physical Review Letters, Vol. 117, Issue 5 https://doi.org/10.1103/physrevlett.117.056805	journal	July 2016
Robust Type-II Weyl Semimetal Phase in Transition Metal Diphosphides X P 2 ( X = Mo , W) Autès, G.; Gresch, D.; Troyer, M. Physical Review Letters, Vol. 117, Issue 6 https://doi.org/10.1103/physrevlett.117.066402	journal	August 2016
Field-Selective Anomaly and Chiral Mode Reversal in Type-II Weyl Materials Udagawa, M.; Bergholtz, E. J. Physical Review Letters, Vol. 117, Issue 8 https://doi.org/10.1103/physrevlett.117.086401	journal	August 2016
Atomic-Scale Visualization of Quasiparticle Interference on a Type-II Weyl Semimetal Surface Zheng, Hao; Bian, Guang; Chang, Guoqing Physical Review Letters, Vol. 117, Issue 26 https://doi.org/10.1103/physrevlett.117.266804	journal	December 2016
Experimental Observation of Anisotropic Adler-Bell-Jackiw Anomaly in Type-II Weyl Semimetal WTe 1.98 Crystals at the Quasiclassical Regime Lv, Yang-Yang; Li, Xiao; Zhang, Bin-Bin Physical Review Letters, Vol. 118, Issue 9 https://doi.org/10.1103/physrevlett.118.096603	journal	March 2017
Type-II Symmetry-Protected Topological Dirac Semimetals Chang, Tay-Rong; Xu, Su-Yang; Sanchez, Daniel S. Physical Review Letters, Vol. 119, Issue 2 https://doi.org/10.1103/physrevlett.119.026404	journal	July 2017
Multiple Types of Topological Fermions in Transition Metal Silicides Tang, Peizhe; Zhou, Quan; Zhang, Shou-Cheng Physical Review Letters, Vol. 119, Issue 20 https://doi.org/10.1103/physrevlett.119.206402	journal	November 2017
Low-energy excitations in type-II Weyl semimetal T d − MoTe 2 evidenced through optical conductivity Santos-Cottin, D.; Martino, E.; Le Mardelé, F. Physical Review Materials, Vol. 4, Issue 2 https://doi.org/10.1103/physrevmaterials.4.021201	journal	February 2020
Fermi Arcs and Their Topological Character in the Candidate Type-II Weyl Semimetal MoTe 2 Tamai, A.; Wu, Q. S.; Cucchi, I. Physical Review X, Vol. 6, Issue 3 https://doi.org/10.1103/physrevx.6.031021	journal	August 2016
Optical Interface States Protected by Synthetic Weyl Points Wang, Qiang; Xiao, Meng; Liu, Hui Physical Review X, Vol. 7, Issue 3 https://doi.org/10.1103/physrevx.7.031032	journal	August 2017
Light-Induced Subpicosecond Lattice Symmetry Switch in MoTe 2 Zhang, M. Y.; Wang, Z. X.; Li, Y. N. Physical Review X, Vol. 9, Issue 2 https://doi.org/10.1103/physrevx.9.021036	journal	May 2019
Weyl and Dirac semimetals in three-dimensional solids Armitage, N. P.; Mele, E. J.; Vishwanath, Ashvin Reviews of Modern Physics, Vol. 90, Issue 1 https://doi.org/10.1103/revmodphys.90.015001	journal	January 2018
Critical enhancement of thermopower in a chemically tuned polar semimetal MoTe ₂ Sakai, Hideaki; Ikeura, Koji; Bahramy, Mohammad Saeed Science Advances, Vol. 2, Issue 11 https://doi.org/10.1126/sciadv.1601378	journal	November 2016
Quasiparticle interference evidence of the topological Fermi arc states in chiral fermionic semimetal CoSi Yuan, Qian-Qian; Zhou, Liqin; Rao, Zhi-Cheng Science Advances, Vol. 5, Issue 12 https://doi.org/10.1126/sciadv.aaw9485	journal	December 2019
A Scanning Tunneling Microscopy Study of Monolayer and Bilayer Transition-Metal Dichalcogenides Grown by Molecular-Beam Epitaxy Xie, Maohai; Chen, Jinglei Surface Review and Letters, Vol. 25, Issue Supp01 https://doi.org/10.1142/s0218625x18410020	journal	December 2018
Type-II Weyl cone transitions in driven semimetals Chan, Ching-Kit; Oh, Yun-Tak; Han, Jung Hoon arXiv https://doi.org/10.48550/arxiv.1605.05696	text	January 2016
Raman signatures of inversion symmetry breaking and structural phase transition in type-II Weyl semimetal MoTe2 Zhang, Kenan; Bao, Changhua; Gu, Qiangqiang arXiv https://doi.org/10.48550/arxiv.1606.05071	text	January 2016
Lorentz-violating type-II Dirac fermions in transition metal dichalcogenide PtTe$_2$ Yan, Mingzhe; Huang, Huaqing; Zhang, Kenan arXiv https://doi.org/10.48550/arxiv.1607.03643	text	January 2016
Type-II Weyl Points in Three-Dimensional Cold Atom Optical Lattices Xu, Yong; Duan, L. -M. arXiv https://doi.org/10.48550/arxiv.1607.04924	text	January 2016
Critical enhancement of thermopower in a chemically tuned polar semimetal MoTe$_{\bf 2}$ Sakai, H.; Ikeura, K.; Bahramy, M. S. arXiv https://doi.org/10.48550/arxiv.1703.04129	text	January 2017
Nodal-knot semimetals Bi, Ren; Yan, Zhongbo; Lu, Ling arXiv https://doi.org/10.48550/arxiv.1704.06849	text	January 2017
Weyl and Dirac Semimetals in Three Dimensional Solids Armitage, N. P.; Mele, E. J.; Vishwanath, Ashvin arXiv https://doi.org/10.48550/arxiv.1705.01111	text	January 2017
Electrically tunable valley polarization in Weyl semimetals with tilted energy dispersion Yesilyurt, Can; Siu, Zhuo Bin; Tan, Seng Ghee arXiv https://doi.org/10.48550/arxiv.1705.07067	preprint	January 2017
Multiple types of topological fermions in transition metal silicides Tang, Peizhe; Zhou, Quan; Zhang, Shou-Cheng arXiv https://doi.org/10.48550/arxiv.1706.03817	text	January 2017
Quasiparticle interference on type-I and type-II Weyl semimetal surfaces: a review Zheng, Hao; Hasan, M. Zahid arXiv https://doi.org/10.48550/arxiv.1805.10590	text	January 2018
Low-energy excitations in type-II Weyl semimetal Td−MoTe2 evidenced through optical conductivity David, Santos-Cottin,; Edoardo, Martino,; Florian, Le Mardelé, American Physical Society https://doi.org/10.5167/uzh-199086	text	January 2020

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