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Title: Quantum oscillations in a two-dimensional electron gas at the rocksalt/zincblende interface of PbTe/CdTe (111) heterostructures

Journal Article · · Nano Letters
 [1];  [2];  [3];  [1];  [1];  [4];  [4];  [1];  [1];  [2];  [3]
  1. Zhejiang Univ., Zhejiang (China)
  2. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
  3. Univ. of North Carolina at Charlotte, Charlotte, NC (United States)
  4. Los Alamos National Lab. (LANL), Los Alamos, NM (United States)

Here, quantum oscillations are observed in the 2DEG system at the interface of novel heterostructures, PbTe/CdTe (111), with nearly identical lattice parameters (aPbTe = 0.6462 nm, aCdTe = 0.648 nm) but very different lattice structures (PbTe: rock salt, CdTe: zinc blende). The 2DEG formation mechanism, a mismatch in the bonding configurations of the valence electrons at the interface, is uniquely different from the other known 2DEG systems. The aberration-corrected scanning transmission electron microscope (AC-STEM) characterization indicates an abrupt interface without cation interdiffusion due to a large miscibility gap between the two constituent materials. Electronic transport measurements under magnetic field up to 60 T, with the observation of Landau level filling factor ν = 1, unambiguously reveal a π Berry phase, suggesting the Dirac Fermion nature of the 2DEG at the heterostructure interface, and the PbTe/CdTe heterostructure being a new candidate for 2D topological crystalline insulators.

Research Organization:
Sandia National Lab. (SNL-NM), Albuquerque, NM (United States); Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA); National Science Foundation (NSF)
Grant/Contract Number:
AC04-94AL85000; AC52-06NA25396
OSTI ID:
1235338
Alternate ID(s):
OSTI ID: 1321762
Report Number(s):
SAND-2015-7566J; LA-UR-15-24704; 603526
Journal Information:
Nano Letters, Vol. 15, Issue 7; ISSN 1530-6984
Publisher:
American Chemical SocietyCopyright Statement
Country of Publication:
United States
Language:
English
Citation Metrics:
Cited by: 21 works
Citation information provided by
Web of Science

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Cited By (3)

Ultrahigh‐Detectivity Photodetectors with Van der Waals Epitaxial CdTe Single‐Crystalline Films journal April 2019
Realization of a New Topological Crystalline Insulator and Lifshitz Transition in PbTe journal July 2018
Electric‐Field Control of Dirac Two‐Dimensional Electron Gas in PbTe/CdTe Heterostructures journal January 2019