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Title: Magnetic Tunnel Junctions Based on CrO2/SnO2 Epitaxial Bilayers

Journal Article · · Applied Physics Letters
DOI:https://doi.org/10.1063/1.2216109· OSTI ID:1003563

Magnetic tunnel junctions (MTJs) were fabricated using thin films of the half-metallic ferromagnet CrO2, employing semiconducting SnO2 tunnel barriers. Heteroepitaxial CrO2/SnO2 bilayers were grown on (100)-TiO2 substrates via chemical vapor deposition under atmospheric conditions. X-ray diffraction and transmission electron microscopy were used to confirm heteroepitaxy. A polycrystalline cobalt film forms the top magnetic electrode, yielding CrO2(001)/SnO2(001)/Co structures after patterning. Tunneling magnetoresistances (TMR) up to +14% at 5 K were observed. The sign of the TMR reverses for barrier thicknesses < 1nm, attributed to tunneling being dominated by Co-3d states at low thicknesses, and Co-4s states at larger thicknesses.

Research Organization:
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Sponsoring Organization:
USDOE Office of Science (SC)
DOE Contract Number:
DE-AC05-00OR22725
OSTI ID:
1003563
Journal Information:
Applied Physics Letters, Vol. 89, Issue 2; ISSN 0003-6951
Country of Publication:
United States
Language:
English