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Ion beam modification of topological insulator bismuth selenide

Journal Article · · Applied Physics Letters
DOI:https://doi.org/10.1063/1.4904936· OSTI ID:1184484
 [1];  [1];  [2];  [1];  [2];  [1];  [2];  [2];  [3];  [3];  [3]
  1. Sandia National Lab. (SNL-NM), Albuquerque, NM (United States)
  2. Sandia National Lab. (SNL-CA), Livermore, CA (United States)
  3. The State Univ. of New Jersey, Piscataway, NJ (United States)
In this study, we demonstrate chemical doping of a topological insulator Bi2Se3 using ion implantation. Ion beam-induced structural damage was characterized using grazing incidence X-ray diffraction and transmission electron microscopy. Ion damage was reversed using a simple thermal annealing step. Carrier-type conversion was achieved using ion implantation followed by an activation anneal in Bi2Se3 thin films. These two sets of experiments establish the feasibility of ion implantation for chemical modification of Bi2Se3, a prototypical topological insulator. Ion implantation can, in principle, be used for any topological insulator. The direct implantation of dopants should allow better control over carrier concentrations for the purposes of achieving low bulk conductivity. Ion implantation also enables the fabrication of inhomogeneously doped structures, which in turn should make possible new types of device designs.
Research Organization:
Sandia National Laboratories (SNL-NM), Albuquerque, NM (United States); Sandia National Laboratories, Livermore, CA (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA)
Grant/Contract Number:
AC04-94AL85000
OSTI ID:
1184484
Alternate ID(s):
OSTI ID: 22395532
Report Number(s):
SAND--2014-18593J; 540398
Journal Information:
Applied Physics Letters, Journal Name: Applied Physics Letters Journal Issue: 24 Vol. 105; ISSN APPLAB; ISSN 0003-6951
Publisher:
American Institute of Physics (AIP)Copyright Statement
Country of Publication:
United States
Language:
English

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Cited By (9)

Surface modification of multilayer FePS3 by Ga ion irradiation journal October 2019
Metallic edge states in zig-zag vertically-oriented MoS2 nanowalls preprint January 2019
Materials analysis and focused ion beam nanofabrication of topological insulator Bi2Se3 journal October 2017
Two-dimensional transition metal dichalcogenide-based counter electrodes for dye-sensitized solar cells journal January 2017
Ion beam modification of two-dimensional materials: Characterization, properties, and applications journal March 2017
Enhanced sputter yields of ion irradiated Au nano particles: energy and size dependence journal July 2015
Modification and Control of Topological Insulator Surface States Using Surface Disorder journal June 2015
Modification and Control of Topological Insulator Surface States Using Surface Disorder text January 2014
Materials analysis and focused ion beam nanofabrication of topological insulator Bi2Se3 text January 2017

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