In-situ study of crystallization kinetics in ternary bulk metallic glass alloys with different glass forming abilities

Lan, Si; Wei, Xiaoya; Zhou, Jie; Lu, Zhaoping; Wu, Xuelian; Feygenson, Mikhail; Neuefeind, Jorg C.; Wang, Xun-Li

doi:10.1063/1.4901905

Title: In-situ study of crystallization kinetics in ternary bulk metallic glass alloys with different glass forming abilities

Journal Article · Tue Nov 18 00:00:00 EST 2014 · Applied Physics Letters

DOI:https://doi.org/10.1063/1.4901905· OSTI ID:1286812

Lan, Si ^[1]; Wei, Xiaoya ^[1]; Zhou, Jie ^[2]; Lu, Zhaoping ^[2]; Wu, Xuelian ^[1]; Feygenson, Mikhail ^[3]; Neuefeind, Jorg C. ^[3]; Wang, Xun-Li ^[1]

City Univ. of Hong Kong (China)
State Key Laboratory for Advanced Metals and Materials, University of Science and Technology Beijing (China)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

In-situ transmission electron microcopy and time-resolved neutron diffraction were used to study crystalline kinetics of two ternary bulk metallic glass alloys during isothermal annealing in the supercooled liquid region. It is found that the crystallization of Zr₅₆Cu₃₆Al₈, an average glass former, follows continuous nucleation and growth, while that of Zr₄₆Cu₄₆Al₈, a better glass former, is characterized by site-saturated nucleation, followed by slow growth. In conclusion, possible mechanisms for the observed differences and the relationship to the glass forming ability are discussed.

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Research Organization:: Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Spallation Neutron Source (SNS)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1286812

Alternate ID(s):: OSTI ID: 1224304; OSTI ID: 1330512

Journal Information:: Applied Physics Letters, Vol. 105, Issue 20; ISSN 0003-6951

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 28 works

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A high temperature gas flow environment for neutron total scattering studies of complex materials Olds, Daniel; Mills, Rebecca A.; McDonnell, Marshall T. Review of Scientific Instruments, Vol. 89, Issue 9 https://doi.org/10.1063/1.5033464	journal	September 2018
A suite-level review of the neutron powder diffraction instruments at Oak Ridge National Laboratory Calder, S.; An, K.; Boehler, R. Review of Scientific Instruments, Vol. 89, Issue 9 https://doi.org/10.1063/1.5033906	journal	September 2018
Elucidating the nature of crystallization kinetics in Zr ₄₆ Cu ₄₆ Al ₈ metallic glass through simultaneous WAXS/SAXS measurements Wu, Xuelian; Lan, Si; Wei, Xiaoya Applied Physics Letters, Vol. 114, Issue 21 https://doi.org/10.1063/1.5088984	journal	May 2019
From Rate Measurements to Mechanistic Data for Condensed Matter Reactions: A Case Study Using the Crystallization of [Zn(OH2)6][ZnCl4] Hillis, Berkley; Losey, Bradley; Weng, James Crystals, Vol. 7, Issue 1 https://doi.org/10.3390/cryst7010011	journal	December 2016

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