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Luminescence Enhancement of CdTe Nanostructures in LaF3:Ce/CdTe Nanocomposites

Journal Article · · Journal of Applied Physics, 108(10):207-213
DOI:https://doi.org/10.1063/1.3506416· OSTI ID:1001133
Radiation detection demands new scintillators with high quantum efficiency, high energy resolution and short luminescence lifetimes. Nanocomposites consisting of quantum dots and Ce3+ doped nanophosphors may be able to meet these requirements. Here we report the luminescence of LaF3:Ce/CdTe nanocomposites which were synthesized by a wet chemistry method. In LaF3:Ce/CdTe nanocomposites the CdTe quantum dots are converted into nanowires, while in LaF3/CdTe nanocomposites no such conversion is observed. The CdTe luminescence in LaF3:Ce/CdTe nanocomposites is enhanced about 5 times, while in LaF3/CdTe nanocomposites no enhancement was observed. Energy transfer, light-re-absorption and surface passivation are likely the reasons for the luminescence enhancement.
Research Organization:
Pacific Northwest National Laboratory (PNNL), Richland, WA (US), Environmental Molecular Sciences Laboratory (EMSL)
Sponsoring Organization:
USDOE
DOE Contract Number:
AC05-76RL01830
OSTI ID:
1001133
Report Number(s):
PNNL-SA-74942; 30431; KP1704020
Journal Information:
Journal of Applied Physics, 108(10):207-213, Journal Name: Journal of Applied Physics, 108(10):207-213 Journal Issue: 10 Vol. 108; ISSN JAPIAU; ISSN 0021-8979
Country of Publication:
United States
Language:
English

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