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High Resolution Electromechanical Imaging of Ferroelectric Materials in a Liquid Environment by Piezoresponse Force Microscopy

Journal Article · · Physical Review Letters

High-resolution imaging of ferroelectric materials using piezoresponse force microscopy (PFM) is demonstrated in an aqueous environment. The elimination of both long-range electrostatic forces and capillary interactions results in a localization of the ac field to the tip-surface junction and allows the tip-surface contact area to be controlled. This approach results in spatial resolutions approaching the limit of the intrinsic domain-wall width. Imaging at frequencies corresponding to high-order cantilever resonances minimizes the viscous damping and added mass effects on cantilever dynamics and allows sensitivities comparable to ambient conditions. PFM in liquids will provide novel opportunities for high-resolution studies of ferroelectric materials, imaging of soft polymer materials, and imaging of biological systems in physiological environments on, ultimately, the molecular level.

Research Organization:
Oak Ridge National Laboratory (ORNL)
Sponsoring Organization:
ORNL LDRD Seed-Money
DOE Contract Number:
AC05-00OR22725
OSTI ID:
1001698
Journal Information:
Physical Review Letters, Journal Name: Physical Review Letters Journal Issue: 23 Vol. 96; ISSN 1079-7114; ISSN 0031-9007
Country of Publication:
United States
Language:
English

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