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Title: Neutron scattering study on the field-induced O{sub xy}-type antiferroquadrupolar ordering of the heavy-fermion superconductor PrOs{sub 4}Sb{sub 12}

Journal Article · · Physical Review. B, Condensed Matter and Materials Physics
;  [1];  [1]; ; ;  [2];  [3]
  1. Advanced Science Research Center, Japan Atomic Energy Agency, Tokai, Naka, Ibaraki 319-1195 (Japan)
  2. Department of Physics, Tokyo Metropolitan University, Hachioji, Tokyo 192-0397 (Japan)
  3. DRFMC-CEA, 38054 Grenoble (France)

Neutron scattering experiments have revealed a field-induced antiferroquadrupolar order parameter in the Pr-based heavy-fermion superconductor PrOs{sub 4}Sb{sub 12}. We observed the field-induced antiferromagnetic dipole moment with the propagation vector q=(100) for the applied field direction both H parallel [110] and [001]. For H parallel [110] at 8 T, it should be noted that the induced antiferromagnetic moment of 0.16(10) {mu}{sub B}/Pr orients parallel to the field within our experimental accuracy. This observation is strong evidence that the O{sub xy} electric quadrupole is the primary order parameter for H parallel [110]. A mean-field calculation, based on {gamma}{sub 1} singlet and {gamma}{sub 4}{sup (2)} excited triplet with the O{sub xy} quadrupolar interaction, reproduces the induced moment direction and its field response. These facts indicate the predominance of O{sub xy}-type antiferroquadrupolar interaction in PrOs{sub 4}Sb{sub 12}.

OSTI ID:
20976723
Journal Information:
Physical Review. B, Condensed Matter and Materials Physics, Vol. 75, Issue 9; Other Information: DOI: 10.1103/PhysRevB.75.094408; (c) 2007 The American Physical Society; Country of input: International Atomic Energy Agency (IAEA); ISSN 1098-0121
Country of Publication:
United States
Language:
English