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Electronic reconstruction at SrMnO{sub 3}-LaMnO{sub 3} superlattice interfaces.

Journal Article · · Physical Review Letters
We use resonant soft-x-ray scattering (RSXS) to study the electronic reconstruction at the interface between the Mott insulator LaMnO{sub 3} and the band insulator SrMnO{sub 3}. Superlattices of these two insulators were shown previously to have both ferromagnetism and metallic tendencies [Koida et al., Phys. Rev. B 66, 144418 (2002)]. By studying a judiciously chosen superlattice reflection, we show that the interface density of states exhibits a pronounced peak at the Fermi level, similar to that predicted in related titanate superlattices by Okamoto et al. [Phys. Rev. B 70, 241104(R) (2004)]. The intensity of this peak correlates with the conductivity and magnetization, suggesting it is the driver of metallic behavior. Our study demonstrates a general strategy for using RSXS to probe the electronic properties of heterostructure interfaces.
Research Organization:
Argonne National Laboratory (ANL)
Sponsoring Organization:
SC
DOE Contract Number:
AC02-06CH11357
OSTI ID:
1000686
Report Number(s):
ANL/MSD/JA-68694
Journal Information:
Physical Review Letters, Journal Name: Physical Review Letters Journal Issue: Nov. 2007 Vol. 99; ISSN 0031-9007
Country of Publication:
United States
Language:
ENGLISH

References (37)

Separating the causes of orbital ordering in LaSr 2 Mn 2 O 7 using resonant soft x-ray diffraction journal June 2006
Artificial charge-modulationin atomic-scale perovskite titanate superlattices journal September 2002
Neutron Diffraction Study of the Magnetic Properties of the Series of Perovskite-Type Compounds [ ( 1 − x ) La ,   x Ca ] Mn O 3 journal October 1955
Signatures of enhanced ordering temperatures in digital superlattices of (LaMnO3)m∕(SrMnO3)2m journal May 2007
Dynamical mean-field study of model double-exchange superlattices journal January 2006
Atomic-scale imaging of nanoengineered oxygen vacancy profiles in SrTiO3 journal August 2004
Symmetry of Multiferroicity in a Frustrated Magnet TbMn 2 O 5 journal April 2007
Effect of A -site cation ordering on the magnetoelectric properties in [ ( LaMnO 3 ) m / ( SrMnO 3 ) m ] n artificial superlattices journal October 2002
Spatial inhomogeneity and strong correlation physics: A dynamical mean-field study of a model Mott-insulator–band-insulator heterostructure journal December 2004
Dynamical mean-field study of model double-exchange superlattices journal January 2006
Controlled-valence properties of La 1 − x Sr x FeO 3 and La 1 − x Sr x MnO 3 studied by soft-x-ray absorption spectroscopy journal August 1992
Unraveling Orbital Ordering in L a 0.5 S r 1.5 M n O 4 journal February 2004
Effects of uniaxial strain in LaMnO 3 journal August 2001
Electrostatic modification of novel materials journal November 2006
Effects of uniaxial strain in LaMnO_3 text January 2000
Photoemission from Buried Interfaces in SrTiO 3 / LaTiO 3 Superlattices journal August 2006
Spatially modulated 'Mottness' in La2-xBaxCuO4 journal December 2005
Effect of A -site cation ordering on the magnetoelectric properties in [ ( LaMnO 3 ) m / ( SrMnO 3 ) m ] n artificial superlattices journal October 2002
Charge-Orbital Ordering and Verwey Transition in Magnetite Measured by Resonant Soft X-Ray Scattering journal March 2006
Symmetry of Multiferroicity in a Frustrated Magnet TbMn 2 O 5 journal April 2007
Novel Orbital Ordering Induced by Anisotropic Stress in a Manganite Thin Film journal January 2006
Soft X-Ray Resonant Diffraction Study of Magnetic and Orbital Correlations in a Manganite Near Half Doping journal June 2004
Spatially modulated "Mottness" in La2-xBaxCuO4 text January 2005
Neutron Diffraction Study of the Magnetic Properties of the Series of Perovskite-Type Compounds [ ( 1 − x ) La ,   x Ca ] Mn O 3 journal October 1955
Photoemission from Buried Interfaces in SrTiO 3 / LaTiO 3 Superlattices journal August 2006
Novel Orbital Ordering Induced by Anisotropic Stress in a Manganite Thin Film journal January 2006
Orbital and magnetic ordering in La 0.5 Sr 1.5 Mn O 4 studied by soft x-ray resonant scattering journal June 2005
Unraveling Orbital Ordering in L a 0.5 S r 1.5 M n O 4 journal February 2004
Separating the causes of orbital ordering in LaSr 2 Mn 2 O 7 using resonant soft x-ray diffraction journal June 2006
Charge-Orbital Ordering and Verwey Transition in Magnetite Measured by Resonant Soft X-Ray Scattering journal March 2006
Spatial inhomogeneity and strong correlation physics: A dynamical mean-field study of a model Mott-insulator–band-insulator heterostructure journal December 2004
Probing depth of soft x-ray absorption spectroscopy measured in total-electron-yield mode journal January 1992
A Structural Probe of the Doped Holes in Cuprate Superconductors journal July 2002
Electrostatic modification of novel materials journal November 2006
Orbital and magnetic ordering in La 0.5 Sr 1.5 Mn O 4 studied by soft x-ray resonant scattering journal June 2005
Soft X-Ray Resonant Diffraction Study of Magnetic and Orbital Correlations in a Manganite Near Half Doping journal June 2004
Controlled-valence properties of La 1 − x Sr x FeO 3 and La 1 − x Sr x MnO 3 studied by soft-x-ray absorption spectroscopy journal August 1992

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