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Grain boundary networks in high-performance, heteroepitaxial, YBCO films on polycrystalline, cube-textured metals

Journal Article · · Philosophical Magazine Letters
 [1];  [2];  [3];  [3]
  1. ORNL
  2. Washington State University
  3. Institute of Physics, Augsburg University, Augsburg, Germany

Grain boundaries (GBs) in high-temperature superconductors suppress the critical current density (Jc) dramatically [1-3]. The Jc drops exponentially when GB-misorientation exceeds 4 [3]. To reduce the number of high-angle GBs, fabrication of biaxially-textured, superconducting wires via epitaxial growth on cube-textured metals has been widely investigated [4-6]. Such wires have exhibited very high-Jc in applied magnetic fields despite having a majority of GBs with total misorientations greater than 4 . Here we show that GB networks in these wires have numerous GBs with out-of-plane misorientations > 4 and few boundaries having in-plane misorientations > 4 . The high performance can be explained if the Jc is determined primarily by in-plane misorientations. This supposition was confirmed by in-field transport measurements on artificially fabricated bicrystals of superconductors having only out-of-plane misorientations. Atomic resolution imaging of bicrystals with out-of-plane misorientations show that superconducting ab-planes are continuous across such GBs in contrast to GBs with in-plane misorientations.

Research Organization:
Oak Ridge National Laboratory (ORNL); Shared Research Equipment Collaborative Research Center
Sponsoring Organization:
OE USDOE - Office of Electric Transmission and Distribution
DOE Contract Number:
AC05-00OR22725
OSTI ID:
1010554
Journal Information:
Philosophical Magazine Letters, Journal Name: Philosophical Magazine Letters Journal Issue: 4 Vol. 91; ISSN 0950-0839
Country of Publication:
United States
Language:
English