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Measurement of the effects of shape resonances on vibrational intensity distribution in molecular photoionization

Technical Report ·
DOI:https://doi.org/10.2172/1178327· OSTI ID:1178327
 [1];  [1];  [1];  [2];  [1];  [3]
  1. National Bureau of Standards, Washington, DC (United States), National Measurement Lab.
  2. Daresbury Lab., Warrington (United Kingdom)
  3. Argonne National Laboratory (ANL), Argonne, IL (United States)
We report striking non-Franck-Condon vibrational intensity distributions associated with the shape resonance in the 5σ photoionization channel of CO. This example confirms the recent theoretical prediction that shape resonances are very sensitive to internuclear separation, leading to different resonance energies and profiles, and non-Franck-Condon intensities in alternative vibrational channels.
Research Organization:
Argonne National Laboratory (ANL), Argonne, IL (United States)
Sponsoring Organization:
USDOE
DOE Contract Number:
W-31109-ENG-38
OSTI ID:
1178327
Report Number(s):
ANL--79-65-Pt.1
Country of Publication:
United States
Language:
English

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