5f delocalization-induced suppression of quadrupolar order in U(Pd1-xPtx)₃

Walker, H. C.; Le, M. D.; McEwen, K. A.; Bleckmann, M.; Süllow, S.; Mazzoli, C.; Wilkins, S. B.; Fort, D.

doi:10.1103/PhysRevB.84.235142

Title: 5f delocalization-induced suppression of quadrupolar order in U(Pd_1-xPt_x)₃

Journal Article · Tue Dec 27 00:00:00 EST 2011 · Physical Review. B, Condensed Matter and Materials Physics

DOI:https://doi.org/10.1103/PhysRevB.84.235142· OSTI ID:1098489

Walker, H. C.; Le, M. D.; McEwen, K. A.; Bleckmann, M.; Süllow, S.; Mazzoli, C.; Wilkins, S. B.; Fort, D.

We present bulk magnetic and transport measurements and x-ray resonant scattering measurements on U(Pd_1-xPt_x)₃ for x=0.005 and 0.01, which demonstrate the high sensitivity of the quadrupolar order in the canonical antiferroquadrupolar ordered system UPd₃ to doping with platinum. Bulk measurements for x=0.005 reveal behavior similar to that seen in UPd₃, albeit at a lower temperature, and x-ray resonant scattering provides evidence of quadrupolar order described by the Q_xy order parameter. In contrast, bulk measurements reveal only an indistinct transition in x=0.01, consistent with the observation of short-range quadrupolar order in our x-ray resonant scattering results.

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Sponsoring Organization:: USDOE

OSTI ID:: 1098489

Journal Information:: Physical Review. B, Condensed Matter and Materials Physics, Journal Name: Physical Review. B, Condensed Matter and Materials Physics Vol. 84 Journal Issue: 23; ISSN 1098-0121

Publisher:: American Physical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 6 works

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References (24)

Quadrupolar Phase Diagram and Fermi Surface Properties in the Localized 5 f ² -Electron System UPd ₃ Tokiwa, Yoshihumi; Sugiyama, Kiyohiro; Takeuchi, Tetuya Journal of the Physical Society of Japan, Vol. 70, Issue 6 https://doi.org/10.1143/JPSJ.70.1731	journal	June 2001
ID20: a beamline for magnetic and resonant X-ray scattering investigations under extreme conditions Paolasini, L.; Detlefs, C.; Mazzoli, C. Journal of Synchrotron Radiation, Vol. 14, Issue 4 https://doi.org/10.1107/S0909049507024879	journal	June 2007
A tri-arc system for growing high-purity crystals of metallic materials Fort, D. Review of Scientific Instruments, Vol. 68, Issue 9 https://doi.org/10.1063/1.1148314	journal	September 1997
$5 f$ Electron Localization-Delocalization Transition from ${UPd}_{3}$ to ${UPt}_{3}$ Petit, L.; Svane, A.; Temmerman, W. M. Physical Review Letters, Vol. 88, Issue 21 https://doi.org/10.1103/PhysRevLett.88.216403	journal	May 2002
Magnetic and electrical properties of dhcp $Np {Pd}_{3}$ and $(U_{1 - x} {Np}_{x}) {Pd}_{3}$ Walker, H. C.; McEwen, K. A.; Boulet, P. Physical Review B, Vol. 76, Issue 17 https://doi.org/10.1103/PhysRevB.76.174437	journal	November 2007
Ultrasound investigations of orbital quadrupolar ordering in ${UPd}_{3}$ Lingg, N.; Maurer, D.; Müller, V. Physical Review B, Vol. 60, Issue 12 https://doi.org/10.1103/PhysRevB.60.R8430	journal	September 1999
Magnetic Quantum Critical Point and Superconductivity in ${UPt}_{3}$ Doped with Pd de Visser, A.; Graf, M. J.; Estrela, P. Physical Review Letters, Vol. 85, Issue 14 https://doi.org/10.1103/PhysRevLett.85.3005	journal	October 2000
UPt3, heavy fermions and superconductivity De Visser, A.; Menovsky, A.; Franse, J. J. M. Physica B+C, Vol. 147, Issue 1 https://doi.org/10.1016/0378-4363(87)90008-8	journal	November 1987
Determination of the Antiferroquadrupolar Order Parameters in ${UPd}_{3}$ Walker, H. C.; McEwen, K. A.; McMorrow, D. F. Physical Review Letters, Vol. 97, Issue 13 https://doi.org/10.1103/PhysRevLett.97.137203	journal	September 2006
Superconductivity in heavy-fermion ${U (P t, P d)}_{3}$ and its interplay with magnetism Keizer, R. J.; de Visser, A.; Graf, M. J. Physical Review B, Vol. 60, Issue 14 https://doi.org/10.1103/PhysRevB.60.10527	journal	October 1999
Polarization dependence of magnetic x-ray scattering Blume, M.; Gibbs, Doon Physical Review B, Vol. 37, Issue 4 https://doi.org/10.1103/PhysRevB.37.1779	journal	February 1988
Thermal expansion and magnetostriction of UPd3 and U(Pd1−xPtx)3 single crystals Zochowski, S. W.; McEwen, K. A. Physica B: Condensed Matter, Vol. 199-200 https://doi.org/10.1016/0921-4526(94)91855-4	journal	April 1994
X-Ray Resonant Scattering Study of the Quadrupolar Order in ${UPd}_{3}$ McMorrow, D. F.; McEwen, K. A.; Steigenberger, U. Physical Review Letters, Vol. 87, Issue 5 https://doi.org/10.1103/PhysRevLett.87.057201	journal	July 2001
X-ray resonant scattering determination of the antiferroquadrupolar ordering in UPd ₃ at low temperatures Walker, H. C.; McEwen, K. A.; Le, M. D. Journal of Physics: Condensed Matter, Vol. 20, Issue 39 https://doi.org/10.1088/0953-8984/20/39/395221	journal	September 2008
Suppression of spin fluctuations by alloying in UPt3 Stewart, G. R.; Giorgi, A. L. Journal of Low Temperature Physics, Vol. 59, Issue 1-2 https://doi.org/10.1007/BF00681511	journal	April 1985
Magnetic calorimetry and thermal expansion of UPd3 Zochowski, S. W.; de Podesta, M.; Lester, C. Physica B: Condensed Matter, Vol. 206-207 https://doi.org/10.1016/0921-4526(94)00499-L	journal	February 1995
Spin and phonon excitations in actinide systems Buyers, W. J. L.; Murray, A. F.; Holden, T. M. Physica B+C, Vol. 102, Issue 1-3 https://doi.org/10.1016/0378-4363(80)90176-X	journal	October 1980
The dual nature of 5f electrons and the origin of heavy fermions in U compounds Zwicknagl, G.; Fulde, P. Journal of Physics: Condensed Matter, Vol. 15, Issue 28 https://doi.org/10.1088/0953-8984/15/28/302	journal	July 2003
Understanding the quadrupolar structures of McEwen, K. A.; Walker, H. C.; Le, M. D. Journal of Magnetism and Magnetic Materials, Vol. 310, Issue 2 https://doi.org/10.1016/j.jmmm.2006.10.520	journal	March 2007
Magnetic susceptibility of single-crystal UPd3 McEwen, K. A.; Ellerby, M.; de Podesta, M. Journal of Magnetism and Magnetic Materials, Vol. 140-144 https://doi.org/10.1016/0304-8853(94)00607-5	journal	February 1995
A new model for the crystal field and the quadrupolar phase transitions of UPd ₃ McEwen, K. A.; Park, J-G; Gipson, A. J. Journal of Physics: Condensed Matter, Vol. 15, Issue 28 https://doi.org/10.1088/0953-8984/15/28/304	journal	July 2003
Possibility of Coexistence of Bulk Superconductivity and Spin Fluctuations in U ${Pt}_{3}$ Stewart, G. R.; Fisk, Z.; Willis, J. O. Physical Review Letters, Vol. 52, Issue 8 https://doi.org/10.1103/PhysRevLett.52.679	journal	February 1984
Resonant magnetic x-ray scattering in the antiferromagnet $Ce {({Fe}_{1 - x} {Co}_{x})}_{2}$ Paolasini, L.; Di Matteo, S.; Deen, P. P. Physical Review B, Vol. 77, Issue 9 https://doi.org/10.1103/PhysRevB.77.094433	journal	March 2008
Specific heat, susceptibility and high-field magnetisation experiments on heavy fermion UPt3 alloyed with Pd De Visser, A.; Klaasse, J. C. P.; Van Sprang, M. Physics Letters A, Vol. 113, Issue 9 https://doi.org/10.1016/0375-9601(86)90127-1	journal	January 1986

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