Skip to main content
U.S. Department of Energy
Office of Scientific and Technical Information

Asymmetrical Self-assembly From Fluorinated and Sulfonated Block Copolymers in Aqueous Media

Journal Article · · Soft Matter
DOI:https://doi.org/10.1039/c1sm06040f· OSTI ID:1024269

Block copolymers of fluorinated isoprene and partially sulfonated styrene form novel tapered rods and ribbon-like micelles in aqueous media due to a distribution of sulfonation sites and a large Flory-Huggins interaction parameter. A combination of microscopy, light scattering, and simulation demonstrates the presence of these unique nanostructures. This study sheds light on the micellization behavior of amphiphilic block polymers by revealing a new mechanism of self-assembly.

Research Organization:
Oak Ridge National Laboratory (ORNL); Center for Nanophase Materials Sciences
Sponsoring Organization:
SC USDOE - Office of Science (SC)
DOE Contract Number:
AC05-00OR22725
OSTI ID:
1024269
Journal Information:
Soft Matter, Journal Name: Soft Matter Journal Issue: 18 Vol. 7; ISSN 1744-683X
Country of Publication:
United States
Language:
English

Similar Records

Aqueous Self‐Assembly of Cylindrical and Tapered Bottlebrush Block Copolymers
Journal Article · Fri Apr 25 00:00:00 EDT 2025 · Angewandte Chemie (International Edition) · OSTI ID:2573251

Understanding the ordering mechanisms of self-assembled nanostructures of block copolymers during zone annealing
Journal Article · Mon Mar 21 00:00:00 EDT 2016 · Journal of Chemical Physics · OSTI ID:22660825

Phase Behavior of Symmetric Sulfonated Block Copolymers
Journal Article · Thu Aug 21 00:00:00 EDT 2008 · Macromolecules · OSTI ID:1006689